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TRANSCRIPT
i
1 .......................................................................................................... 1
TF Kd
......................................................................................................................... 3
................................................................................................................. 3
.............................................. 5
2.2.1. TF ......................................... 5
2.2.1.1 .......................................... 5
2.2.1.2 ................................................................... 5
2.2.2. .................................................................. 6
TF
.......................................................................................................... 7
2.3.1. TF .................. 7
2.3.1.1. .............................................................................. 7
2.3.1.2. ..................................................................................... 7
2.3.1.3. ................................................................................. 7
2.3.1.4. ..................................................................................... 8
2.3.1.5. ................................................................................. 9
2.3.1.6. ............................................................................ 10
2.3.1.7. ....................................................................................... 11
2.3.1.8. 28 ....................................................... 12
2.3.2. 27 .......................................................... 12
2.3.3. TF
.................................................................................................... 12
................................................................... 14
2.4.1. ................................................................ 14
2.4.2. ............................................................................................. 14
2.4.3. .......................................................................................... 14
Kd ............................... 16
2.5.1. 30 .............................. 16
2.5.2. 30 ......................................... 17
2.5.3. 30˚C Kd-137Cs .................................................................... 17
2.5.4. 30˚C Kd-137Cs ..................................................... 17
.................. 18
ii
2.6.1. Cs ................................................................. 18
2.6.1.1. ..................................................................................... 18
2.6.1.2. Cs ..................................................... 18
2.6.2. Cs ...................................................................................... 19
2.6.2.1. ........................................................................................................ 19
2.6.2.2. .................................................................................................... 20
2.6.2.3. ................................................................................................ 20
2.6.2.4. Tag ............................................................................... 20
2.6.3. 137Cs ........................................................................................... 21
2.6.3.1. ....................................................... 21
2.6.3.2. 137Cs ..................................................... 21
2.6.3.3. .................................................................. 23
............................................................................................................... 25
2.7.1. TF ........................................................ 25
2.7.2. TF 25
2.7.3. TF .................................................. 26
2.7.4. ......................................... 26
2.7.5. Cs ...................... 26
.......................................................................................................................... 27
2- 1. ...................................................................................... 30
.......................... 59
............................................................................................................... 59
.......................................................................................................................... 60 14C ............................................................................... 61
3.2.1. 14CO214C .......................................... 61
3.2.1.1. 14C 14C .............................................. 61
3.2.1.2. 14C ........................................................... 62
3.2.2. .................................................................................................................. 63
.......................................................................................................................... 63
............................................................... 65
3.3.1. .......................................................... 65
3.3.2. ..................................................................... 66
3.3.3. ..................................................................... 67
3.3.4. .................................................................................................................. 67
.......................................................................................................................... 68
..................................................................................... 70
3.4.1. ................................................................. 70
3.4.1.1. .................................................................. 70
3.4.1.2. ......................................................................................... 71
iii
3.4.1.3. 14C ........... 71
3.4.2. .................................... 72
3.4.2.1. ............................................................................. 72
3.4.2.2. CO2 .................................................................. 75
3.4.3. ............................................... 75
3.4.3.1. ................................................................................. 76
3.4.3.2. .................................... 77
3.4.3.3. ................................................ 77
3.4.3.4. 14C ........................................................ 78
3.4.4. .................................................................................................................. 79
.......................................................................................................................... 79
............................................................................................................... 81
4 Pu, Am, Th Cl
.................................................................................................... 119
............................................................................................................. 119
Am ................................................................. 120
4.2.1. Am ........................................................ 120
4.2.1.1. ...................................................................................................... 121
4.2.1.2. Aridus-SF-ICP-MS ........................................................ 121
4.2.1.3. ...................................................................................................... 122
4.2.1.4. ............................................................................................................. 122
4.2.1.5. ....................................................................................... 122
4.2.1.6. .............................................................................................. 124
4.2.2. 241Am ................................................................................ 125
4.2.2.1. ...................................................................................................... 125
4.2.2.2. ...................................................................................................... 125
4.2.2.3. .......................................................................................... 125
........................................................................................................................ 127
Th ............................................................................................ 130
4.3.1. ............................................................................................................ 130
4.3.2. ............................................................................................................ 130
4.3.3. ............................................................................................................ 130
4.3.4. ................................................................................................. 131
........................................................................................................................ 132
.................................................................... 133
4.4.1. ............................................................................................................. 133
4.4.2. TMAH ...................................................... 133
4.4.3. TMAH ICP-MS ....................................................... 134
4.4.4. TF .............................................. 134
iv
4.4.5. ........................................................... 135
........................................................................................................................ 135
Pu - .............................................................. 136
4.5.1. ............................................................................................................ 136
4.5.2. ..................................................................................................... 136
4.5.2.1. ....................................................................................................... 136
4.5.2.2. ............................................................................................................... 136
4.5.2.3. Pu .................................................................................... 136
4.5.3. ................................................................................................. 137
4.5.3.1. Pu ................................................. 137
4.5.3.2. Pu ................................................................................................ 138
4.5.3.3. Pu - ............................................................................... 138
..................................................................................................................... 139
Pu, Am, Th Cl - .................... 141
4.6.1. ............................................................................................................ 141
4.6.2. .............................................................................. 141
4.6.3. IAEA TRS-472 .................................................................................... 142
........................................................................................................................ 143
................................................................................................................. 147
4.7.1. Am Cl .......................................................................... 147
4.7.1.1. Am ......................................................... 147
4.7.1.2. ................................................................................... 147
4.7.2. Th ............................................................................................... 147
4.7.3. Pu - ....................................................................... 148
5 ................................................................................................................. 171
............................................................................................................. 171
TF Kd
................................................................................................................. 172
5.2.1. TF ...................................................... 172
5.2.2. TF 172
5.2.3. TF ................................................ 173
5.2.4. Kd ............................ 173
5.2.5 Cs .................................... 173
........................ 175
5.3.1. 14C .......................................................................... 175
5.3.2. .......................................................... 175
5.3.3. ................................................................................ 175
Pu, Am, Th Cl
.......................................................................................................... 177
v
5.4.1 Am Cl ........................................................................... 177
5.4.1.1. Am ..................................................... 177
5.4.1.2. ........................................................................ 177
5.4.2. - ............................................................................... 177
.................................................. 179
..................................................... 181
28 .................. 182
.................................................................................................................................... 183
vi
vii
TF Kd
2.3-1 ........................................................................... 31
2.3-2 ....................................................... 31
2.3-3 ................................................................................... 32
2.3-4 ........................................................... 32
2.3-5 ....................................................................... 33
2.3-6 ........................................................... 35
2.3-7 28 ......................................... 37
2.3-8 14-18 26-28 ................................................................................................................ 37
2.3-9 28 ..................................................... 38
2.3-10 28 ............................................... 39
2.3-11 28 ....................................................... 40
2.3-12 27 ....................................... 41
2.3-13 27 ................................... 42
2.3-14 27 ........................... 43
2.4-1 - 2016 .............. 44
2.4-2 ........... 44
2.4-3 ................... 45
2.4-4 ....................... 45
2.5-1 ............................................................................... 46
2.5-2 Cs Kd 30˚C Kd ....................................... 46
2.6-1 137Cs ..... 47
2.6-2 Cs Tag: m2 kg-1 ................. 47
2.6-3 ................................................................................................... 47
2.6-4 ....................................................................................... 47
2.6-5 137Cs ..................................... 48
2.6-6 δ13C δ15N ......................................................................... 48
2s-1 2015 2016 .......................................... 48
2.2-1 Ni, Sr, Mo Pb .......................................... 49
2.4-1 .................................................................................................................... 50
2.4-2 Fe, Co, Ni, Cu, Zn Sr ........................................................................................................................ 50
2.5-1 1 30 Cs 3 7 30
viii
Kd pH ......................................................................................................... 51
2.5-2 10 23 30˚C Kd-137Cs .............................................. 52
2.5-3 10 23 30˚C Kd-137Cs ........... 52
2.6-1 137Cs ................................................................................................ 53
2.6-2 2012-2016 137CsTag, m2 kg-1 ...................................................................... 54
2.6-3 2011 11 2016 9 ...... 55
2.6-4 ............................................................................................... 55
2.6-5 137Cs ............................................................................................. 56
2.6-6 ........................................................................................................... 56
2.6-7 13C 15N .......................................................................... 57
2.6-8 ................................................... 57
2s-1 2015 2016 Air Soil 20cm ......... 58
2s-2 2015 2016 ........................................ 58
3.3-1 ............................................................... 83
3.3-2 .............................................................................. 83
3.4-1
.......................................................................................................... 84
3.4-2 14C ......................... 84
3.4-3 ....................................................... 85
3.4-4 1 ................................................ 86
3.4-5 1 ........................................ 86
3.4-6 2 ................................................ 87
3.4-7 2 ........................................ 87
3.4-8 3 ................................................ 88
3.4-9 3 ........................................ 88
3.4-10 4 .............................................. 89
3.4-11 4 ...................................... 89
3.4-12 5 ................................................................. 90
3.4-13 5 ......................................................... 90
3.4-14 6 ................................................................. 91
3.4-15 6 ......................................................... 91
3.4-16 7 ................................................................. 92
3.4-17 7 ......................................................... 92
3.4-18 8 ................................................................. 93
ix
3.4-19 8 ......................................................... 93
3.4-20 ................................................................. 94
3.2-1 14C 14C .......................................... 95
3.2-2 14CO2 ............................................................................... 95
3.2-3 14CO2 ......................................... 95
3.2-4 14CO2 ............................................................................... 96
3.2-5 14CO2 ......................................... 96
3.3-1 P2 ................................................. 97
3.3-2 P11 ............................................... 97
3.3-3 14C DGGE ......................................... 98
3.3-4 DGGE DNA ......................................................... 98
3.4-1 ............................................................................................. 99
3.4-2 ....................... 100
3.4-3 14C .......................................... 101
3.4-4 14C .............................................. 101
3.4-5 14C ....................................... 102
3.4-6 -> 14C .......................................................... 103
3.4-7 -> 14C .......................................................... 103
3.4-8 -> 14C ...................................................... 104
3.4-9 4 14C . 105
3.4-10 ................................ 106
3.4-11 1 ............................................................................................. 106
3.4-12 2 ............................................................................................. 106
3.4-13 3 ............................................................................................. 106
3.4-14 4 ............................................................................................. 107
3.4-15 5 ............................................................................................. 107
3.4-16 6 ............................................................................................. 107
3.4-17 7 ............................................................................................. 108
3.4-18 8 ............................................................................................. 108
3.4-19 .................................................................................. 108
3.4-20 CO2 . 109
3.4-21 14C ......................... 110
3.4-22 14C ............................................ 111
3.4-2314C .......................................................................................................... 112
3.4-2414C .......................................................................................................... 112
3.4-2514C ............................................................................................................ 113
x
3.4-2614C ............................................................................................................ 113
3.4-27 14C ............................................................ 114
3.4-28 - ................................... 114
3.4-29 .................................... 115
3.4-30 14C
..................................................................................... 116
3.4-3114C ................................................................................................. 117
3.4-3214C .............................................................................................. 117
4 Pu, Am, Th Cl
4.2-1 CaC2O4 UTEVA + DGA-N Am 5g JSAC-0471
SF-ICP-MS 1mL ............... 149
4.2-2 241Am ...................................... 149
4.2-3 Pu 241Am/239+240Pu activity ............................... 150
4.3-1 Th ................................................................................. 150
4.3-2 Th .............................................................................. 151
4.4-1 TMAH RSD(%) ....... 152
4.4-2 RSD(%) ...................... 152
4.4-3 TF ............................... 153
4.4-4. ................................... 153
4.5-1 Pu 240Pu/239Pu .................................................. 154
4.5-2 239Pu Pu - ................................................ 155
4.5-3 Pu - .......................................................................... 155
4.6-1 2008-2016 Th − ........................ 156
4.6-2 2008-2016 Am − ................. 157
4.6-3 2008-2016 Pu − ................... 158
4.2-1 Aridus II SF-ICP-MS (Element XR)
....................................................................................................................... 159
4.2-2 DGA-N . 159
4.2-3 Fe(OH)3 CaC2O4 CaF2 n = 3
........................................................................................................................... 160
4.2-4 DGN 0.05M HNO3 Am REE (a) TEVA
Am REE (b) ................................................. 160
4.2-5 SF-ICP-MS Am ................................................. 161
xi
4.2-6 DGA-N 0.5M HCl TEVA 4M HCl
Am ......................................................................................................... 161
4.2-7 IAEA-soil-6 and IAEA-375
NIST-4357, IAEA-385 and IAEA-384 (NIST-4354)
241Am .............................................................................. 162
4.2-8 241Am 239+240Pu 137Cs ...... 163
4.2-9 241Am/239+240Pu 241Am
241Am/239+240Pu ................................................................. 164
4.4-1 NAA TMAH -ICP-MS
................................................................................................................ 165
4.4-2 TMAH ..................... 165
4.4-3 1 TMAH 100
............................................................................................................ 166
4.4-4 1 TMAH 100
................................................................................................................ 166
4.5-1 (1-6, 27 ;
7-10, ) ................................................................................... 167
4.5-2 Pu HNO3 - ........................ 168
4.5-3 Pu - IAEA TRS-472
.............................................................. 169
4.6-1 2008 2016 Th - IAEA
TRS-472 .................................................................. 169
4.6-2 2008 2016 Am - IAEA
TRS-472 .................................................................. 170
4.6-3 2008 2016 Pu - IAEA
TRS-472 .................................................................. 172
14C
Pu
Am Th Cl
TF Kd
Pu Am Th Cl
TF Kd -Kd -Kd TF
28
TF
• TF • 5
20
• 20
• TF 27
Kd • TF
• 20 30 137Cs
Kd
• TF
TF TF
1
28
• 14C 14C • 14C • 14C
• 14C
• CO2
•
Pu Am Th Cl
Pu Am Th (Cl)
-
28
27
• 241Am ICP-MS -
• Pu Th Am Cl
• Pu Th Cl
• Pu Th Cl TF
• 25 28 TF
2
TF Kd
Kautsky et al., 2013; Staudt et al., 2013,
Becker et al., 2014
NUMO
Geosphere-Biosphere InterfaceNUMO 2011
Walke et al., 2015
FAO 2017
IAEA 2010
− Transfer Factor, TF
5
- 20
28
3 15
20 TF
TF Kd
Cs Kd Cs Kd
Kd
20 10 23 30
3
Cs 135Cs 2.3×106 y
4
2.2.1. TF
2.2.1.1
Staudt et al., 2013 Kautsky et al., 2013 Becker et al., 2014
Dowdall 2008
Gesellschaft für Anlagen- und Reaktorsicherheit 2008
90Sr 137Cs
TF
TF
2017
csv
web doi
Ref.
Single exponential
p
web doi
2.2.1.2
5
2.2.1.1
2.2.2.
Tagami and Uchida, 2010
FAO
Ni, Sr, Mo Pb 2.2-1 Ni
Zn, Cu, As, Cd Co
Pinson 2015 1763
P, Mg, K, S, Ca, As, Cd, Co, Cu, Fe, Mn, Mo,
Ni, Rb, Sr Zn
TF
6
TF
2.3.1. − TF
5 5
TF
26
15
2.3.1.1.
2.3-1 2.3-2
0-15cm 0-20cm
2.5 kg 0.5kg
100cc
5 kg 5 kg
2.3-22.3-3 2.3-4
2.3-5 2.3-6
2.3.1.2.
100 g
40
2mm
50 g
7
2.3.1.3.
RO Milli-Q
EYELA
FD-550
2.5 kg 0.5 kg 2.3-3
MC-90A
2.3.1.4.
1 pH(H2O)
10 g 25 mL 1pH pH
2 CEC Schollenberger
1M 100 mL
13 mm 120 mm 1M 2/3
8 cm1M 4 20
80 %
80 % 50 mL
10 % 100 mL
200 mL
3 Ca K
2 200 mL
1000 mg/L
< >
SpectrAA240FS
: 766.5 nm 422.7 nm
8
: 2.00 L/min 13.50 L/min
4 Al Fe
1.0 g 250 mL 0.2 M pH3.0 100 mL
4 25 mL 50 mL Superfloc ( ) 1 10 3000 rpm
ICP
<ICP >
ICPE-9000
1100 W 15 L/min
1.2 L/min
0.80 L/min
396.153 nm 238.204 nm
5 Al, Fe 0.05 g HNO3 3 mL HCl 3 mL
HNO3 1 mL HF 1 mL
PTFE HNO3 2 mL 4 mL
HNO3(1+2) 50 mL
ICP
<ICP >
Optima 8300
1300 W
12 L/min
0.2 L/min
0.55 L/min 396.153 nm 238.204 nm( ) 343.489 nm ;
RSD 10
2.3-7
2.3.1.5.
(1)
0.1 0.2 g 500˚C 5 g 900˚C 20
(1+1) (1+1) 20 mL
(1+1) 20 mL 10 No.5C[ ]
900 ˚C20 (W1) 2 3 10
9
mL (W2) 2
(W1-W2)
(2)
0.2 g 550 ˚C 2 1 g900 ˚C 20 155˚C 5 %HNO3
50 mL No.5C[ ] 100 mL
ICP
<ICP >
Optima 8300 1300 W
15 L/min
0.2 L/min
0.55 L/min
208.957 nm
451.131 nm ;
(3)
0.1 g
< > MA-3000
253.7 nm
(4) Cr, P, Co, Ni, Cu, Zn, Sr. Cd
2.3.1.4. (5) 213.617 nm ICP
Cr Co Ni Cu Zn Cd ICP
<ICP >
Agilent 8800
1550 W
15 L/min
1.0 L/min 5 mL/min
m/z 52( ) 59( ) 60( ) 63( ) 66( ) 111( )
103( ; )
2.3.1.6.
(1)
10
0.2 3 g 500 ˚C 5 g 900˚C
20 No.5B[ ]
2.3.1.4. 5 ICP
<ICP >
SPECTRO BLUE
1400 W
( ) 13 L/min
( ) 0.8 L/min
( ) 0.8 L/min 251.612 nm( ) 417.206 nm( ; )
(2) P, Fe, Ni, Cu, Zn, Cd
0.5 0.6 g 5 mL HNO3
50 mL
ICPICP
<ICP >
Optima 8300
1300 W ( ) 12 L/min
( ) 0.2 L/min
( ) 0.55 L/min
213.617 nm( ) 238.204 nm( ) 213.857 nm( )
371.029 nm( ; )
<ICP >
Agilent 8800
1550 W
( ) 15 L/min
( ) 1.0 L/min ( ) 5 mL/min
m/z 59( ) 60( ) 63( ) 111( ),
103( ; )
2.3.1.7.
(1) 100 mg HNO 7 mL HF 7 mL
11
AA-100 CEM MARS5
15 HClO 1 mL
1 mL HNO 0.5 mL H2O2
40%HNO 2.5 mL 50 mL Milli-Q >18MΩ
50mL HNO3 2%1 500
JB-1a JB-3 ICP Horiba Activa-M
ICP Agilent, 7500c
(2)
80˚C 3 500mg HNO3 10mLHF 4 mL 80˚C 10
10
1 mL HNO 0.5 mL H2O2
40%HNO 1 mL 20 mL 20 mL
HNO3 2% 1/40
GBW-07603 NISTSRM-1573a ICP Horiba Activa-M
ICP Agilent, 7500c
2.3.1.8. 28
2.3-8 26 28 14-18
CEC 26-28
t , p<0.05
2.3-9 2.3-10
21 20
TF 2.3-11
2.3.2. 27 2.3.1.7 27 20
TF
2.3-12 2.3-13
TF
2.3-14
12
2.3.3. − TF
28 10 5 5
10 5 5
20 2.3-7 2.3-9 2.3-10
TF 2.3-11
27
2.3-12 2.3-13 TF 2.3-14
13
14-18
5
5-9 2016 2.4-1
1981 2010 30
10.1 19.0
9 5-9 18.4 25.3 7
2.4.1.
26
21
Na, Mg, Al, Si, P, K, Ca, Cr, M, Fe, Co, Ni, Cu, Zn, Sr,
Cd, Ba Ca, K, Al, Fe pHKaleidaGraph ver. 4.1.4 t
2.4-2 2.4-3
p>0.01 Fe pH GM
Reinmann and Caritat, 2012
2.4-1 Fe, Cu, Zn Ba p<0.01
GM 2
2.4.2.
TF Ca, K, Al, Fe mg/kg
2.4-4 TFp<0.01 Fe, Zn Fe TF 2.4-2
p<0.05 Na, Si, K, Co, Ba K TF
TF
TF GM 2 TF
GSD Ca F
p<0.01 GSD TFTF
Na, Mg, Al, Si, P, K, Ca, Sc, Ti, V, Cr, Mn, Fe, Co, Ni,
Cu, Zn, Se, Rb, Sr, Y, Zr, Nb, Mo, Cd, Sn, Sb, Cs, Ba, La, Ce, Sm, Eu, Gd, Pb, Th, U 37
TF TF
14
2.4.3.
Na, Mg, Al, Si, P, K, Ca, Cr, M, Fe, Co, Ni, Cu, Zn, Sr, Cd, Ba
TF Fe, Zn
TFTF Pinson 2015
Ca,
Mg, K
Pinson TF
7
TF
15
10 Cs Kd 23 10
20 20 Kd 23
30 Kd
10 23 30 Wagai et
al., 2013 Cs Kd
Kd
Cs Kd
2.5.1. 30
Kd RI
Kd 30
1 3
1 7 1 30
30 7
- Cs 30
Kd
Kd
2.5-1 1 10 137Cs 120rpmHIMAC CT5L 3000 rpm 10
=0.45 µm PTFE 3mL NaI (Tl)
ARC-380 20
Kd
di l
Ci (Bq/L) 137Cs Cl (Bq/L) RI 137Cs
Wl L Ws Ci (Bq/L) Cl (Bq/L)cpm/mL
2.5-1 30
3 7, 30 Kd
1 30
Kd EP-SD-50Kd 2.5-1
30
16
Kd RI
3 7 30 EP-SD-50 Kd 30
10 23 1 7
2.5.2. 30
30 Kd
20 <2 mm
g 30 mL Milli-Q 10 mL 30˚C
120 rpm 24 137Cs CsCl 14 kBq 30˚C 120 rpm
2.5.1
2.5.3. 30˚C Kd-137Cs
30 Kd 2.5-2 10 23 10
23 30 10 30Kd Kd t-test p=0.0075 2.5-2 Kd
10 30 0.49 Kd 10 3.88×103
20 2.34×103 30 1.91×103
Cs Cs
Cs e.g. Bellenger and Staunton, 2008
Kd 2.5-3R=0.99 10 Kd 1000 Cs
Cs Kd
Sr Başçetin and Atun 2006 Kd
Kd
Cs Cs
2.5.4. 30˚C Kd-137Cs
10 23 30 Kd Kd
10 Kd 1000
30
17
135Cs
2.3 106 y
Cs
2.6.1. 137Cs
137Cs 2011 2013Tagami and Uchida, 2015 Smith et al., 2000
Cs
2.6.1.1.
Fallopia japonica Artemisia indica var.
maximowiczii Petasites japonicus
80˚C U8 Ge
Seiko EG&G Ortec 80,000 150,000
t
Yt
Yt = A*exp(-λa*t)+ B*exp(-λb*t) ….(1)
: A
B
λa Teff=ln(2)/λa
λb Teff=ln(2)/λb
KaleidaGraph ver. 4.1.4
2.6.1.2. Cs 137Cs 2.6-1
R=0.99, R=0.90, R=0.892.7-10.5 10.5
18
137Cs
13-21 2016
2015-2016
Tag m2 kg-1 137Cs
TF
Tag
Tag= 137Cs Bq kg-1 137Cs Bq m-2 ….(2)
Bq m-2 0-5cm
5 cm 137Cs 5% 2011-2016
(2) Tag 5.3×10-5 1.6×10-4 m2 kg-1 Tag
2.5×10-3 1.2×10-2 m2 kg-1 IAEA, 2010 1-2
Cs
2.6.2. Cs
Cs
2017 Cs
2.6.1137Cs
Tag
2017
2017 in-situ
Bq m-2
2016 12
2.6.2.1. Tag 325 1177 183 968 205
2.6-2 Tag=10-5
N.D. 2015-2016
R=-0.51, p<0.001 Tag 0.2
19
137Cs
1.8y 9.3 2016
Cs 134+137Cs134Cs
Cs134Cs
137Cs137Cs
Tag Tag
Tag 3.4×10-3 m2 kg-1 2.6-2 IAEA 2010 5×10-4
3.4×10-1 m2 kg-1 Tag
2016
2.6.2.2. Tag 97 78 44 83 359
2.6-2
p
3.6- Tag Tag
Tag 5.5×10-3 m2 kg-1 2.6-2 t
p<0.01 Red deer
Roe deer 1×10-2 5×10-2 m2 kg-1 5×10-3 5×10-2 m2 kg-1 IAEA, 2010
Tag Red deer Roe deer
2.6.2.3.
Tag 50 56 346 200
Tag 2.6-2
Tag
Tag
Tag 3.8×10-3 m2 kg-1 2.6-2IAEA TRS472
2010
2.6.2.4. Tag 137Cs Tag
Tag Tag
3.4×10-3 m2 kg-1 5.5×10-3 m2 kg-1 3.8×10-3 m2 kg-1
20
Cs Tag
2017aHohmann & Huckschlag, 2005
Cs
2.6.3. 137Cs
Cs Cs
Cs
Tsuji et al. 2014
Cs
Kurita et al. (2015) Cs 2011
3 Cs
Tagami and Uchida, 2016 6
Cs2015 9
137Cs 2016 3
2.6.3.1.
2.6-3
134+137Cs
, on line 2011 11 5 30k Bq/m2
, 2017b 2011 11 2016 92.6-3 28 12 6 9 2
348 Bq/kg-dry 357 Bq/kg-dry
2011 11 2016
9 20 1 Bq/L
2.6.3.2. 137Cs
21
2016 3 2 12 8 51
2.6-4 - - 2.6-4
37 15 2 1
80
U U8,
JSAC0473, 137Cs 2.6-5 137Cs
137Cs 32-49%
21-43% 137Cs4-8%
Yankovich, 2009
137Cs
Cs137Cs 137Cs
100 Bq/kg
137Cs
137Cs
2.6-5 2 2
7 3 2 2 2137Cs 2
6 3
37 22137Cs 18
5 10
10 137Cs 86 Bq/kg-dry137Cs
137Cs 137Cs 137Cs
22
137Cs
2.6.3.3.
Rybczynski et al. 2008, Perkins et al. 2014
2010, 2013
, 2:1
Logan and Lutcavage 2008
10 mg
2.6-6 2015 12 14
10-20 mg 2 mL
=2:1 1.5 mL
5,500
× g 5 1.5 mL1
2 2 3
50 24
DELTA V Advantage, Thermo Fisher
Scientific Inc. 3 SI Science Reference Material; Amino Standard13C 15N
13C 15N 2.6-7 1 13C -42.8 -26.6
2 1 13C
3 13C13C
13C 13C15N
23
Eliot and Eliot (2016) 15N
3 3
2015 9 13C 15N
2.6-6 2.6-8
15N 15N
Minagawa and Wada, 1984 15N 13C
, 2013 2 13C
137Cs
15N 13.2 15.9 2.715N 3-4 2013
15N 16.1
15N 16.813C 15N
137Cs
24
TF Kd
—TF Cs Kd
135Cs
Cs
2.7.1. TF
90Sr 137Cs
Ni, Sr, Mo Pb
Ni
5 Co, Zn, Cu, As, Cd
2.7.2. − TF 28 10
10
26
15 20
TF
TF26 28
14-18
26-28
TF
2.420
25
2.7.3 TF
Na, Mg, Al, Si, P, K, Ca, Cr, M, Fe, Co, Ni, Cu, Zn, Sr, Cd, Ba 14-18
TF
18.4 25.3 7
TF Fe, Zn, p<0.01
Pinson 2015
TF 7
TF37 Na, Mg, Al, Si, P, K, Ca, Sc, Ti, V, Cr, Mn, Fe, Co, Ni, Cu, Zn, Se, Rb, Sr,
Y, Zr, Nb, Mo, Cd, Sn, Sb, Cs, Ba, La, Ce, Sm, Eu, Gd, Pb, Th, U TF
2.7.4.
20 30 Kd
10 23 Kd Kd 10 3.88×103
20 2.34×103 30 1.91×103 Kd
10 Kd 1000
30
2.7.5 Cs
27-28
Tag 5.3×10-5 1.6×10-4 m2 kg-1
137Cs
Tag 3.4×10-3 m2 kg-1
5.5×10-3 m2 kg-1 3.8×10-3 m2 kg-1 Cs Tag
26
137Cs
137Cs137Cs 137Cs
137Cs13C 15N
TF Tag Kd
Başçetin, E., & Atun, G. (2006). Adsorption behavior of strontium on binary mineral mixtures of Montmorillonite
and Kaolinite. Applied radiation and isotopes, 64(8), 957-964.
Becker, J. K., Lindborg, T., & Thorne, M. C. (2014). Influence of climate on landscape characteristics in safety
assessments of repositories for radioactive wastes. Journal of environmental radioactivity, 138, 192-204.
Bellenger J.-P., Staunton, S. (2008) Adsorption and desorption of 85Sr and 137Cs on reference minerals, withi and without inorganic and organic surface coatings. J. Environ. Radioactiv. 99, 831-840.
Dowdall, M., Standring, W., Shaw, G., & Strand, P. (2008). Will global warming affect soil-to-plant transfer of
radionuclides?. Journal of environmental radioactivity, 99(11), 1736-1745.
Elliott, K. H., & Elliott, J. E. (2016). Lipid extraction techniques for stable isotope analysis of bird eggs:
Chloroform–methanol leads to more enriched 13C values than extraction via petroleum ether. Journal of
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Fuma, S., Kubota, Y., Ihara, S., Takahashi, H., Watanabe, Y., Aono, T., H. Soeda & Yoshida, S. (2016).
Radiocaesium contamination of wild boars in Fukushima and surrounding regions after the Fukushima
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51(4), 263-270.
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27
Kurita, Y., Shigenobu, Y., Sakuma, T., & Ito, S.-i. (2015). Radiocesium contamination histories of Japanese
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radionuclide transfer to tree leaves?. Radiation and environmental biophysics, 49(4), 583-590.
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Demersal Fish Based on Field Observation Results Obtained after the Fukushima Accident. Environmental
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Radioanalytical and Nuclear Chemistry, 307(1), 741-746.
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deposition after the nuclear power plant accident in Fukushima. Water Res, 60, 15-27.
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28
microbial physiology. Global Change Biology, 19(4), 1114-1125. Walke, R. C., Kirchner, G., Xu, S., & Dverstorp, B. (2015). Post-closure biosphere assessment modelling:
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fish tissues using stable analogues. J Environ Radioact, 100(9), 795-801. 2017a
https://www.env.go.jp/nature/choju/plan/plan3-2a/ 2017/1/17
2017b . .
http://www.env.go.jp/jishin/monitoring/results_r-pw.html 2017/1/6
2017 http://www.data.jma.go.jp/gmd/risk/obsdl/ 2017.1.10
2017
http://www.mhlw.go.jp/stf/kinkyu/0000045250.html 2017/1/17
2016 29 90 .
, , , , , & . (2013).
. Journal of Fisheries
Technology, 6(1), 57-68. , & . (2010). / (TCEA/IRMS)
. Researches in organic
geochemistry, 26, 31-37.
2017 -137 http://ramap.jmc.or.jp/map/
2017/1/17
2017http://www.pref.fukushima.lg.jp/site/portal/wildlife-radiationmonitoring1.html 2017/1/17
, 2016. 27
, .
29
- 1. 2014 11 2015 11
2015 1 1 2015
12 31 2016 1 2016 12 31
(1)
20 cm 0.5 m
20 cm 1.5 mSK-L210T
TR-71wf 5
6 0-4 4-8 8-12 12-16 16-20 20-24
2 6 10 14 18 22
2017 2015 20161 1 12 31
(2) 2s-1 2015 2016
2015
2016 2s-2 2015 2016
0.996 p<0.001
2s-1 2015 2016 1
R>0.90,
p<0.001
30
2.3-1
Sample code EPII-CF- 21 2016/7/28 EPII-CF- 22 2016/7/28 EPII-CF- 23 2016/8/13 EPII-CF- 24 2016/6/10 EPII-CF- 25 2016/9/17 EPII-CF- 26 2016/9/21 EPII-CF- 27 2016/9/17 EPII-CF- 28 2016/10/11 EPII-CF- 29 2016/9/25 EPII-CF- 30 2016/10/20 EFII-CF- 41 2016/5/29 EFII-CF- 42 2016/5/31 EFII-CF- 43 2016/6/1 EFII-CF- 44 2016/6/2 EFII-CF- 45 2016/6/9 EFII-CF- 46 2016/7/4 EFII-CF- 47 2016/7/12 EFII-CF- 48 2016/8/6 EFII-CF- 49 2016/8/9 EFII-CF- 50 2016/8/10
2.3-2
Sample code EPII-SD- 21 2016/7/30 0.82 EPII-SD- 22 2016/8/2 1.06 EPII-SD- 23 2016/8/17 0.15 EPII-SD- 24 2016/9/5 1.49 EPII-SD- 25 2016/9/20 0.9 EPII-SD- 26 2016/9/27 0.66 EPII-SD- 27 2016/10/14 1.05 EPII-SD- 28 2016/10/20 1.15 EPII-SD- 29 2016/10/22 0.74 EPII-SD- 30 2016/10/20 0.1 EFII-SD- 41 2016/5/29 0.87 EFII-SD- 42 2016/5/31 0.9 EFII-SD- 43 2016/6/1 0.8 EFII-SD- 44 2016/6/2 0.92 EFII-SD- 45 2016/6/9 0.81 EFII-SD- 46 2016/7/4 0.72 EFII-SD- 47 2016/7/12 0.65 EFII-SD- 48 2016/8/6 0.73 EFII-SD- 49 2016/8/9 0.86 EFII-SD- 50 2016/8/10 0.92
31
2.3-3
2.3-4
(g)
EPII-CF- 21 9.3 % 480.02 435.40 90.7 %
EPII-CF- 22 9.5 % 480.04 436.99 91.0 %
EPII-CF- 23 9.6 % 480.05 438.25 91.3 %
EPII-CF- 24 10.1 % 480.07 440.74 91.8 %
EPII-CF- 25 9.2 % 480.03 439.69 91.6 % EPII-CF- 26 10.9 % 480.06 437.74 91.2 % EPII-CF- 27 10.4 % 480.08 439.11 91.5 %
EPII-CF- 28 9.5 % 480.05 438.38 91.3 %
EPII-CF- 29 8.3 % 480.01 437.74 91.2 %
EPII-CF- 30 9.7 % 480.09 441.01 91.9 %
EFII-CF- 41 2.3 % 81.2 % EFII-CF- 42 8.0 % 79.0 % EFII-CF- 43 4.7 % 82.6 % EFII-CF- 44 8.8 % 79.6 % EFII-CF- 45 2.4 % 79.8 % EFII-CF- 46 7.9 % 78.4 % EFII-CF- 47 4.5 % 81.8 % EFII-CF- 48 7.2 % 81.3 % EFII-CF- 49 5.7 % 78.9 % EFII-CF- 50 2.1 % 76.5 %
32
2.3-5
21
2016.8.2 2016.8.2
22
2016.8.5 2016.8.5
23
2016.8.18 2016.8.18
24
2016.9.14 2015.9.14
25
2016.9.23 2016.9.23
33
2.3-5
26
2016.9.29 2016.9.29
27
2016.10.17 2016.10.17
28
2016.10.24 2016.10.24
29
2016.10.24 2016.10.24
30
2016.10.28 2016.10.28
34
2.3-6
41
2016.5.31 2016.5.31
42
2016.6.2 2016.6.2
43
2016.6.2 2016.6.2
44
2016.6.6 2016.6.6
45
2016.6.10 2016.6.10
35
2.3-6
46
2016.7.6 2016.7.6
47
2016.7.13 2016.7.13
48
2016.8.8 2016.8.8
49 1
2016.8.11 2016.8.11
50 2
2016.8.12 2016.8.12
36
2.3-7 28
pH CEC Ca K Al Fe
No. (H2O) meq/100g mg/100g mg/100g g/kg g/kg
EPII-SD- 21 5.7 15 156 10 2.3 4.7 EPII-SD- 22 5.5 10 96 13 2.2 3.9 EPII-SD- 23 4.7 10 49 12 1.2 2.1 EPII-SD- 24 6.6 8 137 9 3.2 3.7 EPII-SD- 25 5.5 20 186 15 3.0 10.4 EPII-SD- 26 5.5 24 169 61 4.8 3.0 EPII-SD- 27 5.8 19 141 27 9.6 9.7 EPII-SD- 28 5.6 18 165 17 2.1 11.5 EPII-SD- 29 5.3 37 329 29 3.2 10.9 EPII-SD- 30 5.2 39 246 18 14.5 16.5 EFII-SD- 41 3.9 20 30 41 5.0 6.0 EFII-SD- 42 5.4 10 64 25 3.2 3.8 EFII-SD- 43 5 19 158 29 4.1 5.9 EFII-SD- 44 7 16 354 25 2.2 4.7 EFII-SD- 45 6.9 21 461 39 3.6 3.6 EFII-SD- 46 6 26 354 56 12.4 3.7 EFII-SD- 47 5.6 26 268 71 28.6 10.6 EFII-SD- 48 4.5 36 28 30 10.7 14.5 EFII-SD- 49 6.1 31 435 47 3.3 7.1 EFII-SD- 50 5 13 85 10 2.7 6.1
2.3-8 14-18 26-28
p<0.05
pH CEC Ca K Al Fe
Sample (H2O) meq/100g mg/100g mg/100g g/kg g/kg
Paddy field H14−18 5.7 13.3 171 19 3.5 6.6 H26-28 5.7 15.2 140 18 3.9 6.0
Upland field H14−18 6.3 14.1 252 44 6.2 7.6 H26-28 5.9 20.4* 192 33 9.6 7.2
37
2.3-9 28
B Na Mg Al Si P K Ca Cr Mn Fe Sample code mg/kg mg/kg mg/kg g/kg g/kg g/kg mg/kg mg/kg mg/kg mg/kg g/kg EPII-SD- 21 4.1E+1 1.4E+4 3.8E+3 6.7E+1 3.0E+2 1.7E+0 1.3E+4 4.8E+3 4.7E+1 2.7E+2 2.6E+1 EPII-SD- 22 3.0E+1 1.5E+4 4.7E+3 8.5E+1 2.8E+2 8.3E-1 1.6E+4 6.8E+3 2.6E+1 3.8E+2 2.8E+1 EPII-SD- 23 4.3E+1 8.2E+3 2.0E+3 5.9E+1 3.3E+2 7.4E-1 2.1E+4 9.3E+2 4.6E+1 1.3E+2 1.3E+1 EPII-SD- 24 2.1E+1 5.4E+3 3.4E+3 5.1E+1 3.5E+2 7.5E-1 1.3E+4 3.3E+3 5.4E+1 5.6E+2 2.7E+1 EPII-SD- 25 1.7E+1 1.2E+4 6.1E+3 8.4E+1 2.6E+2 1.3E+0 9.6E+3 1.1E+4 2.7E+1 6.1E+2 4.7E+1 EPII-SD- 26 1.6E+1 1.5E+4 6.5E+3 7.7E+1 2.6E+2 2.0E+0 9.9E+3 1.0E+4 1.8E+1 4.3E+2 2.8E+1 EPII-SD- 27 2.2E+1 1.3E+4 8.1E+3 8.0E+1 2.5E+2 2.1E+0 1.2E+4 1.4E+4 4.7E+1 7.5E+2 4.1E+1 EPII-SD- 28 7.0E+0 1.1E+4 2.4E+4 9.1E+1 2.1E+2 1.2E+0 4.1E+3 2.3E+4 4.2E+2 1.4E+3 6.2E+1 EPII-SD- 29 3.2E+1 1.0E+4 1.1E+4 7.2E+1 2.6E+2 1.1E+0 1.3E+4 1.2E+4 6.4E+1 4.3E+2 3.6E+1 EPII-SD- 30 1.4E+1 7.0E+3 5.0E+3 7.8E+1 2.1E+2 5.2E+0 4.2E+3 9.7E+3 5.5E+1 5.8E+2 5.7E+1 EFII-SD- 41 1.8E+1 1.3E+3 6.5E+2 4.5E+1 1.8E+2 2.7E+0 4.3E+3 7.3E+2 1.7E+2 9.8E+2 8.9E+1 EFII-SD- 42 5.1E+1 1.4E+4 1.1E+4 6.4E+1 3.0E+2 1.8E+0 2.1E+4 1.1E+4 8.4E+1 1.0E+3 4.0E+1 EFII-SD- 43 1.7E+1 8.7E+2 4.6E+2 4.1E+1 1.8E+2 1.6E+0 2.4E+3 7.3E+2 5.7E+1 1.3E+3 8.1E+1 EFII-SD- 44 2.7E+1 1.5E+4 9.8E+3 7.0E+1 2.7E+2 2.2E+0 1.5E+4 1.4E+4 8.8E+1 8.8E+2 4.2E+1 EFII-SD- 45 6.9E+1 5.3E+3 3.2E+3 6.4E+1 2.8E+2 3.8E+0 1.9E+4 8.7E+3 6.6E+1 6.1E+2 2.7E+1 EFII-SD- 46 1.0E+1 1.5E+4 8.5E+3 6.8E+1 2.6E+2 3.0E+0 8.1E+3 1.9E+4 2.2E+1 7.9E+2 3.1E+1 EFII-SD- 47 2.4E+1 1.1E+4 6.5E+3 7.2E+1 2.1E+2 2.2E+0 9.7E+3 8.7E+3 4.6E+1 9.0E+2 4.9E+1 EFII-SD- 48 4.6E+1 6.2E+3 3.1E+3 6.1E+1 2.3E+2 1.8E+0 1.4E+4 2.4E+3 7.1E+1 6.9E+2 3.8E+1 EFII-SD- 49 2.9E+1 8.4E+3 3.9E+3 6.0E+1 2.4E+2 2.0E+0 9.0E+3 7.6E+3 9.9E+1 4.2E+2 3.3E+1 EFII-SD- 50 2.7E+1 1.4E+4 2.3E+4 7.2E+1 2.4E+2 1.9E+0 7.3E+3 4.1E+4 4.7E+1 1.5E+3 6.9E+1
Co Ni Cu Zn Rb Sr Mo Cd Ba Hg Sample code mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg EPII-SD- 21 8.2E+0 1.7E+1 2.1E+1 9.7E+1 5.7E+1 5.8E+1 3.2E-1 2.1E-1 2.6E+2 9.0E-2 EPII-SD- 22 8.5E+0 1.0E+1 1.4E+1 7.2E+1 8.3E+1 7.9E+1 4.5E-1 1.4E-1 3.5E+2 7.0E-2 EPII-SD- 23 4.2E+0 1.5E+1 1.7E+1 6.1E+1 4.2E+1 4.3E+1 1.9E-1 2.2E-1 3.9E+2 1.8E-1 EPII-SD- 24 1.1E+1 2.2E+1 2.3E+1 6.8E+1 3.6E+1 3.4E+1 5.0E-1 1.4E-1 2.0E+2 3.0E-2 EPII-SD- 25 1.2E+1 1.1E+1 1.7E+1 8.9E+1 9.5E+1 8.8E+1 8.3E-1 2.0E-1 3.9E+2 9.0E-2 EPII-SD- 26 7.3E+0 8.9E+0 3.3E+1 1.2E+2 8.9E+1 8.1E+1 9.2E-1 4.7E-1 3.1E+2 2.0E-1 EPII-SD- 27 1.3E+1 2.2E+1 3.5E+1 1.5E+2 1.2E+2 1.1E+2 1.4E+0 4.9E-1 3.6E+2 1.7E-1 EPII-SD- 28 3.1E+1 7.6E+1 6.2E+1 1.1E+2 2.5E+2 2.3E+2 5.9E-1 3.1E-1 2.8E+2 4.0E-2 EPII-SD- 29 1.1E+1 2.3E+1 2.4E+1 1.1E+2 1.2E+2 1.2E+2 2.1E+0 4.1E-1 4.0E+2 1.4E-1 EPII-SD- 30 1.8E+1 1.9E+1 3.9E+1 1.2E+2 6.1E+1 5.6E+1 1.6E+0 7.6E-1 2.0E+2 2.1E-1 EFII-SD- 41 3.2E+1 4.2E+1 3.6E+1 1.4E+2 8.0E+0 8.2E+0 1.4E+0 7.2E-2 3.1E+2 7.0E-2 EFII-SD- 42 1.4E+1 3.4E+1 4.3E+1 1.7E+2 1.8E+2 1.8E+2 6.1E-1 3.5E-1 4.2E+2 4.0E-2 EFII-SD- 43 3.3E+1 2.9E+1 3.0E+1 1.5E+2 5.9E+0 6.2E+0 1.1E+0 1.5E-1 3.6E+2 3.0E-2 EFII-SD- 44 1.5E+1 3.5E+1 1.8E+2 5.4E+2 1.6E+2 1.6E+2 9.6E-1 1.0E+0 3.7E+2 3.5E-1 EFII-SD- 45 9.5E+0 2.1E+1 4.1E+1 2.2E+2 4.4E+1 4.4E+1 6.8E-1 3.2E-1 3.4E+2 2.0E-1 EFII-SD- 46 1.1E+1 1.2E+1 2.0E+1 9.1E+1 1.9E+2 1.9E+2 2.9E-1 2.4E-1 2.1E+2 6.0E-2 EFII-SD- 47 1.4E+1 1.7E+1 1.5E+1 1.1E+2 7.6E+1 7.5E+1 1.8E+0 2.0E-1 2.6E+2 1.0E-1 EFII-SD- 48 9.6E+0 2.4E+1 2.5E+1 1.2E+2 3.7E+1 3.7E+1 2.2E+0 4.2E-1 2.1E+2 1.4E-1 EFII-SD- 49 1.4E+1 3.0E+1 2.6E+1 8.3E+1 5.2E+1 5.1E+1 7.3E-1 2.7E-1 3.0E+2 2.1E-1 EFII-SD- 50 2.4E+1 1.8E+1 3.8E+1 1.1E+2 2.2E+2 2.1E+2 7.2E-1 1.9E-1 2.7E+2 5.0E-2
38
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Sample code Li mg/kg
Na mg/kg
Mg mg/kg
Al mg/kg
Si mg/kg
P mg/kg
K mg/kg
Ca mg/kg
Cr mg/kg
Mn mg/kg
EPII-CF- 21 4.7E-3 2.3E+1 1.4E+3 4.9E+0 1.7E+2 4.3E+3 3.1E+3 8.5E+1 1.4E-1 2.4E+1 EPII-CF- 22 4.4E-3 3.2E+1 1.3E+3 2.9E-1 2.2E+2 3.8E+3 3.2E+3 9.1E+1 1.2E-1 3.1E+1 EPII-CF- 23 5.6E-3 1.6E+1 1.1E+3 1.2E+0 4.5E+2 3.6E+3 3.3E+3 8.0E+1 1.2E-1 3.8E+1 EPII-CF- 24 7.3E-3 2.8E+1 1.1E+3 8.9E+0 3.1E+2 3.5E+3 3.3E+3 7.7E+1 2.5E-1 2.8E+1 EPII-CF- 25 2.5E-3 1.8E+1 1.2E+3 1.4E+0 1.2E+2 4.0E+3 3.4E+3 8.0E+1 1.3E-1 2.8E+1 EPII-CF- 26 5.7E-3 1.0E+1 1.2E+3 1.1E+0 3.0E+2 3.3E+3 2.9E+3 1.0E+2 1.4E-1 2.9E+1 EPII-CF- 27 1.8E-3 2.2E+1 1.2E+3 2.8E-1 3.3E+2 3.8E+3 3.2E+3 9.2E+1 1.3E-1 4.3E+1 EPII-CF- 28 1.8E-3 8.5E+0 1.2E+3 4.2E-1 6.9E+1 3.2E+3 2.7E+3 8.8E+1 1.6E-1 3.3E+1 EPII-CF- 29 3.6E-3 1.8E+1 1.3E+3 3.5E+0 1.6E+2 3.1E+3 2.9E+3 8.3E+1 1.6E-1 4.4E+1 EPII-CF- 30 1.4E-3 1.0E+1 1.4E+3 1.6E-1 2.0E+2 3.3E+3 2.9E+3 8.7E+1 1.5E-1 3.3E+1 EFII-CF- 41 1.2E-2 3.5E+1 1.0E+3 5.9E+1 5.7E+1 2.5E+3 1.9E+4 1.4E+2 9.4E-2 5.2E+1 EFII-CF- 42 3.6E-3 2.7E+1 1.0E+3 7.4E+0 1.7E+1 3.9E+3 2.5E+4 1.6E+2 6.2E-2 9.7E+0 EFII-CF- 43 2.8E-3 3.3E+1 1.0E+3 1.4E+1 1.7E+1 2.9E+3 2.3E+4 3.8E+2 4.1E-2 1.2E+1 EFII-CF- 44 1.6E-3 1.6E+1 8.7E+2 3.5E+0 9.9E+0 3.4E+3 2.1E+4 5.1E+2 5.8E-2 5.3E+0 EFII-CF- 45 9.3E-4 1.4E+1 1.0E+3 3.9E+0 7.8E+0 3.5E+3 2.4E+4 3.5E+2 5.6E-2 7.3E+0 EFII-CF- 46 1.5E-3 2.1E+1 1.2E+3 6.2E+0 1.0E+1 3.1E+3 2.3E+4 1.7E+2 4.7E-2 7.3E+0 EFII-CF- 47 3.6E-3 2.1E+1 9.9E+2 3.4E+0 6.8E+0 2.4E+3 2.3E+4 1.8E+2 5.0E-2 6.7E+0 EFII-CF- 48 1.2E-3 2.4E+1 9.1E+2 1.6E+0 4.2E+0 2.1E+3 2.2E+4 1.4E+2 4.7E-2 9.6E+0 EFII-CF- 49 1.4E-3 1.2E+1 1.0E+3 3.4E+0 9.2E+0 3.5E+3 2.2E+4 2.9E+2 4.8E-2 5.7E+0 EFII-CF- 50 1.8E-3 1.7E+1 8.7E+2 5.1E+0 1.1E+1 2.6E+3 1.7E+4 1.6E+2 3.5E-2 6.5E+0
Sample code Fe mg/kg
Co mg/kg
Ni mg/kg
Cu mg/kg
Zn mg/kg
Rb mg/kg
Sr mg/kg
Mo mg/kg
Cd mg/kg
Ba mg/kg
EPII-CF- 21 1.6E+1 1.1E-2 9.1E-2 2.0E+0 2.4E+1 3.7E+0 2.0E-1 7.4E-1 8.5E-3 3.6E-1 EPII-CF- 22 1.0E+1 1.2E-2 8.6E-2 2.9E+0 2.6E+1 2.8E+0 2.8E-1 1.2E+0 1.3E-2 1.6E+0 EPII-CF- 23 1.1E+1 6.0E-3 8.0E-1 3.9E+0 3.0E+1 3.2E+0 2.0E-1 2.1E+0 1.8E-1 8.0E-1 EPII-CF- 24 3.4E+1 2.2E-2 1.5E-1 3.1E+0 3.8E+1 2.7E+0 3.5E-1 1.3E+0 2.0E-3 4.3E-1 EPII-CF- 25 8.5E+0 1.4E-2 7.2E-2 9.9E-1 2.3E+1 7.4E+0 1.6E-1 1.2E+0 1.7E-2 1.4E-1 EPII-CF- 26 1.2E+1 4.0E-3 1.6E-1 3.9E+0 2.4E+1 1.5E+0 1.9E-1 8.5E-1 1.1E-1 4.6E-1 EPII-CF- 27 8.3E+0 8.5E-3 9.2E-2 3.3E+0 2.4E+1 4.2E+0 1.7E-1 9.9E-1 6.3E-2 4.2E-1 EPII-CF- 28 1.1E+1 1.1E-2 1.4E-1 2.5E+0 2.5E+1 8.8E+0 2.8E-1 5.9E-1 2.1E-2 5.9E-1 EPII-CF- 29 1.1E+1 9.0E-3 8.9E-1 3.0E+0 2.5E+1 8.5E+0 2.0E-1 1.5E+0 3.1E-1 6.1E-1 EPII-CF- 30 1.0E+1 7.5E-3 9.4E-2 2.1E+0 2.3E+1 2.2E+0 1.1E-1 5.1E-1 8.5E-3 1.3E-1 EFII-CF- 41 4.0E+1 2.0E+0 4.1E-1 4.5E+0 2.1E+1 1.6E+1 5.4E-1 7.5E-2 4.0E-2 2.5E+0 EFII-CF- 42 1.4E+1 5.8E-2 2.1E-1 4.8E+0 1.4E+1 1.2E+1 4.4E-1 2.7E-1 5.0E-2 1.1E+0 EFII-CF- 43 2.6E+1 1.3E-1 1.2E-1 4.1E+0 1.8E+1 1.8E+1 1.9E+0 3.8E-2 1.6E-1 8.5E+0 EFII-CF- 44 1.5E+1 2.1E-2 8.2E-2 5.7E+0 1.8E+1 6.6E+0 1.4E+0 6.2E-1 1.1E-1 9.8E-1 EFII-CF- 45 1.8E+1 2.3E-2 6.1E-2 4.0E+0 1.7E+1 9.8E+0 7.0E-1 3.1E-1 3.0E-2 4.4E-1 EFII-CF- 46 2.1E+1 4.1E-2 5.6E-2 2.1E+0 1.5E+1 9.3E+0 5.9E-1 6.8E-1 5.0E-2 2.7E-1 EFII-CF- 47 1.9E+1 3.5E-2 2.0E-1 2.5E+0 1.5E+1 7.3E+0 1.0E+0 2.3E-1 1.1E-1 4.9E-1 EFII-CF- 48 1.5E+1 8.3E-2 3.0E-1 5.2E+0 2.0E+1 1.7E+1 4.8E-1 7.5E-2 1.2E-1 1.7E+0 EFII-CF- 49 1.6E+1 8.7E-2 2.1E-1 4.8E+0 1.3E+1 4.7E+0 9.4E-1 1.6E-1 1.5E-1 1.5E+0 EFII-CF- 50 1.4E+1 6.8E-2 6.0E-1 4.5E+0 1.1E+1 4.9E+0 6.9E-1 1.3E-1 7.0E-2 1.1E+0
39
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Sample code Na Mg Al Si P K ex. K* Ca ex. Ca* EPII-CF-21 1.6E-3 3.6E-1 7.3E-5 5.6E-4 2.5E+0 2.4E-1 3.0E+1 1.8E-2 5.4E-2 EPII-CF-22 2.1E-3 2.8E-1 3.4E-6 7.9E-4 4.5E+0 2.0E-1 2.5E+1 1.3E-2 9.5E-2 EPII-CF-23 2.0E-3 5.5E-1 1.9E-5 1.3E-3 4.8E+0 1.6E-1 2.9E+1 8.6E-2 1.7E-1 EPII-CF-24 5.1E-3 3.4E-1 1.8E-4 9.0E-4 4.7E+0 2.6E-1 3.7E+1 2.3E-2 5.6E-2 EPII-CF-25 1.5E-3 2.0E-1 1.7E-5 4.8E-4 3.0E+0 3.5E-1 2.4E+1 7.3E-3 4.3E-2 EPII-CF-26 6.6E-4 1.9E-1 1.4E-5 1.2E-3 1.6E+0 2.9E-1 4.7E+0 1.0E-2 6.0E-2 EPII-CF-27 1.7E-3 1.5E-1 3.5E-6 1.3E-3 1.8E+0 2.7E-1 1.2E+1 6.8E-3 6.5E-2 EPII-CF-28 7.4E-4 5.0E-2 4.7E-6 3.2E-4 2.6E+0 6.6E-1 1.6E+1 3.8E-3 5.3E-2 EPII-CF-29 1.7E-3 1.2E-1 4.9E-5 6.0E-4 2.9E+0 2.3E-1 1.0E+1 7.1E-3 2.5E-2 EPII-CF-30 1.5E-3 2.9E-1 2.0E-6 9.6E-4 6.4E-1 6.9E-1 1.6E+1 9.0E-3 3.6E-2 EFII-CF-41 2.6E-2 1.6E+0 1.3E-3 3.2E-4 9.4E-1 4.4E+0 4.6E+1 1.9E-1 4.6E-1 EFII-CF-42 2.0E-3 9.7E-2 1.2E-4 5.9E-5 2.1E+0 1.2E+0 9.9E+1 1.4E-2 2.5E-1 EFII-CF-43 3.8E-2 2.2E+0 3.4E-4 9.6E-5 1.8E+0 9.7E+0 7.8E+1 5.2E-1 2.4E-1 EFII-CF-44 1.1E-3 8.8E-2 5.0E-5 3.6E-5 1.5E+0 1.4E+0 8.4E+1 3.6E-2 1.5E-1 EFII-CF-45 2.7E-3 3.1E-1 6.0E-5 2.8E-5 9.4E-1 1.2E+0 6.1E+1 4.0E-2 7.6E-2 EFII-CF-46 1.4E-3 1.4E-1 9.1E-5 4.1E-5 1.1E+0 2.9E+0 4.2E+1 8.7E-3 4.8E-2 EFII-CF-47 2.0E-3 1.5E-1 4.7E-5 3.2E-5 1.1E+0 2.4E+0 3.2E+1 2.0E-2 6.6E-2 EFII-CF-48 3.8E-3 2.9E-1 2.7E-5 1.8E-5 1.2E+0 1.6E+0 7.4E+1 5.7E-2 5.0E-1 EFII-CF-49 1.5E-3 2.6E-1 5.6E-5 3.9E-5 1.8E+0 2.5E+0 4.8E+1 3.9E-2 6.8E-2 EFII-CF-50 1.2E-3 3.8E-2 7.0E-5 4.4E-5 1.3E+0 2.4E+0 1.7E+2 3.8E-3 1.8E-1
Cr Mn Fe Co Ni Cu Zn Rb Sr Cd Ba
EPII-CF-21 3.1E-3 8.7E-2 6.3E-4 1.3E-3 5.5E-3 9.5E-2 2.5E-1 6.5E-2 3.4E-3 4.1E-2 1.4E-3 EPII-CF-22 4.7E-3 8.1E-2 3.6E-4 1.4E-3 8.3E-3 2.0E-1 3.7E-1 3.4E-2 3.6E-3 9.2E-2 4.6E-3 EPII-CF-23 2.7E-3 2.9E-1 8.7E-4 1.4E-3 5.3E-2 2.3E-1 5.0E-1 7.6E-2 4.6E-3 7.9E-1 2.0E-3 EPII-CF-24 4.6E-3 5.0E-2 1.3E-3 2.1E-3 6.6E-3 1.4E-1 5.6E-1 7.3E-2 1.0E-2 1.4E-2 2.2E-3 EPII-CF-25 4.9E-3 4.7E-2 1.8E-4 1.1E-3 6.4E-3 5.9E-2 2.6E-1 7.7E-2 1.8E-3 8.3E-2 3.6E-4 EPII-CF-26 7.7E-3 6.7E-2 4.2E-4 5.5E-4 1.7E-2 1.2E-1 2.0E-1 1.7E-2 2.3E-3 2.3E-1 1.5E-3 EPII-CF-27 2.8E-3 5.7E-2 2.0E-4 6.5E-4 4.1E-3 9.5E-2 1.6E-1 3.4E-2 1.5E-3 1.3E-1 1.2E-3 EPII-CF-28 3.9E-4 2.4E-2 1.7E-4 3.4E-4 1.8E-3 4.1E-2 2.4E-1 3.6E-2 1.2E-3 6.8E-2 2.1E-3 EPII-CF-29 2.4E-3 1.0E-1 3.1E-4 8.5E-4 3.9E-2 1.3E-1 2.3E-1 6.8E-2 1.7E-3 7.6E-1 1.5E-3 EPII-CF-30 2.7E-3 5.6E-2 1.8E-4 4.2E-4 4.9E-3 5.4E-2 1.8E-1 3.5E-2 2.1E-3 1.1E-2 6.7E-4 EFII-CF-41 5.6E-4 5.3E-2 4.6E-4 6.3E-2 9.9E-3 1.2E-1 1.5E-1 2.0E+0 6.6E-2 4.9E-1 8.1E-3 EFII-CF-42 7.4E-4 9.4E-3 3.6E-4 4.2E-3 6.0E-3 1.1E-1 8.1E-2 6.6E-2 2.5E-3 1.4E-1 2.6E-3 EFII-CF-43 7.2E-4 9.1E-3 3.3E-4 4.1E-3 4.2E-3 1.4E-1 1.3E-1 3.0E+0 3.1E-1 1.1E+0 2.4E-2 EFII-CF-44 6.6E-4 6.0E-3 3.6E-4 1.4E-3 2.3E-3 3.2E-2 3.4E-2 4.1E-2 8.9E-3 1.1E-1 2.7E-3 EFII-CF-45 8.5E-4 1.2E-2 6.6E-4 2.4E-3 2.9E-3 9.9E-2 7.7E-2 2.2E-1 1.6E-2 1.0E-1 1.3E-3 EFII-CF-46 2.1E-3 9.2E-3 6.6E-4 3.8E-3 4.8E-3 1.1E-1 1.6E-1 4.8E-2 3.1E-3 2.2E-1 1.3E-3 EFII-CF-47 1.1E-3 7.5E-3 3.8E-4 2.6E-3 1.2E-2 1.6E-1 1.3E-1 9.6E-2 1.3E-2 5.5E-1 1.9E-3 EFII-CF-48 6.6E-4 1.4E-2 4.0E-4 8.6E-3 1.3E-2 2.1E-1 1.7E-1 4.7E-1 1.3E-2 2.9E-1 8.1E-3 EFII-CF-49 4.8E-4 1.4E-2 4.8E-4 6.2E-3 7.1E-3 1.9E-1 1.5E-1 9.1E-2 1.9E-2 5.5E-1 5.1E-3 EFII-CF-50 7.6E-4 4.3E-3 2.0E-4 2.9E-3 3.4E-2 1.2E-1 9.8E-2 2.3E-2 3.2E-3 3.9E-1 3.9E-3
* K Ca TF.
40
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Sample code Li Be V Ga As Mo Cd Cs Ba La Ce Pr Nd
mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg EPII-SD-11 2.8E+1 1.2E+0 1.2E+2 5.1E+0 1.3E+1 2.9E-1 1.6E-1 3.5E+0 2.5E+2 1.5E+1 4.0E+1 3.9E+0 1.5E+1 EPII-SD-12 5.0E+1 1.9E+0 8.9E+1 5.6E+0 7.4E+0 4.0E-1 3.6E-1 6.6E+0 2.7E+2 2.5E+1 6.0E+1 6.2E+0 2.3E+1 EPII-SD-13 4.3E+1 1.9E+0 8.1E+1 4.8E+0 7.5E+0 4.7E-1 2.7E-1 6.5E+0 1.6E+2 1.1E+1 3.2E+1 2.8E+0 1.1E+1 EPII-SD-14 3.1E+1 1.5E+0 6.0E+1 6.5E+0 5.5E+0 7.6E-1 3.3E-1 6.3E+0 4.0E+2 2.2E+1 4.5E+1 5.1E+0 1.9E+1 EPII-SD-15 2.1E+1 9.0E-1 1.2E+2 5.0E+0 6.1E+0 7.3E-1 4.2E-1 1.7E+0 2.9E+2 1.0E+1 2.5E+1 2.7E+0 1.1E+1 EPII-SD-16 1.3E+1 1.1E+0 1.2E+2 5.6E+0 7.2E+0 7.7E-1 4.7E-1 2.0E+0 3.0E+2 1.6E+1 3.3E+1 4.0E+0 1.7E+1 EPII-SD-17 2.2E+1 1.1E+0 9.4E+1 5.1E+0 1.2E+1 9.1E-1 5.8E-1 3.5E+0 2.6E+2 1.0E+1 2.6E+1 3.0E+0 1.2E+1 EPII-SD-18 2.9E+1 1.3E+0 1.9E+2 5.1E+0 1.3E+1 9.1E-1 5.3E-1 2.5E+0 2.0E+2 2.0E+1 3.4E+1 6.1E+0 2.5E+1 EPII-SD-19 2.1E+1 8.0E-1 8.1E+1 5.5E+0 1.6E+1 1.2E+0 3.9E-1 4.5E+0 4.1E+2 1.4E+1 3.2E+1 3.8E+0 1.5E+1 EPII-SD-20 2.5E+1 1.2E+0 1.3E+2 6.8E+0 1.8E+1 8.5E-1 2.8E-1 5.4E+0 5.0E+2 1.7E+1 4.0E+1 4.3E+0 1.7E+1 EFII-SD-31 3.6E+1 8.1E-1 7.5E+1 4.6E+0 1.2E+1 1.5E+0 3.8E-1 4.4E+0 2.3E+2 1.4E+1 3.9E+1 3.6E+0 1.4E+1 EFII-SD-32 1.5E+1 1.1E+0 1.2E+2 4.5E+0 6.9E+0 1.6E+0 4.4E-1 2.4E+0 1.5E+2 1.4E+1 2.6E+1 3.9E+0 1.6E+1 EFII-SD-33 3.4E+1 1.4E+0 1.2E+2 4.7E+0 8.1E+0 8.4E-1 2.4E-1 4.5E+0 1.9E+2 1.6E+1 3.6E+1 4.5E+0 1.7E+1 EFII-SD-34 2.9E+1 1.2E+0 9.5E+1 4.6E+0 1.9E+1 8.5E-1 6.6E-1 4.9E+0 2.1E+2 1.7E+1 3.8E+1 4.4E+0 1.7E+1 EFII-SD-35 3.2E+1 1.5E+0 8.2E+1 4.9E+0 1.8E+1 1.7E+0 4.5E-1 4.8E+0 1.6E+2 1.3E+1 2.4E+1 3.6E+0 1.5E+1 EFII-SD-36 4.1E+1 9.0E-1 1.4E+2 4.8E+0 2.3E+1 1.0E+0 6.2E-1 1.7E+0 1.6E+2 9.7E+0 2.4E+1 2.9E+0 1.3E+1 EFII-SD-37 2.8E+1 9.5E-1 7.4E+1 5.4E+0 1.3E+1 1.5E+0 3.2E-1 3.4E+0 3.6E+2 1.5E+1 3.4E+1 3.6E+0 1.4E+1 EFII-SD-38 3.9E+1 1.8E+0 1.4E+2 6.3E+0 2.0E+1 2.4E+0 5.2E-1 6.9E+0 2.7E+2 2.3E+1 5.3E+1 5.4E+0 2.1E+1 EFII-SD-39 2.6E+1 1.2E+0 1.5E+2 6.1E+0 1.7E+1 1.4E+0 4.1E-1 5.9E+0 3.3E+2 1.6E+1 4.0E+1 4.5E+0 1.8E+1 EFII-SD-40 9.0E+0 4.8E-1 9.3E+1 4.5E+0 6.6E+0 1.3E+0 4.1E-1 1.3E+0 2.0E+2 7.6E+0 1.7E+1 2.5E+0 1.2E+1
Sample code Sm Eu Gd Tb Dy Ho Er Tm Yb Lu Pb Th U
mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg EPII-SD-11 3.1E+0 7.6E-1 3.3E+0 3.4E-1 2.5E+0 5.2E-1 1.5E+0 2.2E-1 1.5E+0 2.1E-1 1.2E+1 6.1E+0 2.0E+0
EPII-SD-12 4.2E+0 8.3E-1 3.8E+0 3.7E-1 2.4E+0 4.8E-1 1.4E+0 2.1E-1 1.5E+0 2.1E-1 2.4E+1 5.7E+0 3.3E+0 EPII-SD-13 2.0E+0 4.2E-1 2.1E+0 1.9E-1 1.6E+0 3.5E-1 1.1E+0 1.7E-1 1.2E+0 1.8E-1 2.5E+1 3.8E+0 2.7E+0
EPII-SD-14 4.1E+0 9.8E-1 4.5E+0 5.9E-1 4.2E+0 8.9E-1 2.7E+0 4.0E-1 2.8E+0 4.2E-1 2.3E+1 1.0E+1 3.7E+0
EPII-SD-15 2.5E+0 8.4E-1 2.8E+0 3.5E-1 2.8E+0 6.0E-1 1.9E+0 2.8E-1 2.0E+0 2.9E-1 1.5E+1 3.2E+0 2.3E+0 EPII-SD-16 4.1E+0 1.2E+0 4.8E+0 6.7E-1 4.8E+0 1.0E+0 3.0E+0 4.3E-1 2.9E+0 4.4E-1 1.6E+1 5.0E+0 2.2E+0
EPII-SD-17 2.9E+0 8.6E-1 3.2E+0 4.2E-1 3.2E+0 6.8E-1 2.1E+0 3.2E-1 2.3E+0 3.3E-1 3.4E+1 3.5E+0 2.7E+0
EPII-SD-18 5.5E+0 1.4E+0 5.8E+0 7.6E-1 4.9E+0 1.0E+0 3.0E+0 4.2E-1 2.8E+0 4.1E-1 2.0E+1 7.1E+0 3.0E+0
EPII-SD-19 3.6E+0 8.4E-1 4.2E+0 5.9E-1 4.3E+0 9.0E-1 2.8E+0 4.0E-1 2.8E+0 4.1E-1 2.0E+1 5.4E+0 2.8E+0
EPII-SD-20 3.7E+0 1.0E+0 4.1E+0 5.3E-1 3.7E+0 7.6E-1 2.3E+0 3.3E-1 2.3E+0 3.4E-1 2.1E+1 6.8E+0 2.5E+0
EFII-SD-31 2.8E+0 5.9E-1 2.9E+0 3.7E-1 2.6E+0 5.4E-1 1.7E+0 2.6E-1 1.8E+0 2.7E-1 2.8E+1 8.5E+0 3.1E+0
EFII-SD-32 3.8E+0 1.0E+0 4.1E+0 5.9E-1 4.0E+0 8.4E-1 2.6E+0 3.7E-1 2.6E+0 3.8E-1 1.6E+1 5.5E+0 2.2E+0
EFII-SD-33 3.6E+0 7.8E-1 3.4E+0 4.4E-1 2.9E+0 6.0E-1 1.9E+0 2.8E-1 2.0E+0 2.9E-1 2.0E+1 5.6E+0 2.7E+0
EFII-SD-34 3.5E+0 8.9E-1 3.5E+0 4.4E-1 2.8E+0 5.6E-1 1.7E+0 2.4E-1 1.6E+0 2.4E-1 2.6E+1 5.6E+0 2.8E+0
EFII-SD-35 3.1E+0 6.6E-1 3.0E+0 4.1E-1 2.8E+0 6.0E-1 1.9E+0 2.9E-1 2.1E+0 3.1E-1 2.9E+1 4.4E+0 2.6E+0
EFII-SD-36 3.0E+0 8.1E-1 3.3E+0 4.8E-1 3.3E+0 7.0E-1 2.2E+0 3.2E-1 2.3E+0 3.4E-1 2.8E+1 2.7E+0 2.0E+0
EFII-SD-37 2.8E+0 8.3E-1 2.9E+0 3.9E-1 2.7E+0 5.6E-1 1.7E+0 2.5E-1 1.8E+0 2.6E-1 2.2E+1 5.6E+0 1.8E+0
EFII-SD-38 4.3E+0 8.7E-1 4.4E+0 6.0E-1 3.8E+0 7.5E-1 2.3E+0 3.2E-1 2.2E+0 3.1E-1 3.1E+1 8.3E+0 3.9E+0
EFII-SD-39 4.2E+0 1.1E+0 4.6E+0 6.9E-1 4.5E+0 9.4E-1 2.9E+0 4.2E-1 2.9E+0 4.3E-1 2.6E+1 7.1E+0 3.0E+0
EFII-SD-40 3.5E+0 1.1E+0 4.5E+0 7.3E-1 5.1E+0 1.1E+0 3.4E+0 5.0E-1 3.4E+0 5.2E-1 8.5E+0 1.8E+0 2.5E+0
41
2.3-13 27
Sample code Li Be V Ga As Mo Cd Cs Ba La Ce Pr Nd mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg
EPII-CF-11 2.8E-3 1.2E-3 1.8E-2 3.5E-3 1.8E-1 4.6E-1 2.4E-2 5.4E-3 5.5E-1 3.3E-4 2.2E-3 n.d. 1.4E-4 EPII-CF-12 7.2E-3 1.7E-3 3.0E-2 4.9E-3 9.1E-2 7.8E-1 2.7E-2 3.0E-3 7.1E-1 1.5E-3 4.6E-3 n.d. 1.3E-3
EPII-CF-13 8.1E-3 1.5E-3 2.5E-2 4.1E-3 3.0E-1 7.8E-1 8.5E-3 5.9E-3 5.1E-1 1.5E-3 4.5E-3 n.d. 1.2E-3 EPII-CF-14 6.7E-3 1.7E-3 2.5E-2 2.5E-3 6.5E-2 6.1E-1 2.6E-2 2.0E-2 4.1E-1 6.2E-4 2.2E-3 n.d. 3.6E-4
EPII-CF-15 5.2E-3 1.1E-3 1.4E-2 3.4E-3 5.0E-2 1.1E+0 5.5E-2 3.2E-3 4.8E-1 3.4E-4 1.5E-3 n.d. 4.1E-4
EPII-CF-16 4.5E-3 9.4E-4 1.4E-2 3.0E-3 4.6E-2 3.9E-1 1.7E-2 2.1E-3 3.7E-1 3.6E-4 1.9E-3 n.d. 2.6E-4 EPII-CF-17 5.1E-3 7.0E-4 1.1E-2 2.5E-3 9.1E-2 6.1E-1 1.0E-1 7.8E-3 3.3E-1 4.7E-4 1.3E-3 n.d. 1.8E-4
EPII-CF-18 3.2E-3 9.0E-4 6.9E-3 1.6E-3 3.0E-1 3.8E-1 2.2E-2 7.5E-3 1.6E-1 3.2E-4 5.2E-4 n.d. 1.5E-4
EPII-CF-19 3.0E-3 2.8E-4 1.6E-2 8.4E-4 9.5E-2 4.8E-1 2.1E-2 1.7E-3 1.0E-1 2.9E-4 1.0E-3 n.d. 2.9E-4 EPII-CF-20 2.4E-3 4.0E-4 1.2E-2 1.3E-3 1.4E-1 7.7E-1 2.2E-2 6.0E-3 9.7E-2 2.0E-4 6.7E-4 n.d. 3.5E-4 EFII-CF-31 7.9E-3 2.7E-3 5.8E-2 1.4E-2 3.4E-2 7.4E-1 3.1E-2 1.0E-2 9.6E-1 7.3E-3 6.2E-3 1.4E-3 5.6E-3
EFII-CF-32 8.6E-3 2.6E-3 5.3E-2 9.0E-3 3.1E-2 4.9E-1 4.6E-2 6.5E-2 3.7E-1 1.8E-3 3.3E-3 3.9E-4 1.8E-3
EFII-CF-33 1.6E-2 3.0E-3 1.4E-1 2.7E-2 3.0E-2 3.3E-1 4.6E-2 2.8E-2 2.6E+0 4.8E-3 6.8E-3 9.6E-4 3.5E-3 EFII-CF-34 1.5E-2 3.8E-3 1.5E-1 1.1E-2 3.4E-2 3.7E-1 9.0E-2 7.5E-3 6.6E-1 5.2E-3 1.1E-2 1.2E-3 5.0E-3
EFII-CF-35 1.5E-2 3.0E-3 4.7E-2 1.4E-2 2.1E-2 3.4E-1 7.3E-2 2.6E-2 1.2E+0 2.2E-3 3.9E-3 4.5E-4 1.7E-3
EFII-CF-36 7.6E-3 2.4E-3 5.1E-2 9.3E-3 2.9E-2 5.1E-1 1.4E-1 8.8E-3 5.8E-1 2.2E-3 3.4E-3 4.9E-4 1.9E-3
EFII-CF-37 1.0E-2 2.2E-3 5.0E-2 8.8E-3 2.1E-2 3.5E-1 5.5E-2 1.1E-2 4.2E-1 6.4E-3 1.1E-2 1.4E-3 5.2E-3
EFII-CF-38 1.2E-2 2.6E-3 5.5E-2 1.5E-2 2.3E-2 4.2E-1 7.8E-2 7.7E-3 1.3E+0 8.3E-3 1.4E-2 1.6E-3 6.2E-3
EFII-CF-39 8.3E-3 2.6E-3 5.6E-2 8.0E-3 2.1E-2 1.7E-1 5.6E-2 3.9E-2 6.4E-1 6.5E-3 1.1E-2 1.2E-3 5.2E-3
EFII-CF-40 4.5E-3 2.0E-3 3.1E-2 4.6E-3 4.5E-3 3.1E-1 2.8E-2 3.1E-2 2.0E-1 9.6E-4 1.5E-3 1.9E-4 9.3E-4
Sample code Sm Eu Gd Tb Dy Ho Er Tm Yb Lu Pb Th U
mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg mg/kg EPII-CF-11 n.d. n.d. 4.2E-4 n.d. n.d. n.d. 2.9E-4 n.d. 1.7E-4 n.d. 7.5E-3 2.3E-3 5.4E-5 EPII-CF-12 n.d. n.d. 3.6E-4 n.d. n.d. n.d. 2.8E-4 n.d. 1.4E-4 n.d. 7.3E-3 1.2E-3 2.6E-4
EPII-CF-13 n.d. n.d. 4.3E-4 n.d. n.d. n.d. 2.5E-4 n.d. 2.5E-4 n.d. 6.0E-3 9.0E-4 1.8E-4
EPII-CF-14 n.d. n.d. 5.0E-5 n.d. n.d. n.d. 1.9E-4 n.d. 1.1E-4 n.d. 3.8E-3 5.5E-4 1.6E-4 EPII-CF-15 n.d. n.d. 1.1E-4 n.d. n.d. n.d. 1.1E-4 n.d. 6.3E-5 n.d. 1.8E-3 3.8E-4 1.1E-4
EPII-CF-16 n.d. n.d. 4.7E-4 n.d. n.d. n.d. 3.0E-4 n.d. 9.4E-5 n.d. 5.9E-3 2.7E-4 6.0E-5
EPII-CF-17 n.d. n.d. 1.6E-4 n.d. n.d. n.d. 1.1E-4 n.d. 1.0E-4 n.d. 1.3E-3 3.2E-4 9.2E-5 EPII-CF-18 n.d. n.d. 3.9E-5 n.d. n.d. n.d. 1.8E-4 n.d. 7.3E-5 n.d. 2.2E-3 2.1E-4 3.4E-5
EPII-CF-19 n.d. n.d. 3.0E-4 n.d. n.d. n.d. 2.5E-4 n.d. 1.1E-4 n.d. 4.6E-4 2.4E-4 5.8E-5 EPII-CF-20 n.d. n.d. 3.9E-5 n.d. n.d. n.d. 9.6E-5 n.d. 1.1E-4 n.d. 3.4E-4 1.4E-4 3.2E-5
EFII-CF-31 1.8E-3 2.5E-4 1.4E-3 n.d. 6.1E-4 2.5E-4 7.3E-4 1.2E-4 5.2E-4 7.2E-5 2.9E-2 5.7E-4 3.0E-4
EFII-CF-32 9.8E-4 5.1E-5 7.0E-4 n.d. 3.2E-5 8.7E-5 2.7E-4 3.5E-5 3.5E-4 5.5E-5 9.6E-3 4.5E-4 2.0E-4 EFII-CF-33 1.3E-3 5.5E-4 9.2E-4 n.d. 4.3E-4 1.7E-4 3.5E-4 9.3E-5 5.2E-4 6.6E-5 1.3E-2 7.9E-4 6.0E-4
EFII-CF-34 1.5E-3 3.4E-4 1.4E-3 n.d. 3.8E-4 3.1E-4 6.4E-4 1.6E-4 7.5E-4 2.7E-4 1.7E-2 1.5E-3 2.1E-3
EFII-CF-35 1.1E-3 3.4E-4 5.1E-4 n.d. 3.1E-4 1.9E-4 3.3E-4 1.1E-4 3.1E-4 3.1E-4 9.9E-3 5.1E-4 2.3E-4
EFII-CF-36 1.1E-3 3.0E-4 8.8E-4 n.d. 5.9E-4 1.6E-4 3.0E-4 1.1E-4 3.6E-4 2.7E-4 1.1E-2 3.0E-4 3.2E-4
EFII-CF-37 1.3E-3 3.4E-4 1.4E-3 n.d. 1.1E-3 2.0E-4 5.4E-4 8.1E-5 5.3E-4 2.5E-4 1.5E-2 1.3E-3 6.4E-4
EFII-CF-38 1.8E-3 3.3E-4 1.3E-3 n.d. 1.3E-3 2.1E-4 5.2E-4 9.5E-5 6.0E-4 2.5E-4 1.4E-2 2.0E-3 1.2E-3
EFII-CF-39 1.8E-3 3.9E-4 1.3E-3 n.d. 1.0E-3 2.6E-4 7.0E-4 1.3E-4 8.8E-4 3.4E-4 3.7E-2 1.3E-3 8.7E-4
EFII-CF-40 6.2E-4 1.3E-4 4.5E-4 n.d. 2.7E-4 1.3E-4 3.0E-4 7.2E-5 2.9E-4 2.2E-4 6.6E-3 1.9E-4 5.2E-4
42
2.3-14 27
Sample code Sm Eu Gd Tb Dy Ho Er Tm Yb Lu Pb Th U EPII-CF-11 − − 1.3E-4 − − − 1.9E-4 − 1.2E-4 − 6.5E-4 3.7E-4 2.7E-5 EPII-CF-12 − − 9.5E-5 − − − 2.0E-4 − 9.6E-5 − 3.0E-4 2.1E-4 8.0E-5 EPII-CF-13 − − 2.0E-4 − − − 2.3E-4 − 2.0E-4 − 2.4E-4 2.4E-4 6.5E-5 EPII-CF-14 − − 1.1E-5 − − − 7.0E-5 − 4.0E-5 − 1.6E-4 5.4E-5 4.2E-5 EPII-CF-15 − − 3.9E-5 − − − 5.9E-5 − 3.2E-5 − 1.2E-4 1.2E-4 4.8E-5 EPII-CF-16 − − 9.9E-5 − − − 9.9E-5 − 3.2E-5 − 3.7E-4 5.3E-5 2.7E-5 EPII-CF-17 − − 5.1E-5 − − − 5.3E-5 − 4.4E-5 − 3.9E-5 9.0E-5 3.4E-5 EPII-CF-18 − − 6.7E-6 − − − 5.9E-5 − 2.6E-5 − 1.1E-4 2.9E-5 1.1E-5 EPII-CF-19 − − 7.2E-5 − − − 8.8E-5 − 3.8E-5 − 2.3E-5 4.5E-5 2.1E-5 EPII-CF-20 − − 9.5E-6 − − − 4.2E-5 − 4.8E-5 − 1.6E-5 2.1E-5 1.3E-5 EFII-CF-31 6.4E-4 4.2E-4 5.0E-4 − 2.3E-4 4.6E-4 4.2E-4 4.5E-4 2.8E-4 2.7E-4 1.1E-3 6.7E-5 9.9E-5 EFII-CF-32 2.6E-4 5.1E-5 1.7E-4 − 8.1E-6 1.0E-4 1.0E-4 9.5E-5 1.4E-4 1.5E-4 6.0E-4 8.3E-5 9.3E-5 EFII-CF-33 3.7E-4 7.1E-4 2.7E-4 − 1.5E-4 2.8E-4 1.8E-4 3.3E-4 2.6E-4 2.2E-4 6.6E-4 1.4E-4 2.2E-4 EFII-CF-34 4.2E-4 3.8E-4 4.0E-4 − 1.4E-4 5.5E-4 3.8E-4 7.0E-4 4.6E-4 1.2E-3 6.5E-4 2.7E-4 7.5E-4 EFII-CF-35 3.5E-4 5.1E-4 1.7E-4 − 1.1E-4 3.2E-4 1.8E-4 4.0E-4 1.5E-4 1.0E-3 3.4E-4 1.2E-4 8.8E-5 EFII-CF-36 3.8E-4 3.7E-4 2.7E-4 − 1.8E-4 2.3E-4 1.4E-4 3.5E-4 1.6E-4 8.1E-4 3.8E-4 1.1E-4 1.6E-4 EFII-CF-37 4.8E-4 4.1E-4 4.7E-4 − 4.2E-4 3.6E-4 3.1E-4 3.2E-4 3.0E-4 9.7E-4 6.8E-4 2.4E-4 3.5E-4 EFII-CF-38 4.3E-4 3.8E-4 3.0E-4 − 3.5E-4 2.8E-4 2.3E-4 3.0E-4 2.7E-4 7.9E-4 4.6E-4 2.4E-4 3.0E-4 EFII-CF-39 4.3E-4 3.6E-4 2.9E-4 − 2.3E-4 2.8E-4 2.4E-4 3.1E-4 3.0E-4 7.9E-4 1.4E-3 1.8E-4 2.8E-4 EFII-CF-40 1.8E-4 1.1E-4 1.0E-4 − 5.3E-5 1.1E-4 8.8E-5 1.4E-4 8.4E-5 4.2E-4 7.8E-4 1.0E-4 2.1E-4
Sample code Li Be V Ga As Mo Cd Cs Ba La Ce Pr Nd
EPII-CF-11 1.0E-4 9.9E-4 1.5E-4 7.0E-4 1.4E-2 1.6E+0 1.5E-1 1.6E-3 2.2E-3 2.2E-5 5.4E-5 9.2E-6
EPII-CF-12 1.4E-4 8.7E-4 3.4E-4 8.8E-4 1.2E-2 2.0E+0 7.6E-2 4.5E-4 2.6E-3 6.3E-5 7.6E-5 5.7E-5
EPII-CF-13 1.9E-4 8.1E-4 3.1E-4 8.5E-4 4.0E-2 1.7E+0 3.2E-2 9.1E-4 3.2E-3 1.4E-4 1.4E-4 1.1E-4
EPII-CF-14 2.2E-4 1.2E-3 4.1E-4 3.9E-4 1.2E-2 8.0E-1 7.6E-2 3.2E-3 1.0E-3 2.8E-5 4.9E-5 1.9E-5
EPII-CF-15 2.5E-4 1.2E-3 1.2E-4 6.9E-4 8.3E-3 1.5E+0 1.3E-1 1.9E-3 1.7E-3 3.4E-5 6.0E-5 3.7E-5
EPII-CF-16 3.5E-4 8.8E-4 1.2E-4 5.4E-4 6.4E-3 5.1E-1 3.5E-2 1.1E-3 1.2E-3 2.3E-5 5.7E-5 1.5E-5
EPII-CF-17 2.3E-4 6.1E-4 1.1E-4 5.0E-4 7.6E-3 6.7E-1 1.8E-1 2.2E-3 1.3E-3 4.5E-5 5.1E-5 1.5E-5
EPII-CF-18 1.1E-4 6.8E-4 3.7E-5 3.1E-4 2.4E-2 4.1E-1 4.2E-2 3.0E-3 7.8E-4 1.6E-5 1.5E-5 5.9E-6
EPII-CF-19 1.4E-4 3.5E-4 1.9E-4 1.5E-4 5.8E-3 4.1E-1 5.5E-2 3.8E-4 2.5E-4 2.0E-5 3.2E-5 1.9E-5
EPII-CF-20 9.3E-5 3.4E-4 8.7E-5 1.9E-4 7.8E-3 9.0E-1 7.7E-2 1.1E-3 1.9E-4 1.2E-5 1.7E-5 2.0E-5
EFII-CF-31 2.2E-4 3.4E-3 7.8E-4 3.0E-3 2.9E-3 4.8E-1 8.1E-2 2.4E-3 4.1E-3 5.3E-4 1.6E-4 3.9E-4 4.1E-4
EFII-CF-32 5.7E-4 2.4E-3 4.4E-4 2.0E-3 4.5E-3 3.0E-1 1.0E-1 2.7E-2 2.4E-3 1.3E-4 1.3E-4 9.9E-5 1.1E-4
EFII-CF-33 4.6E-4 2.1E-3 1.2E-3 5.8E-3 3.7E-3 3.9E-1 1.9E-1 6.4E-3 1.4E-2 2.9E-4 1.9E-4 2.2E-4 2.0E-4
EFII-CF-34 5.0E-4 3.1E-3 1.5E-3 2.4E-3 1.8E-3 4.4E-1 1.4E-1 1.5E-3 3.1E-3 3.2E-4 2.9E-4 2.7E-4 2.9E-4
EFII-CF-35 4.6E-4 2.0E-3 5.8E-4 3.0E-3 1.2E-3 2.0E-1 1.6E-1 5.5E-3 7.8E-3 1.7E-4 1.6E-4 1.2E-4 1.2E-4
EFII-CF-36 1.9E-4 2.7E-3 3.7E-4 1.9E-3 1.2E-3 4.8E-1 2.2E-1 5.4E-3 3.7E-3 2.3E-4 1.4E-4 1.7E-4 1.5E-4
EFII-CF-37 3.8E-4 2.3E-3 6.8E-4 1.6E-3 1.6E-3 2.3E-1 1.7E-1 3.3E-3 1.1E-3 4.2E-4 3.4E-4 4.0E-4 3.8E-4
EFII-CF-38 3.1E-4 1.4E-3 4.0E-4 2.4E-3 1.2E-3 1.8E-1 1.5E-1 1.1E-3 4.7E-3 3.6E-4 2.6E-4 3.0E-4 3.0E-4
EFII-CF-39 3.2E-4 2.1E-3 3.8E-4 1.3E-3 1.2E-3 1.2E-1 1.3E-1 6.5E-3 1.9E-3 4.0E-4 2.7E-4 2.6E-4 2.8E-4
EFII-CF-40 5.0E-4 4.1E-3 3.3E-4 1.0E-3 6.8E-4 2.4E-1 6.7E-2 2.4E-2 9.9E-4 1.3E-4 9.1E-5 7.5E-5 7.6E-5
43
2.4-1 - 2016
, ˚C 5-9 , ˚C
7.5 (-3.7 – 20.2) 15.8
10.6 (-0.7 – 23.3) 18.8
11.7 (0.1 – 24.9) 20.4
10.4 (-0.8 – 22.8) 18.6
10.1 18.4
23.9 (7.5 – 27.0) 23.9
24.8 (5.7 – 28.2) 24.8
24.4 (7.5 – 27.3) 24.4
26.0 (11.7 – 28.5) 26.0 27.2 (17.0 – 28.9) 27.2
19.0 25.3
2.4-2
*1 mg/100g. *2 g/kg. *3 p<0.05, p<0.01.
(mg/kg)
GM t n GM (A) GSD n GM (B) GSD A/B p
Na 26 1.2E+4 1.3 21 1.1E+4 2.1 1.1 0.643 Mg 26 6.2E+3 1.6 21 5.5E+3 2.1 1.1 0.535 Al 26 7.3E+4 1.3 21 7.2E+4 1.5 1.0 0.939 Si 25 2.6E+5 1.1 21 2.7E+5 1.2 1.0 0.252 P 25 1.6E+3 1.6 21 1.7E+3 2.1 1.0 0.808 K 26 9.3E+3 1.5 21 1.2E+4 1.5 0.8 0.024 Ca 26 1.2E+4 1.6 21 9.4E+3 3.0 1.3 0.341 Cr 26 4.9E+1 1.7 21 6.1E+1 2.2 0.8 0.289 Mn 26 5.6E+2 1.9 21 5.4E+2 1.7 1.0 0.800 Fe 26 3.9E+4 1.3 21 3.3E+4 1.5 1.2 0.105 Co 26 1.2E+1 1.5 21 1.1E+1 1.7 1.1 0.619 Ni 26 2.0E+1 1.9 21 1.9E+1 2.1 1.1 0.706 Cu 26 2.5E+1 1.4 21 2.9E+1 2.0 0.9 0.430 Zn 26 1.0E+2 1.2 21 8.8E+1 1.4 1.2 0.031 Sr 26 9.0E+1 1.7 21 1.0E+2 1.9 0.9 0.458 Cd 26 3.5E-1 1.5 21 2.5E-1 1.6 1.4 0.017 Ba 26 2.6E+2 1.4 21 2.9E+2 1.3 0.9 0.290
Ca*1 25 1.7E+2 1.5 21 1.2E+2 1.8 1.5 0.015 *1 25 2.1E+1 1.6 21 1.6E+1 1.8 1.3 0.119
Al*2 25 4.2E+0 2.1 21 4.1E+0 2.7 1.0 0.896 Fe*2 25 9.0E+0 1.6 21 4.4E+0 1.9 2.1 0.000
pH*3 25 5.4 5.9 0.002
44
2.4-3
p<0.05, p<0.01.
2.4-4
*1 mg/kg TF . p<0.05, p<0.01.
(mg/kg)
GM t n GM (A) GSD n GM (B) GSD A/B p
Na 26 1.3E+1 2.9 21 2.4E+1 2.5 0.5 0.036 Mg 26 1.3E+3 1.1 21 1.4E+3 1.2 0.9 0.123 Al 21 1.7E+0 1.9 17 2.9E+0 2.2 0.6 0.032 Si 25 1.2E+2 1.9 21 2.1E+2 2.1 0.6 0.015 P 25 3.1E+3 1.1 21 3.3E+3 1.1 0.9 0.024 K 26 2.6E+3 1.1 21 2.6E+3 1.1 1.0 0.974 Ca 26 9.3E+1 1.3 21 9.8E+1 1.4 1.0 0.564 Cr 26 1.4E-1 3.0 21 1.8E-1 2.8 0.7 0.351 Mn 26 2.8E+1 1.4 21 2.7E+1 1.3 1.0 0.865 Fe 26 9.4E+0 1.3 21 1.3E+1 1.3 0.7 0.000 Co 26 9.4E-3 1.8 21 1.3E-2 1.5 0.7 0.031 Ni 26 2.2E-1 2.7 21 1.8E-1 2.3 1.2 0.477 Cu 26 2.2E+0 1.6 21 3.0E+0 1.4 0.7 0.008 Zn 26 2.1E+1 1.1 21 2.7E+1 1.1 0.8 < .0001 Sr 26 1.7E-1 1.6 21 2.2E-1 1.7 0.7 0.049 Cd 26 2.9E-2 3.3 21 1.7E-2 2.9 1.6 0.140 Ba 26 2.9E-1 2.2 21 5.4E-1 2.1 0.5 0.008
GM t n GM (A) GSD n GM (B) GSD A/B p
Na 26 1.0E-3 3.0 21 2.1E-3 2.9 0.5 0.031 Mg 26 2.1E-1 1.6 21 2.5E-1 2.1 0.8 0.333 Al 21 2.4E-5 2.4 17 4.0E-5 2.7 0.6 0.112 Si 25 4.7E-4 2.0 21 7.7E-4 2.1 0.6 0.025 P 25 2.0E+0 1.7 21 2.0E+0 2.2 1.0 0.888 K 26 2.8E-1 1.6 21 2.2E-1 1.4 1.3 0.024 Ca 26 7.7E-3 1.7 21 1.0E-2 3.0 0.7 0.266 Cr 26 2.8E-3 3.3 21 3.0E-3 3.2 0.9 0.839 Mn 26 4.9E-2 1.8 21 5.1E-2 1.8 1.0 0.856 Fe 26 2.4E-4 1.5 21 3.9E-4 1.7 0.6 0.002 Co 26 8.0E-4 1.6 21 1.2E-3 1.9 0.7 0.022 Ni 26 1.1E-2 2.6 21 9.8E-3 2.5 1.1 0.675 Cu 26 8.9E-2 1.6 21 1.1E-1 2.0 0.8 0.323 Zn 26 2.0E-1 1.2 21 3.0E-1 1.4 0.7 < .0001 Sr 26 1.8E-3 2.0 21 2.2E-3 2.5 0.8 0.457 Cd 26 8.2E-2 3.1 21 6.9E-2 2.9 1.2 0.614 Ba 26 1.1E-3 2.6 21 1.9E-3 2.0 0.6 0.032
Ca*1 25 5.5E-2 1.7 21 8.3E-2 2.0 0.7 0.027 *1 25 1.3E+1 1.7 21 1.7E+1 1.9 0.8 0.122
Al*1 21 4.5E-4 2.6 16 5.6E-4 3.0 0.8 0.530 Fe*1 25 1.3E-2 2.3 21 4.7E-2 3.4 0.3 0.000
45
2.5-1
2.5-2 Cs Kd 30˚C Kd RI
Code 10˚C 23˚C 30˚C
EP-SD-35 4810 1930 2550 ±130 EP-SD-36 3180 680 1310 ±30 EP-SD-37 1610 570 470 ±30 EP-SD-38 4580 2360 2530 ±130 EP-SD-39 7290 7800 8610 ±1170 EP-SD-40 7920 3560 3850 ±230 EP-SD-41 8490 5710 4810 ±80 EP-SD-42 8090 2950 3610 ±240 EP-SD-43 840 340 250 ±30 EP-SD-44 5160 2950 2660 ±280 EP-SD-45 5200 11700 2370 ±10 EP-SD-46 4960 4410 2250 ±40 EP-SD-47 4580 1640 780 ±40 EP-SD-48 6690 6710 3710 ±190 EP-SD-49 2040 880 850 ±50 EP-SD-50 1190 770 450 ±10 EP-SD-51 3900 5030 2070 ±100 EP-SD-52 3340 2340 3240 ±20 EP-SD-53 5370 4470 4810 ±40
EP-SD-54 2350 1500 1370 ±60
GM 3880 2340 1910
GSD 1.9 2.6 2.5
pH Sand Silt Clay EC (1:5) Code H2O (%) (%) (%) (µS/cm)
EP-SD-43 5.8 50 35 15 10.9 108 EP-SD-49 5.2 68 18 14 2.6 77 EP-SD-50 6.1 61 25 14 8.4 97 EP-SD-51 5.6 45 28 27 8.3 72 EP-SD-52 5.2 40 33 27 8.0 88
46
2.6-1 137Cs
2.6-2 Cs Tag: m2 kg-1
2.6-3
11.55 km2 ( : 6.26 km2, : 5.29 km2)
19.7 × 106 m3
26.4 km
1.7 m ( 2.5 m)
22
2.6-4
(cm) (g) 37 8.5-42.0 9-1238 6 45.0-72.0 1012-4777
3 32.5-36.5 584-894 2 14.0-14.5 56-62
2 54.0-55.0 1070-1738 1 40 526
A λa, d-1 Teff y B λb, d-1 Teff y 172 0.00482 0.39 28.5 0.000782 4.7
404 0.00675 0.28 14.9 0.000142 10.5 125 0.00675 0.63 8.3 0.000399 2.7
2016
144 0.00402 0.47 14.9 0.000142 13.4
N GM 95
2790 3.4E-3 4.0E-4 2.9E-2
630 5.5E-3 7.3E-4 4.1E-2
644 3.8E-3 5.6E-4 2.5E-2
47
2.6-5 137Cs
2.6-6 13C 15N
2s-1 2015 2016
*1 2017 *2 5
*1 *2 *2
2015 —
1/1 – 12/31
16.8 -0.6 – 36.8
16.7 (-2.8 – 38.8)
16.6 (0.8 – 28.7)
16.3 (-3.4 – 36.7)
15.4 (2.1 – 28.5)
2016 —
1/1 – 12/31
16.8 (-0.6 – 36.3)
16.6 (-2.4 – 40.0)
16.9 (6.3 – 27.0)
16.2 (-3.4 – 36.2)
15.4 (3.4 – 26.4)
48
2.2-1 Ni, Sr, Mo Pb
49
2.4-1
2.4-2 Fe, Co, Ni, Cu, Zn Sr
10-1
100
101
102
103
104
105
106
10-1 100 101 102 103 104 105 106
GM-ColdGM-Warm
Ele
men
tal c
once
ntra
tion,
mg/
kg
World Average, mg/kg
50
2.5-1 1 30 Cs 3 7 30 Kd pH
p<0.05
102
103
104
P43_1d-3dP43_1d-7dP43_1d-30dP43_30d-7d
Kd
1d-3d 1d-7d 1d-30d 30d-7d
5.0
5.5
6.0
6.5
7.0
P43_1d-3dP43_1d-7dP43_1d-30dP43_30d-7d
pH
1d-3d 1d-7d 1d-30d 30d-7d
102
103
104
P49_1d-3dP49_1d-7dP49_1d-30dP49_30d-7d
Kd
1d-3d 1d-7d 1d-30d 30d-7d
5.0
5.5
6.0
6.5
7.0
P49_1d-3dP49_1d-7dP49_1d-30dP49_30d-7d
pH
1d-3d 1d-7d 1d-30d 30d-7d
102
103
104
P50_1d-3dP50_1d-7dP50_1d-30dP50_30d-7d
Kd
1d-3d 1d-7d 1d-30d 30d-7d
5.0
5.5
6.0
6.5
7.0P50_1d-3dP50_1d-7dP50_1d-30dP50_30d-7d
pH
1d-3d 1d-7d 1d-30d 30d-7d
51
d d RI
2.5-1 1 30 Cs 3 7 30 Kd pHp<0.05
102
103
104
P51_1d-3dP51_1d-7dP51_1d-30dP51_30d-7d
Kd
1d-3d 1d-7d 1d-30d 30d-7d
102
103
104
P52_1d-3dP52_1d-7dP52_1d-30dP52_30d-7d
Kd
1d-3d 1d-7d 1d-30d 30d-7d
5.0
5.5
6.0
6.5
7.0P51_1d-3dP51_1d-7dP51_1d-30dP51_30d-7d
pH
1d-3d 1d-7d 1d-30d 30d-7d
5.0
5.5
6.0
6.5
7.0P52_1d-3dP52_1d-7dP52_1d-30dP52_30d-7d
pH
1d-3d 1d-7d 1d-30d 30d-7d
52
2.5-2 10 23 30˚C Kd-137Cs RI
2.5-3 10 23 30˚C Kd-137Cs
aab b
1500
2000
2500
3000
3500
4000
5 10 15 20 25 30 35
Kd-
Cs
Temperature, ˚C
53
2.6-1 137Cs
1
10
100
1000
0 500 1000 1500 2000
137 C
s co
ncen
tratio
n, B
q kg
-1-d
ry
Days after March 11, 2011
1
10
100
1000
0 500 1000 1500 2000
137 C
s co
ncen
tratio
n, B
q kg
-1-d
ry
Days after March 11, 2011
1
10
100
1000
0 500 1000 1500 2000
137 C
s co
ncen
tratio
n, B
q kg
-1-d
ry
Days after March 11, 2011
54
2.6-2 2012-2016 137Cs
Tag, m2 kg-1
55
2.6-3 2011 11 2016 9
2.6-4 1. 2 3 4 5 6
1
2
3
4
5
6
56
2.6-5 137Cs n % 137Cs
2.6-6
1) 20 mg 2 mL 2) 1.5 mL , 2 1 3) 4) 5,500 × g, 5 , 5) 6) 1.5 mL 7) 5,500 × g, 5 , 8) 9) 6 8 1-2 10) 50˚C 24 11) 12)
57
2.6-7 13C 15N
2.6-8
58
2015.1.1-12.31 2016.1.1-12.31
2015.1.1-12.31 2016.1.1-12.31
2s-1 2015 2016 Air Soil 20cm
2s-2 2015 2016
59
60
MOX
TRU14C 5730
TRU
JAEA and FEPC, 2007 14C
, 1999 14C
14C 14C
14C
Ishii et al., 2015 25 114C
- Kd -
TF 14C
14C
Ishii et al., 2015 14C 14C14C
14C
Frölicher et al., 2014
Castro et al., 2010; Schindlbacher et al., 201114C
pH14C
ATP14C
, 2015 14C14C-
95
, 201614C
61
14C
, 2016
14C 14C 14C 14C
14C
3.2 3.3
3.4
Castro, H. F., Classen, A. T., Austin, E. E., Norby, R. J., & Schadt, C. W. (2010). Soil microbial community
responses to multiple experimental climate change drivers. Appl Environ Microbiol, 76(4), 999-1007.
Frölicher, T. L., Winton, M., & Sarmiento, J. L. (2014). Continued global warming after CO2 emissions
stoppage. Nature Climate Change, 4, 40-44.
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disposal (pp. 303-309). Tokyo: Springer.
Japan Atomic Energy Agency, & The Federation of Electric Power Companies of Japan. (2007). Second
Progress Report on Research and Development for TRU Waste Disposal in Japan Repository Design,
Safety Assessment and Means of Implementation in the Generic Phase . Ibaraki, Japan.
Schindlbacher, A., Rodler, A., Kuffner, M., Kitzler, B., Sessitsch, A., & Zechmeister-Boltenstern, S. (2011). Experimental warming effects on the microbial community of a temperate mountain forest soil. Soil Biol
Biochem, 43(7), 1417-1425.
. (1999). —
2 —.
. (2015). 26
. . . (2016). 27
. .
62
14C
TRU 14C
Kaneko et al.,
2003 14C2013 14C 14C
Ishii et al., 2015 14C
14C
2013
2016 14C 14C
14C [1,2-14C] 14C14C
3.2.1. 14CO214C
, 1990
TRU [1,2-14C] 14C14C 14C
3.2.1.1. 14C 14C
26
63
, 2015
3.2-1 0.5 g-dry < 2 mm 30 mL
5 mL [1,2-14C][1,2-14C] pH 14C 1.7 × 103 Bq/mL 4.2 × 103 Bq/mL
8.6 × 103 Bq/mL 1.7 × 104 Bq/mL 4.2 × 104 Bq/mL 8.4 × 104 Bq/mL 1 0.5 g
8.6 × 103 Bq 4.2 × 105 Bq 14C
0.2 µm
25 15 14CO2
20 mL/min 10 30 mL 14C
63
200 mL
16 g 1 mol/L 314CO2
14C Hionic-Fluor
PerkinElmer Tri-Carb-25WTR Liquid Scintilation Analyzer14C 0-156 KeV 3
dpm 14C 14CO2 3.2-2
4 14CO214CO2
Ishii et al., 2010 4 14CO214C 8.4 × 104 Bq/mL
[1,2-14C] 4.07 × 109 Bq/mmol Bq/mL mol/L
20.6 µmol/L 0.5 g 5 mL
1 kg 2.06 × 10-2 cmol/kg
, 1994 50 14CO2
14C 3.2-2 8.4 × 104 Bq/mL 14C
[1,2-14C] 1 2 5.8 × 104 Bq14C 14CO2 8.6 × 103 Bq/mL 14C [1,2-14C]
14C 4.2 × 104 Bq 14CO2
1 2
8.6 × 103 Bq/mL 14C [1,2-14C] 14CO2
[1,2-14C]14CO2
3.2-3
8.6 × 103 Bq/mL 14C [1,2-14C] 3 1514CO2
14C14CO2
14C [1,2-14C]8.6 × 103 Bq/mL 14C
1
3.2.1.2. 14C [1,2-14C] 3.2.1.1.
[1,2-14C] 14C 8.6 × 103 Bq/mL 15 20 25
30 4 14CO214C 3.2.1.1.
14CO2 3.2-4 4 14CO2
, 2016 4 14CO2
64
25
30
25 2514CO2
14CO2
3.2-5 14CO214C 3.2-4
25 30 4
25 30 14CO214C
14CO2
3.2.2. 14C [1,2-14C] 14C
14C
2 × 10-2 cmol/kg-soil 14CO2
[1,2-14C] 4.07 × 109 Bq/mmol14C 8.4 × 104 Bq/mL 14C
14C- 14C 14CO214CO2
14C
14CO2 25 30 2514CO2
Ishii, N., Koiso, H., Takeda, H., & Uchida, S. (2010). Partitioning of 14C into solid, liquid, and gas phases in
various paddy soils in Japan. Journal of Nuclear Science and Technology, 47(3), 238-243.
Ishii, N., Ogiyama, S., Sakurai, S., Tagami, K., & Uchida, S. (2015). Environmental transfer of carbon-14 in
Japanese paddy fields. In K. Nakajima (Ed.), Nuclear Back-end and transmutation technology for waste
disposal (pp. 303-309). Tokyo: Springer.
Kaneko, S., Tanabe, H., Sasoh, M., Takahashi, R., Shibano, T., & Tateyama, S. (2003). A study on the chemical forms and migration behavior of Carbon-14 leached from the simulated hull waste in the underground
condition. Materials Research Society Proceedings, 757, II3.8.1.
. (1994). . In (Ed.), 19
(pp. 91-118). : .
. (2013).
6 19 24 [ ]. . . (2015). 26
65
. .
. (2016). 27
. .
, , , & . (1990).
. , 61(6), 572-578.
66
14C Ishii et al., 2015
95
, 2016
14CO214CO2
3.3.1.
P2P11 P2
52% 31% 17%
84.7 g/kg 6.4 g/kg P11
36% 35% 29% 21.3 g/kg
2.2 g/kg P2 P11
, 2016
0.5 g-dry < 2 mm 50 mL
0.5 mL
15 20 25 30 7
3
DNA DNA ISOIL for Beads Beating
FastPrep 24 Instrument MP Biomedicals 6 m/sec 45
DNA 16S rRNA (PCR)
PCR 341f-GC 907R
3.3-1 PCR 50 µL 0.25 µL Takara Ex Taq polymerase
Hot Start Version (Takara Bio Inc) 0.5 µL 25 µM 341F-GC forward primer 0.5 µL 25 µM 907R reverse primer 1 µL 0.1% Bovine Serum Albumin (Takara Bio Inc.) 4 µL dNTP Mixture ( 2.5 mM)
5 µL 10 × Ex Taq Buffer 1 µL DNA 50 µL PCR
TProfessional 96 Gradient Thermocycler (Biometra GmbH) touch-down PCR
1) 95 , 60 sec, 2) 94 , 30 sec, 3) 65 , 30 sec, 4) 72 , 60 sec, 5) 94 , 30 sec,
6) 55 , 30 sec, 7) 72 , 60 sec, 8) 72 , 600 sec. 3), 4), 5) 20
3) 0.5 5) 5) 7) 98) PCR PCR QIAquick PCR Purification
67
Kit (QIAGEN) 2100 Bioanalyzer (Agilent) DNA Bp
(ng/µL)
DNA DGGE DGGE
D-code system (Bio-Rad Laboratories, Inc.) 120 ng DNA DGGE
61.5 50V 20 TAE buffer DGGE5.5% (w/v) 45% 60%
100% 7 M + 40% SYBR Gold
Nucleic Acid Gel Stain (ThermoFisher Scientific Inc.) Molecular Imager FX (Bio-Rad
Laboratories, Inc.)
P2 3.3-1
15
15
3.3-1
1 100% 15
P11 3.3-2 P2
P11
3.3.2.
14CO214CO2
P21 P33
P21 [1,2-14C] 7
75% 14C P33 47%, 2015 P21
47% 32% 21% 20.2 g/kg 2.2 g/kg
P33 50%
27% 22% 36.2 g/kg 4.2 g/kg
, 2016
3.3.1. DNA 0.5 g0.5 mL 7 ISOIL for Beads Beating
DNA 30 DNA QIAquick PCR Purification
Kit (QIAGEN) DGGE DGGE
200 ng DNA 62 50V 20
DGGE 6% (w/v)
40% 55% 3.3-3 P21 P33 P21
68
14C P33 , 2015P21 P33 14CO2
, 2006341f-GC/907R
PARCH 340f-GC PARCH 519R 3.3-1 PCR
3.3.3. 14CO2 16S rRNA
DGGE
3.3-3 5 CS0814C CS08
DGGE 40 µL 10mM Tris-Cl (pH8.5)
DNA TOPO TA Cloning Kits for Sequencing kit (ThermoFisher Scientific Inc.)
5 3
Ribosomal Database Project Release 11
3.3-2
MEGA: Molecular Evolutionary
Genetics Analysis Tamura et al. 2007
3.3-4 DNA
Clostridium carboxidivorans, Massilia aerilata, Bacillus niacini, Tumebacillus ginsengisoli, Ramlibacter solisilvae C. carboxidivorans
(Liou et al. 2005) 4M. aerilata Weon et al., 2008 B.
niacini (Nagel and
Andereesen, 1991) T. ginsengisoli (Baek et al, 2011) R. solisilvaeBiolog GN plate (Heulin et al, 2003)
3.3. 4. 14CO2
14CO2
15 30
14CO2
69
14C4
16S rRNA 4 31
14C14C
Baek, S.H., Cui, Y., Kim, S.C., Cui, C.H., Yin, C., Lee, S.T., Im, W.T., 2011. Tumebacillus ginsengisoli sp.
nov., isolated from soil of a ginseng field. International journal of systematic and evolutionary microbiology 61, 1715-1719.
Heulin, T., Barakat, M., Christen, R., Lesourd, M., Sutra, L., De Luca, G., Achouak, W., 2003. Ramlibacter
tataouinensis gen. nov., sp. nov., and Ramlibacter henchirensis sp. nov., cyst-producing bacteria isolated from
subdesert soil in Tunisia. International journal of systematic and evolutionary microbiology 53, 589-594.
Ishii, N., Ogiyama, S., Sakurai, S., Tagami, K., Uchida, S., 2015. Environmental transfer of carbon-14 in
Japanese paddy fields, in: Nakajima, K. (Ed.), Nuclear Back-end and transmutation technology for waste disposal. Springer, Tokyo, pp. 303-309.
Liou, J.S., Balkwill, D.L., Drake, G.R., Tanner, R.S., 2005. Clostridium carboxidivorans sp. nov., a
solvent-producing clostridium isolated from an agricultural settling lagoon, and reclassification of the
acetogen Clostridium scatologenes strain SL1 as Clostridium drakei sp. nov. International journal of
systematic and evolutionary microbiology 55, 2085-2091.
Muyzer, G., Brinkhoff, T., Nübel, U., Santegoeds, C., Schäfer, H., Wawer, C., 2004. Denaturing gradient gel electrophoresis (DGGE) in microbial ecology, in: Kowalchuk, G.A., de Bruijn, F., Head, I.M., Van der Zijpp,
A.J., van Elsas, J.D. (Eds.), Molecular Microbial Ecology Manual. Springer Netherlands, Netherlands.
Muyzer, G., de Waal, E., Uitterlinden, A., 1993. Profiling of complex microbial populations by denaturing
gradient gel electrophoresis analysis of polymerase chain reaction-amplified genes coding for 16S rRNA.
Applied and environmental microbiology 59, 695-700.
Nagel, M., Andreesen, J.R., 1991. Bacillus niacini sp. nov. a Nicotinate-Metabolizing Mesophile Isolated from Soil. International journal of systematic and evolutionary microbiology 41, 134-139.
Ovreås, L., Forney, L., Daae, F.L., Torsvik, V., 1997. Distribution of bacterioplankton in meromictic Lake
Saelenvannet, as determined by denaturing gradient gel electrophoresis of PCR-amplified gene fragments
coding for 16S rRNA. Applied and environmental microbiology 63, 3367-3373.
Tamura, K., Dudley, J., Nei, M., Kumar, S., 2007. MEGA4: Molecular Evolutionary Genetics Analysis
(MEGA) software version 4.0. Molecular biology and evolution 24, 1596-1599. Weon, H.Y., Kim, B.Y., Son, J.A., Jang, H.B., Hong, S.K., Go, S.J., Kwon, S.W., 2008. Massilia aerilata sp.
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1422-1425.
, , 2006. .
5, 81-89.
, 2015. 26 , .
70
, 2016. 27
, .
71
14C 14C
3.4-1 TRU14C
14C14C Ishii et al., 2015
14C
3.4.1.
3
3.4.1.1.
• • 3.4-1
72
• PREP (Homma and Saltelli, 1992)
• 100
• day
•
PREP
3.4-2
3.4.1.2.
14C
3.4-3 14C 3.4-414C 14C
1
3.4-5 14C 14C
1
2
14C
3.4-6 1 14C 3.4-7 14C14C 1 1
14C 2
3.4-8 14C 12
14C
14C 14C 114C
3.4.1.3. 14C
SPOP (Saltelli and Homma, 1992)
PCC Partial Correlation Coefficient
PRCC Partial Rank Correlation Coefficient PCC
squrious correlation
x,y,z x,y Rxy,x z Rxz y z
73
Ryz z Rxy.z 1 R 1
1
(3.4-1)
PRCC
PRCC 1 R 1 1
(3.4-2)
3.4-2 PCC PRCC
6
1
4 14C 3.4-9
2 1
14C14C
3.4.2.
Migration Of GRound Additions (MOGRA)
Amano, 2003 14C 3.4-1
3.4.2.1.
50 m × 20 m DS 2, Decagon Devices, Inc. 3.4-10
3 21 cm
18 cm 108 cm 94 cm
3.4-3
10 6 24
1 2018 6 15 9 7 8
74
1 6 15
3.4-11
3.4-4 3.4-5
0˚ 315˚ 0˚45˚ 135˚ 225˚
45˚ 135˚ 225˚ 315˚
1/2
0.7 m/s
0.92 0.30 m/s0.28 m/s (=0.92 × 0.30)
2 7 12
3.4-12
3.4-6 3.4-7
1 m/s
1
0.4 m/s
1 m/s
0.64 0.36
0.00
0.26 m/s
0.09 m/s (=0.36 × 0.26)
3 7 20 3.4-13
3.4-8 3.4-9
1/2
2 1 m/s
6:40 8:40
75
6:40 15 0.3 m/s
0.5 m/s 1/2
0.29 0.62 0.08
0.19 m/s 0.12 m/s (=0.62 ×
0.19)
4 7 28
3.4-14
3.4-10 3.4-11
1/3
19 27 5.89 m/s 21 33 5.85 m/s
0.58 0.41 0.02
0.20 m/s
0.08 m/s (=0.41 × 0.20)
4
5 8 4
3.4-15 1
3.4-12 3.4-13
1/3 1/2
6 8 23
3.4-16 1
3.4-14 3.4-15
0.1 0.4 m/s0.24
76
0.46 0.38
70cm 97cm 59cm
7 8 31
3.4-17 1
3.4-16 3.4-17
0.1 0.4m/s
0.20 0.40 0.42 6
70cm 92cm 74cm
8 9 6
3.4-18
3.4-18 3.4-19 6 7 0.1 0.4m/s
0.19 0.36 0.43
3.4.2.2. CO2 CO2 CO2
CO2 3.4-19 8 4 23
24 9 1 4
3.4-20 CO2
CO2
1.5 CO2
CO2
CO2
CO2 CO2
3.4.3.
77
3.4.3.1.
0.08 m/s 0.28 m/s
0.05 m/s 0.25 m/s
10 m 50 m
30 m 100 m 0.05 m/s 0.25 m/s
(10 m / 2) / 0.25 m/s 20 sec ( 2×10-4 day) (100 m / 2) / 0.05 m/s 1000 sec 0.28 hr ( 0.01 day)
0.01 day 1
day 0.1 day3 i) iii) 0.01 0.1 1 day
i)
ii)
iii)
3 i) 0.1 0.3 0.5 day ii) 0.5 2 4 dayiii) 4 20 40 day
78
3.4.3.2.
0.1 day 14C
3.4-21 271
14C 1 1
11
3.4-22 14C
14C 2 14C 114C
14C
14C
20 day 0.1day 1
3.4-23 0.01 day) 3.4-24 1 day)14C
3.4-25 14C
3.4-26 14C
14C 14C 14C
3.4-27 14C 3.4-2814C
2 2
- 14C
3.4.3.3.
79
3
50
0.01 4 day
0.5 2 day
1 1.9 24 day
3.4-29 3 50
3.4-30 3 14C
14C
3.4.1. 14C
3.4.1.3.4-31 2
3.4.3.4. 14C TF
TF
TF= 14C (Bq/g) 14C
(Bq/g) TF TF
1 14C 3.4-32 1 14C
14C 90 day 120 day14C 14C 14C
3.4-20
day 90 14C 4.63 × 10-5 Bq/g 5.35 × 10-5 Bq/g day 12014C 1.14 × 10-4 Bq/g 1.17 × 10-4 Bq/g day 150
14C 1.39 × 10-5 Bq/g 1.37 × 10-4 Bq/g
TF 0.12 2.56 14C
3.4-20 TF14C
14C -
TF - IAEA grain TF 0.1 IAEA, 2003 13C
80
TF 0.05 2.2 14C TF
, 2009 TF14C TF
3.4.4.
12
0.01 day 1 day
20 day
14C
3
TF0.05-2.2 , 2009
TF
Amano, H., Takahashi, T., Uchida, S., Matsuoka, S., Ikeda, H., Hayashi, H., Kurosawa, N., 2003. Development
of a code MOGRA for predicting the migration of ground additions and its application to various land
utilization areas. Journal of Nuclear Science and Technology 40, 975-979.
Homma, T., Saltelli, A., 1992. LISA package user guide, Part 1: PREP (Statistical PRE Processor) preparation of input sample for Monte Carlo simulations program description and user guide, 33 pp.
IAEA, 2003. Derivation of activity limits for the disposal of radioactive waste in near surface disposal facilities,
IAEA-TECDOC-1380, 145 pp.
Ishii, N., Ogiyama, S., Sakurai, S., Tagami, K., Uchida, S., 2015. Environmental transfer of carbon-14 in
Japanese paddy fields, in: Nakajima, K. (Ed.), Nuclear Back-end and transmutation technology for waste
disposal. Springer, Tokyo, pp. 303-309. Saltelli, A., Homma, T., 1992. LISA : Package user guide - Part III : SPOP (Statistical POst Processor) :
81
Uncertainty and sensitivity analysis for model output : Program description and user guide, 51 pp.
, , , 2009.
. Radioisotopes 58, 641-648.
82
14C14C 14C
14C14C
14C14C
14C 14C TRU
[1,2-14C] 0.5 g4.2 × 105 Bq 14C 14C
14C 4.2 × 103
Bq/mL 14C 14C14C
14C 25 3014C 14C
14C
77
14CO2
14C
4 3
14C
1
14C
14C
83
-
84
3.3-1
3.3-2
341F Bacteria 5′-CCTACGGGAGGCAGCAG Muyzer et al, 1993907R Bacteria 5′-CCGTCAATTCCTTT(A/G)AGTTT Muyzer et al, 2004PARCH340f Archae 5′-GCCTACGGGG(C/T)GCA(C/G)CAG Øvreås et al, 1997PARCH519r Archae 5′-TTACCGCGGC(T/G)GCTG Øvreås et al, 1997GC clamp 1 5′-CGCCCGCCGCGCCCCGCGCCCGTCCCGCCGCCCCCGCCCG Muyzer et al, 2004GC clamp 2 5′-CGCCCGCCGCGCGCGGCGGGCGGGGCGGGGGCACGGGGG Øvreås et al, 1997GC clamp 1 341F 5′GC clamp 2 PARCH340f 5′
Band ID Sequeice
CS07
CS08
CS09
CS10
CS11
85
3.4-1
3.4-2 14C
3.4-3
0-79day 0.3 0.1-0.5 day80-90day120-150day
2 0.5-4 day
91-119day 20 4-40 day2 0.5-2 day25 4-25 day
2.5 1.9-24 day
67 27-114 day
1 25 4-25 day6.1 1.9-24 day6.1 1.9-24 day
2 1.5 1.5-10 day2 0.5-2 day
10000 day1 10000 day
0.1 day730 730-2810 day73 73-168 day
PCC PRCC(R2) (R2)
( ) -0.06 10 0.04 11( ) -0.2 7 -0.02 12
) 0.87 1 0.92 10.02 12 -0.05 90.21 6 0.22 6-0.75 2 -0.75 2-0.12 8 -0.16 7
1 0.57 4 0.64 40.27 5 0.28 50.03 11 0.05 10
2 -0.62 3 -0.64 3-0.11 9 -0.08 8
PCCPRCC
cm)
1 2016.6.15 23 21 79 108 18 42 942 2016.7.12 67 21 50 108 18 42 943 2016.7.20 75 21 64 108 18 57 944 2016.7.28 83 21 64 108 18 73 945 2016.8.4 94 21 70 1086 2016.8.23 97 59 21 70 1087 2016.8.31 92 74 21 70 1088 2016.9.6 94 69 21 70 108
86
3.4-
4
3.4-
5
m/s
m/s
star
ten
d14
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15:2
90.
570.
960.
171.
372.
800.
871.
402.
290.
160.
570.
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171.
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1615
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060.
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340.
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603.
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080.
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661.
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390.
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260.
651.
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170.
290.
451.
620.
0122
:30
23:2
90.
210.
400.
010.
811.
240.
360.
521.
000.
030.
210.
400.
010.
811.
240.
360.
521.
000.
0323
:30
0:29
0.16
0.48
0.04
0.92
1.16
0.58
0.38
0.93
0.09
0.16
0.48
0.04
0.92
1.16
0.58
0.38
0.93
0.09
0:30
1:29
0.13
0.36
0.02
0.97
1.46
0.62
0.33
0.74
0.01
0.13
0.36
0.02
0.97
1.46
0.62
0.33
0.74
0.01
1:30
2:29
0.16
0.39
0.01
0.87
1.20
0.38
0.39
1.26
0.04
0.16
0.39
0.01
0.87
1.20
0.38
0.39
1.26
0.04
2:30
3:29
0.11
0.36
0.00
0.96
1.21
0.64
0.23
0.60
0.03
0.11
0.36
0.00
0.96
1.21
0.64
0.23
0.60
0.03
3:30
4:29
0.11
0.32
0.01
0.93
1.36
0.50
0.27
0.80
0.01
0.11
0.32
0.01
0.93
1.36
0.50
0.27
0.80
0.01
4:30
5:29
0.15
0.32
0.04
0.80
1.03
0.61
0.37
0.80
0.05
0.15
0.32
0.04
0.80
1.03
0.61
0.37
0.80
0.05
5:30
6:29
0.20
0.49
0.05
0.74
1.00
0.37
0.49
1.17
0.09
0.20
0.49
0.05
0.74
1.00
0.37
0.49
1.17
0.09
6:30
7:29
0.23
0.54
0.05
0.74
1.49
0.42
0.50
1.14
0.03
0.23
0.54
0.05
0.74
1.49
0.42
0.50
1.14
0.03
7:30
8:29
0.22
0.61
0.01
0.81
1.79
0.13
0.54
1.73
0.06
0.22
0.61
0.01
0.81
1.79
0.13
0.54
1.73
0.06
8:30
9:29
0.25
0.84
0.04
0.78
1.71
0.13
0.93
1.86
0.02
0.25
0.84
0.04
0.78
1.71
0.13
0.93
1.86
0.02
9:30
10:2
90.
200.
530.
010.
381.
090.
040.
381.
450.
030.
200.
530.
010.
381.
090.
040.
381.
450.
0310
:30
11:2
90.
240.
740.
040.
420.
960.
050.
771.
580.
010.
240.
740.
040.
420.
960.
050.
771.
580.
0111
:30
12:2
90.
230.
530.
020.
430.
890.
070.
561.
530.
030.
230.
530.
020.
430.
890.
070.
561.
530.
0312
:30
13:2
90.
200.
500.
030.
400.
940.
050.
551.
510.
020.
200.
500.
030.
400.
940.
050.
551.
510.
0213
:30
14:2
90.
401.
060.
070.
841.
740.
130.
861.
970.
010.
401.
060.
070.
841.
740.
130.
861.
970.
0114
:30
15:0
00.
370.
670.
070.
761.
270.
200.
821.
930.
160.
370.
670.
070.
761.
270.
200.
821.
930.
16
-6.
8.E-
042.
7.E-
032.
7.E-
025.
5.E-
029.
3.E-
023.
5.E-
02-
8.3.
E-02
1.5.
E-01
4.5.
E-01
2.9.
E-02
4.2.
E-02
4.3.
E-02
-7.
0.E-
016.
0.E-
014.
4.E-
019.
2.E-
018.
7.E-
019.
2.E-
01-
2.2.
E-01
2.2.
E-01
8.1.
E-02
-0.
0.E+
002.
1.E-
020.
0.E+
00-
0.0.
E+00
0.0.
E+00
0.0.
E+00
-0.
0.E+
000.
0.E+
000.
0.E+
00-
0.0.
E+00
0.0.
E+00
0.0.
E+00
87
3.4-
6
3.4-
7
m/s
m/s
star
ten
d14
:30
15:2
90.
180.
320.
020.
340.
740.
041.
462.
090.
670.
110.
230.
040.
110.
330.
010.
932.
030.
1415
:30
16:2
90.
170.
330.
040.
320.
690.
071.
462.
520.
700.
100.
180.
030.
100.
280.
020.
882.
060.
1816
:30
17:2
90.
160.
250.
060.
260.
610.
021.
172.
070.
530.
100.
200.
030.
090.
200.
010.
631.
580.
0917
:30
18:2
90.
160.
290.
070.
210.
450.
021.
041.
790.
440.
080.
170.
010.
070.
140.
010.
521.
070.
0718
:30
19:2
90.
150.
230.
080.
170.
560.
020.
731.
230.
200.
050.
110.
000.
060.
160.
010.
280.
720.
0319
:30
20:2
90.
280.
400.
100.
150.
310.
030.
461.
080.
080.
040.
100.
010.
070.
140.
010.
240.
750.
0320
:30
21:2
90.
280.
340.
240.
080.
290.
020.
190.
630.
010.
060.
090.
030.
080.
130.
050.
190.
360.
0421
:30
22:2
90.
240.
270.
180.
030.
100.
000.
290.
600.
020.
040.
090.
010.
090.
120.
060.
130.
450.
0222
:30
23:2
90.
220.
250.
160.
050.
130.
010.
200.
390.
010.
060.
090.
030.
090.
130.
050.
160.
340.
0323
:30
0:29
0.24
0.26
0.20
0.08
0.13
0.02
0.17
0.38
0.02
0.07
0.09
0.04
0.09
0.13
0.06
0.16
0.38
0.01
0:30
1:29
0.26
0.38
0.20
0.11
0.23
0.06
0.25
0.50
0.05
0.08
0.10
0.05
0.12
0.16
0.08
0.16
0.48
0.06
1:30
2:29
0.35
0.40
0.28
0.14
0.26
0.07
0.50
0.79
0.19
0.09
0.12
0.06
0.12
0.20
0.06
0.28
0.55
0.07
2:30
3:29
0.38
0.42
0.33
0.08
0.14
0.02
0.30
0.50
0.09
0.08
0.10
0.06
0.13
0.16
0.09
0.16
0.33
0.03
3:30
4:29
0.40
0.50
0.30
0.11
0.24
0.05
0.39
0.79
0.11
0.07
0.10
0.04
0.13
0.17
0.09
0.25
0.58
0.03
4:30
5:29
0.48
0.50
0.46
0.11
0.16
0.07
0.15
0.61
0.00
0.08
0.13
0.02
0.12
0.16
0.10
0.11
0.41
0.01
5:30
6:29
0.50
0.53
0.46
0.10
0.16
0.05
0.26
0.50
0.02
0.10
0.12
0.07
0.14
0.19
0.10
0.17
0.40
0.01
6:30
7:29
0.49
0.53
0.45
0.17
0.36
0.05
0.46
1.02
0.04
0.08
0.15
0.02
0.16
0.23
0.11
0.20
0.58
0.01
7:30
8:29
0.48
0.54
0.37
0.14
0.31
0.04
0.63
1.23
0.21
0.18
0.36
0.04
0.17
0.24
0.10
0.34
0.84
0.08
8:30
9:29
0.18
0.40
0.11
0.10
0.27
0.02
0.54
1.14
0.07
0.26
0.35
0.12
0.10
0.22
0.02
0.27
0.78
0.01
9:30
10:2
90.
140.
190.
080.
080.
220.
010.
420.
770.
100.
340.
410.
290.
050.
160.
010.
290.
840.
0610
:30
11:2
90.
150.
210.
090.
060.
180.
010.
471.
210.
120.
370.
400.
340.
050.
090.
010.
250.
760.
0311
:30
12:2
90.
140.
200.
070.
060.
170.
000.
400.
770.
150.
350.
390.
280.
040.
100.
010.
220.
580.
0312
:30
13:2
90.
160.
230.
120.
080.
240.
020.
390.
810.
040.
280.
340.
240.
040.
090.
000.
170.
460.
0113
:30
14:2
90.
140.
200.
050.
080.
280.
010.
631.
370.
230.
280.
330.
230.
050.
130.
010.
411.
190.
0214
:30
15:0
00.
140.
210.
060.
080.
290.
010.
521.
150.
180.
300.
360.
260.
040.
100.
000.
261.
010.
02
-1.
0.E-
012.
9.E-
021.
7.E-
026.
4.E-
012.
0.E-
021.
1.E-
01-
2.1.
E-01
1.5.
E-01
1.4.
E-01
7.1.
E-04
2.9.
E-01
3.4.
E-02
-3.
7.E-
012.
5.E-
013.
9.E-
013.
6.E-
016.
9.E-
018.
6.E-
01-
3.1.
E-01
2.5.
E-01
3.2.
E-01
-5.
4.E-
031.
7.E-
018.
2.E-
02-
0.0.
E+00
7.4.
E-02
2.5.
E-02
-6.
8.E-
044.
6.E-
021.
2.E-
02-
0.0.
E+00
2.6.
E-02
3.4.
E-03
88
3.4-
8
3.4-
9
m/s
m/s
star
ten
d14
:40
15:3
90.
190.
380.
080.
480.
910.
181.
201.
860.
520.
090.
190.
030.
200.
450.
020.
661.
650.
0715
:40
16:3
90.
180.
310.
050.
470.
830.
111.
152.
240.
530.
090.
210.
000.
180.
410.
060.
601.
430.
1116
:40
17:3
90.
170.
260.
090.
390.
910.
090.
991.
580.
460.
080.
160.
040.
150.
360.
040.
531.
610.
0717
:40
18:3
90.
140.
340.
040.
350.
860.
071.
011.
940.
350.
080.
170.
030.
160.
550.
040.
782.
040.
2118
:40
19:3
90.
140.
320.
010.
370.
980.
060.
941.
560.
390.
060.
160.
000.
150.
320.
040.
751.
500.
2119
:40
20:3
90.
210.
360.
070.
350.
940.
010.
931.
690.
230.
050.
150.
000.
150.
330.
050.
842.
030.
1020
:40
21:3
90.
280.
380.
150.
210.
600.
010.
671.
280.
230.
030.
090.
000.
100.
260.
010.
501.
670.
0321
:40
22:3
90.
290.
400.
160.
260.
710.
020.
871.
610.
280.
040.
100.
000.
130.
340.
030.
671.
330.
0222
:40
23:3
90.
290.
430.
160.
260.
560.
080.
981.
780.
410.
040.
100.
000.
140.
380.
040.
711.
480.
0723
:40
0:39
0.27
0.47
0.15
0.27
1.00
0.06
0.96
1.69
0.38
0.05
0.15
0.00
0.14
0.33
0.03
0.69
1.63
0.11
0:40
1:39
0.27
0.43
0.15
0.31
0.67
0.04
1.15
2.30
0.42
0.05
0.17
0.00
0.16
0.40
0.05
0.83
1.53
0.23
1:40
2:39
0.25
0.39
0.09
0.34
0.77
0.07
1.16
2.14
0.46
0.06
0.27
0.01
0.17
0.36
0.04
0.86
1.57
0.14
2:40
3:39
0.22
0.34
0.13
0.29
0.66
0.08
1.11
1.96
0.41
0.06
0.13
0.01
0.16
0.39
0.05
0.76
1.88
0.17
3:40
4:39
0.18
0.28
0.09
0.27
0.69
0.02
0.91
1.58
0.43
0.04
0.13
0.00
0.13
0.30
0.03
0.52
1.00
0.08
4:40
5:39
0.11
0.19
0.03
0.18
0.45
0.01
0.66
1.37
0.13
0.06
0.13
0.00
0.11
0.23
0.05
0.32
0.98
0.00
5:40
6:39
0.13
0.21
0.07
0.22
0.54
0.01
0.58
1.08
0.04
0.08
0.14
0.05
0.42
2.51
0.09
0.23
1.09
0.06
6:40
7:39
0.13
0.24
0.06
0.21
0.46
0.01
0.62
1.19
0.21
0.06
0.13
0.01
5.74
7.82
2.53
1.80
2.49
0.34
7:40
8:39
0.14
0.28
0.03
0.24
0.54
0.02
0.77
1.52
0.20
0.05
0.11
0.01
7.38
7.86
6.01
2.12
2.43
1.42
8:40
9:39
0.16
0.28
0.07
0.23
0.69
0.02
0.83
1.39
0.30
0.04
0.11
0.00
2.86
3.14
2.07
9:40
10:3
90.
190.
300.
080.
270.
650.
040.
991.
830.
450.
040.
120.
002.
833.
292.
5710
:40
11:3
90.
220.
330.
080.
230.
910.
020.
911.
650.
330.
040.
110.
012.
443.
311.
1211
:40
12:3
90.
160.
320.
050.
280.
670.
060.
921.
930.
250.
070.
150.
014.
406.
712.
8412
:40
13:3
90.
140.
270.
060.
190.
500.
010.
741.
460.
210.
110.
210.
058.
439.
556.
6113
:40
14:3
90.
130.
230.
040.
220.
520.
090.
791.
240.
450.
120.
220.
0410
.15
11.8
67.
7614
:40
14:4
90.
140.
220.
090.
200.
460.
020.
771.
370.
29
-2.
8.E-
032.
5.E-
011.
6.E-
012.
9.E-
012.
9.E-
023.
3.E-
01-
7.4.
E-02
2.7.
E-01
5.2.
E-01
8.4.
E-02
2.3.
E-01
3.0.
E-02
-5.
9.E-
012.
7.E-
012.
4.E-
016.
2.E-
017.
4.E-
016.
4.E-
01-
3.1.
E-01
1.3.
E-01
7.1.
E-02
-1.
9.E-
026.
2.E-
036.
9.E-
04-
0.0.
E+00
4.1.
E-03
0.0.
E+00
-7.
0.E-
046.
9.E-
030.
0.E+
00-
0.0.
E+00
6.6.
E-02
4.8.
E-03
89
3.4-
10
3.4-
11
m/s
m/s
star
ten
d14
:30
15:2
90.
150.
260.
060.
100.
260.
010.
551.
320.
030.
050.
160.
010.
210.
510.
050.
471.
340.
0215
:30
16:2
90.
150.
300.
060.
140.
440.
010.
841.
470.
470.
070.
170.
010.
360.
720.
140.
671.
570.
2416
:30
17:2
90.
140.
220.
070.
110.
310.
010.
591.
230.
110.
050.
120.
010.
230.
610.
060.
361.
200.
0417
:30
18:2
90.
180.
340.
110.
080.
220.
020.
381.
050.
030.
030.
100.
000.
090.
230.
010.
160.
630.
0218
:30
19:2
90.
280.
370.
190.
120.
320.
010.
290.
660.
030.
050.
120.
000.
885.
890.
040.
160.
420.
0219
:30
20:2
90.
220.
270.
170.
060.
140.
010.
280.
510.
010.
040.
110.
000.
193.
830.
010.
120.
290.
0420
:30
21:2
90.
140.
220.
100.
050.
130.
010.
220.
560.
020.
040.
060.
020.
090.
180.
010.
130.
370.
0321
:30
22:2
90.
130.
160.
110.
030.
060.
010.
140.
330.
040.
030.
060.
010.
435.
850.
060.
140.
360.
0622
:30
23:2
90.
120.
150.
110.
030.
070.
000.
100.
220.
030.
050.
090.
010.
130.
160.
080.
120.
170.
0723
:30
0:29
0.15
0.18
0.13
0.08
0.13
0.05
0.16
0.35
0.01
0.08
0.10
0.03
0.16
0.30
0.09
0.15
0.27
0.08
0:30
1:29
0.15
0.17
0.11
0.06
0.12
0.01
0.23
0.47
0.05
0.09
0.11
0.07
0.19
0.27
0.13
0.21
0.40
0.11
1:30
2:29
0.15
0.18
0.11
0.07
0.11
0.04
0.14
0.37
0.01
0.09
0.11
0.05
0.17
0.25
0.12
0.19
0.28
0.12
2:30
3:29
0.15
0.18
0.12
0.07
0.11
0.04
0.12
0.35
0.02
0.08
0.09
0.06
0.16
0.21
0.14
0.15
0.24
0.10
3:30
4:29
0.16
0.18
0.12
0.07
0.11
0.02
0.19
0.51
0.05
0.07
0.10
0.05
0.18
0.36
0.13
0.21
0.53
0.10
4:30
5:29
0.18
0.32
0.14
0.08
0.15
0.02
0.21
0.44
0.02
0.09
0.11
0.07
0.22
0.41
0.16
0.20
0.38
0.08
5:30
6:29
0.36
0.45
0.28
0.12
0.25
0.03
0.40
0.77
0.19
0.08
0.11
0.04
0.24
0.44
0.13
0.32
0.59
0.09
6:30
7:29
0.44
0.53
0.36
0.13
0.43
0.02
0.48
0.92
0.19
0.10
0.16
0.06
0.18
0.42
0.00
0.25
0.71
0.04
7:30
8:29
0.39
0.50
0.31
0.13
0.29
0.02
0.45
0.90
0.04
0.10
0.16
0.04
0.17
0.44
0.03
0.25
0.70
0.01
8:30
9:29
0.25
0.48
0.06
0.14
0.38
0.01
0.38
0.86
0.11
0.05
0.12
0.00
0.15
0.44
0.01
0.35
0.85
0.05
9:30
10:2
90.
160.
260.
090.
120.
200.
040.
360.
800.
020.
040.
100.
010.
130.
310.
030.
340.
990.
0710
:30
11:2
90.
190.
310.
120.
130.
380.
030.
480.
900.
050.
070.
130.
020.
140.
290.
020.
280.
760.
0411
:30
12:2
90.
180.
320.
050.
180.
390.
030.
771.
500.
270.
080.
160.
030.
200.
700.
030.
290.
720.
0512
:30
13:2
90.
180.
320.
080.
250.
600.
041.
111.
660.
500.
110.
200.
050.
310.
680.
050.
602.
230.
1113
:30
14:2
90.
180.
340.
050.
260.
630.
051.
101.
720.
350.
100.
190.
020.
421.
240.
130.
641.
390.
0914
:30
15:0
00.
150.
300.
040.
130.
340.
000.
831.
450.
400.
090.
140.
050.
330.
770.
110.
531.
030.
05
-6.
2.E-
037.
0.E-
024.
3.E-
025.
8.E-
013.
8.E-
013.
8.E-
01-
1.4.
E-01
1.7.
E-01
9.5.
E-02
1.6.
E-02
1.6.
E-01
1.7.
E-02
-4.
9.E-
011.
8.E-
012.
7.E-
014.
1.E-
014.
5.E-
016.
0.E-
01-
3.5.
E-01
1.7.
E-01
3.4.
E-01
-6.
2.E-
031.
6.E-
011.
2.E-
01-
0.0.
E+00
1.1.
E-01
4.0.
E-02
-0.
0.E+
009.
9.E-
025.
1.E-
02-
0.0.
E+00
3.3.
E-02
4.4.
E-02
90
3.4-12
3.4-13
m/s
start end14:30 15:29 0.22 0.33 0.16 0.07 0.21 0.01 0.25 0.65 0.0415:30 16:29 0.19 0.28 0.13 0.12 0.34 0.01 0.56 1.08 0.2116:30 17:29 0.22 0.34 0.09 0.13 0.31 0.02 0.77 1.41 0.3317:30 18:29 0.24 0.33 0.16 0.10 0.27 0.00 0.53 0.95 0.1518:30 19:29 0.27 0.31 0.24 0.09 0.20 0.01 0.33 0.59 0.0519:30 20:29 0.25 0.29 0.21 0.09 0.21 0.01 0.33 0.69 0.1320:30 21:29 0.24 0.29 0.21 0.09 0.19 0.04 0.31 0.49 0.1721:30 22:29 0.22 0.25 0.19 0.11 0.21 0.04 0.32 0.66 0.0322:30 23:29 0.23 0.26 0.19 0.10 0.17 0.07 0.23 0.47 0.0623:30 0:29 0.21 0.26 0.17 0.10 0.18 0.05 0.21 0.58 0.050:30 1:29 0.22 0.25 0.17 0.11 0.16 0.09 0.19 0.42 0.051:30 2:29 0.18 0.21 0.15 0.10 0.13 0.07 0.11 0.21 0.022:30 3:29 0.17 0.19 0.14 0.11 0.16 0.08 0.15 0.34 0.013:30 4:29 0.15 0.18 0.11 0.12 0.22 0.09 0.25 0.46 0.064:30 5:29 0.15 0.18 0.13 0.09 0.14 0.05 0.16 0.39 0.035:30 6:29 0.22 0.29 0.17 0.09 0.16 0.04 0.17 0.67 0.026:30 7:29 0.28 0.35 0.22 0.09 0.24 0.01 0.56 1.06 0.227:30 8:29 0.27 0.39 0.17 0.12 0.25 0.03 0.60 1.22 0.188:30 9:29 0.14 0.26 0.06 0.11 0.33 0.01 0.46 0.95 0.169:30 10:29 0.16 0.29 0.09 0.10 0.27 0.03 0.33 0.66 0.0610:30 11:29 0.23 0.35 0.15 0.10 0.25 0.01 0.41 0.96 0.1511:30 12:29 0.26 0.39 0.18 0.10 0.26 0.01 0.47 1.07 0.0612:30 13:29 0.20 0.31 0.09 0.10 0.27 0.00 0.55 1.09 0.1413:30 14:29 0.16 0.27 0.07 0.08 0.26 0.01 0.53 1.08 0.1314:30 15:00 0.14 0.26 0.05 0.08 0.20 0.01 0.49 0.96 0.20
- 6 48 46- 174 442 58
- 1141 209 220- 131 254 525
- 0 176 331- 0 150 144
- 0 139 94- 0 31 35
91
3.4-14
3.4-15
m/s
start end14:49 15:48 0.27 0.43 0.16 0.72 1.24 0.27 0.98 1.57 0.4315:49 16:48 0.29 0.41 0.17 0.60 1.22 0.23 0.90 1.77 0.3116:49 17:48 0.41 0.55 0.28 0.53 1.29 0.19 0.83 1.59 0.3817:49 18:48 0.34 0.44 0.29 0.21 0.64 0.02 0.34 0.96 0.0518:49 19:48 0.35 0.45 0.31 0.20 0.48 0.03 0.38 1.16 0.0519:49 20:48 0.35 0.44 0.30 0.25 0.56 0.03 0.55 0.90 0.1320:49 21:48 0.32 0.38 0.25 0.27 0.50 0.05 0.65 1.11 0.2321:49 22:48 0.31 0.49 0.11 0.51 0.96 0.01 1.21 2.16 0.4822:49 23:48 0.19 0.31 0.11 0.27 0.69 0.04 0.75 1.40 0.2423:49 0:48 0.17 0.26 0.13 0.15 0.35 0.03 0.38 0.96 0.070:49 1:48 0.17 0.21 0.12 0.14 0.58 0.01 0.31 1.23 0.031:49 2:48 0.20 0.35 0.15 0.20 0.58 0.03 0.47 1.19 0.112:49 3:48 0.18 0.26 0.10 0.24 0.48 0.08 0.62 1.31 0.213:49 4:48 0.25 0.39 0.08 0.45 1.02 0.09 0.69 1.47 0.224:49 5:48 0.23 0.34 0.17 0.35 0.68 0.05 0.47 1.21 0.025:49 6:48 0.21 0.29 0.16 0.23 0.58 0.01 0.37 0.74 0.056:49 7:48 0.29 0.46 0.17 0.32 0.80 0.06 0.71 1.53 0.067:49 8:48 0.23 0.36 0.12 0.25 0.53 0.04 0.51 0.94 0.068:49 9:48 0.30 0.48 0.19 0.48 0.94 0.10 0.84 1.61 0.359:49 10:48 0.31 0.45 0.19 0.65 1.04 0.32 1.21 1.82 0.7410:49 11:48 0.31 0.51 0.16 0.50 1.10 0.11 0.92 1.75 0.2411:49 12:48 0.31 0.59 0.05 0.44 1.55 0.05 0.74 2.24 0.2212:49 13:48 0.35 0.47 0.2813:49 14:52 0.37 0.53 0.25
- 0 166 223- 135 176 273
- 1178 231 223- 127 236 249
- 0 210 178- 0 90 60
- 0 54 20- 0 100 36
92
3.4-16 7
3.4-17
m/s
start end14:23 15:22 0.28 0.56 0.06 1.23 2.81 0.50 1.93 3.50 0.8915:23 16:22 0.32 0.66 0.11 1.45 2.47 0.73 2.10 3.54 1.0216:23 17:22 0.37 0.62 0.14 1.02 2.12 0.46 1.48 3.08 0.5417:23 18:22 0.32 0.62 0.09 1.11 1.79 0.26 1.54 2.34 0.7418:23 19:22 0.19 0.33 0.09 0.98 1.49 0.55 1.15 1.91 0.5719:23 20:22 0.17 0.26 0.09 0.62 1.55 0.20 1.00 1.85 0.6220:23 21:22 0.18 0.22 0.14 0.41 0.70 0.18 0.95 1.47 0.6021:23 22:22 0.21 0.27 0.16 0.50 0.84 0.29 1.07 1.51 0.7222:23 23:22 0.22 0.28 0.16 0.45 0.83 0.24 1.03 1.62 0.7523:23 0:22 0.23 0.30 0.14 0.66 1.39 0.26 1.19 1.72 0.720:23 1:22 0.25 0.40 0.10 0.62 1.22 0.24 0.95 1.69 0.491:23 2:22 0.23 0.33 0.15 0.54 0.96 0.22 0.89 1.37 0.432:23 3:22 0.22 0.33 0.17 0.57 0.93 0.23 0.88 1.46 0.483:23 4:22 0.22 0.27 0.17 0.42 0.82 0.15 0.66 1.29 0.094:23 5:22 0.22 0.29 0.15 0.51 0.83 0.20 0.77 1.42 0.205:23 6:22 0.20 0.24 0.15 0.33 0.46 0.19 0.34 0.88 0.036:23 7:22 0.24 0.37 0.17 0.55 0.85 0.28 0.58 1.11 0.097:23 8:22 0.28 0.43 0.18 0.60 1.01 0.26 0.80 1.82 0.348:23 9:22 0.35 0.48 0.19 0.67 1.30 0.38 0.85 1.82 0.319:23 10:22 0.26 0.42 0.15 0.71 1.55 0.37 0.80 1.50 0.2710:23 11:22 0.28 0.50 0.11 0.65 1.21 0.25 0.87 2.19 0.3911:23 12:22 0.25 0.41 0.15 0.62 1.07 0.36 0.83 2.00 0.3912:23 13:22 0.23 0.36 0.12 0.55 1.00 0.23 0.70 1.35 0.0513:23 14:22 0.22 0.32 0.15 0.45 0.76 0.20 0.49 1.27 0.0314:23 14:56 0.25 0.37 0.17 0.55 0.96 0.25 0.58 1.22 0.21
- 1 0 10- 6 0 4
- 1269 0 3- 190 20 183
- 3 780 708- 0 397 262
- 0 237 163- 0 29 109
93
3.5-18
3.4-19
m/s
start end14:04 15:03 0.27 0.42 0.16 1.16 2.17 0.72 1.30 2.48 0.6415:04 16:03 0.26 0.42 0.04 1.54 2.42 0.55 2.02 3.34 0.7816:04 17:03 0.27 0.47 0.06 1.19 1.89 0.70 1.49 2.57 0.5117:04 18:03 0.28 0.50 0.12 1.01 1.67 0.48 1.19 3.09 0.4718:04 19:03 0.43 0.65 0.31 1.02 1.74 0.48 1.28 2.41 0.2619:04 20:03 0.40 0.52 0.21 0.84 1.45 0.49 0.89 1.69 0.4120:04 21:03 0.33 0.48 0.21 0.86 1.25 0.44 1.02 1.78 0.3621:04 22:03 0.31 0.44 0.18 0.89 1.49 0.41 1.28 2.09 0.3222:04 23:03 0.17 0.21 0.14 0.34 0.51 0.10 0.28 0.61 0.0123:04 0:03 0.21 0.26 0.16 0.55 0.97 0.26 0.54 1.14 0.090:04 1:03 0.24 0.28 0.22 0.45 0.89 0.15 0.51 1.01 0.131:04 2:03 0.24 0.29 0.18 0.40 0.79 0.11 0.44 0.91 0.092:04 3:03 0.24 0.31 0.21 0.50 1.15 0.32 0.47 1.04 0.093:04 4:03 0.26 0.33 0.20 0.63 1.71 0.14 0.75 1.85 0.054:04 5:03 0.28 0.34 0.20 0.85 1.67 0.52 1.10 1.89 0.565:04 6:03 0.28 0.32 0.24 0.78 1.38 0.31 0.74 1.24 0.446:04 7:03 0.27 0.31 0.22 0.59 0.99 0.29 0.58 1.15 0.247:04 8:03 0.24 0.33 0.19 0.40 0.78 0.07 0.61 1.38 0.068:04 9:03 0.23 0.34 0.18 0.55 1.34 0.06 0.83 1.78 0.139:04 10:03 0.25 0.43 0.15 1.00 1.70 0.47 1.44 2.13 0.8610:04 11:03 0.29 0.45 0.20 1.07 1.69 0.47 1.55 2.11 1.0711:04 12:03 0.28 0.46 0.13 1.10 1.67 0.63 1.40 2.31 0.5412:04 13:03 0.30 0.47 0.17 0.86 1.47 0.51 1.10 2.40 0.5113:04 13:28 0.28 0.38 0.22 0.89 1.09 0.60 1.17 1.55 0.84
- 1 0 5- 2 1 12
- 1255 5 36- 146 158 376
- 0 745 655- 0 420 239
- 0 58 71- 0 0 2
94
3.4-20
day
14C 90 4.42 4.48 5.1
Bq) 1Bq 120 10.84 10.87 11.14
150 6.97E-04 1.26E-03 6.85E-03
14C 90 4.63E-05 4.70E-05 5.35E-05
Bq/g 120 1.14E-04 1.14E-04 1.17E-04
150 1.39E-05 2.51E-05 1.37E-04
TF 90 0.30 0.53 2.56
120 0.12 0.22 1.17
95
96
3.2-1 14C 14C
3.2-2 14CO2
3.2-3 14CO2
97
3.2-4 14CO2
3.2-5 14CO2
98
3.3-1 P2 15˚C
3.3-2 P11
99
3.3-3 14C DGGE
3.3-4 DGGE DNA
100
3.4-
1
101
3.4-
2
0.0
0.2
0.4
0.6
0.8
020
4060
8010
0
day)
()
0.0
1.0
2.0
3.0
4.0
5.0
6.0
020
4060
8010
0
day)
()
0 10
20
30
40
50
60
020
4060
8010
0
day)
)
0.0
0.5
1.0
1.5
2.0
2.5
3.0
020
4060
8010
0
day)
→
0 10
20
30
40
020
4060
8010
0
day)
→
0 10
20
30
40
020
4060
8010
0
day)
→
0 50
100
150
020
4060
8010
0
day)
→
0 10
20
30
40
020
4060
8010
0
day)
→1
0 10
20
30
40
020
4060
8010
0
day)
→
0 10
20
30
40
020
4060
8010
0
day)
→
0 2 4 6 8 10
12
14
020
4060
8010
0
day)
2→
0 1 2 3
020
4060
8010
0
day)
→
102
3.4-
314
C3.
4-4
14C
103
3.4-5 14C 80-90 day 120 day
104
3.4-
6->
14C
3.4-
7->
14C
80
-90
day
120
day
80-9
0 da
y12
0 da
y
105
3.4-8 -> 14C 80-90 day 120 day
106
3.4-9 4 14C
y = 0.0167e0.0365x
R² = 0.5652
1.E-03
1.E-02
1.E-01
1.E+00
0 10 20 30 40
14C
-1B
qB
q)
(day
)
y = 0.0547e-0.03x
R² = 0.1424
1.E-03
1.E-02
1.E-01
1.E+00
0 10 20 30
14C
-1B
qB
q)
1→ (day
→
y = 0.0512e-0.056x
R² = 0.0732
1.E-03
1.E-02
1.E-01
1.E+00
0 5 10 15
14C
-1B
qB
q)
2→ 1 (day
2→
y = 0.0266e0.0232x
R² = 0.0779
1.E-03
1.E-02
1.E-01
1.E+00
0 10 20 30
14C
-1B
qB
q)
→ 1 (day
→ 1
107
3.4-10
3.4-11 1
108
3.4-12
3.4-13
3.4-14
109
3.4-15
3.4-16
3.4-17
110
3.4-18
3.4-19
111
3.4-
20C
O2
(0.4
)
(0.3
)
(0.2
)
(0.1
)
0.0
0.1
0.2
0.3
0.4
0.5
0.6
0
1000
2000
3000
4000
5000
6000
0
1200
2400
3600
(m/s)
CO2 (ppm)
sec
84
Dry
ice
CO
2C
O2
(0.4
)
(0.3
)
(0.2
)
(0.1
)
0.0
0.1
0.2
0.3
0.4
0.5
0.6
0
500
1000
1500
2000
2500
500
1100
1700
2300
(m/s)
CO2 (ppm)
sec
823
Dry
iceC
O2
CO
2
(0.4
)
(0.3
)
(0.2
)
(0.1
)
0.0
0.1
0.2
0.3
0.4
0.5
0.6
0
1000
2000
3000
4000
5000
6000
7000
0
600
1200
1800
(m/s)
CO2 (ppm)
sec
824
Dry
ice
CO
2C
O2
(0.4
)
(0.3
)
(0.2
)
(0.1
)
0.0
0.1
0.2
0.3
0.4
0.5
0.6
0
500
1000
1500
2000
2500
0
600
1200
1800
(m/s)
CO2 (ppm)se
c
91
Dry
ice
CO
2
CO
2
112
3.4-21 14C
113
3.4-22 14C
114
3.4-23
14C
3.4-24
14C
115
3.4-25
14C
3.4-26
14C
116
3.4-27 14C
3.4-28 -
0
0.002
0.004
0.006
0.008
0.01
0.012
0
0.1
0.2
0.3
0.4
0.5
0.6
0 50 100 150 200
14C
1Bq
Bq)
14C
(1B
qB
q)
(day)
117
3.4-29
0
1
2
3
4
5
0 10 20 30 40 50
day)
0.0
0.5
1.0
1.5
2.0
2.5
3.0
0 10 20 30 40 50
day)
→
0
10
20
30
40
0 10 20 30 40 50
day)
→
118
3.4-30 14C
y = 0.0023e0.601x
R² = 0.8311
1.E-04
1.E-03
1.E-02
1.E-01
1.E+00
0.0 1.0 2.0 3.0 4.0 5.0
14C
1Bq
)
(day
y = 0.0073e0.026x
R² = 0.0002
1.E-04
1.E-03
1.E-02
1.E-01
1.E+00
0.0 0.5 1.0 1.5 2.0 2.5
14C
1Bq
)
→ (day
→
y = 0.0089e-0.013x
R² = 0.0113
1.E-04
1.E-03
1.E-02
1.E-01
1.E+00
0 5 10 15 20 25
14C
1Bq
)
1→ (day
1→ )
119
3.4-31 14C
3.4-32 14C
y = 0.0055x0.6577
R² = 0.9193
1.E-04
1.E-03
1.E-02
1.E-01
1.E+00
0 5 10 15 20 25 30 35 40 45
14C
1Bq
)
(day
0.1 4day
4 40day
0
0.002
0.004
0.006
0.008
0.01
0.012
0
5
10
15
20
25
30
0 50 100 150 200
14C
1Bq
Bq)
114
C(1
Bq
Bq)
(day)1
1 1 1
120
4 Pu, Am, Th Cl
14 18
− TF - Kd
Pu, Am, Th Cl
Pu, Am, ThTF
Am Am
Am
Am
-
− ICP-MSTh Th Pu
25 Pu
Pu - Pu
Pu −
Pu, Am, Th TF 2015 -2016
27Am
121
Am
4.2.1. Am 241Am 241Am
241Am
Bennett, 1978 241Pu241Pu 241Am 241Am Zheng et al. (2012)
FDNPP 241Am
Am
Am241Pu 241Am Zheng et al., 2013a
241Am Amoli and
Barker, 2012; Maxwell and Faison, 2008; Zheng and Yamada, 2008241Am 0.1 1 Bq/kg
Xiao et al., 2014241Am Zheng et al.,
2013b Varga 2007
3-10238Pu, 210Po, 228Th 232U
10 Vajda and
Kim, 2010 ICP-MSAMS 241Am Kazi et al., 2015; Li et al., 2010
ICP-MS 241Am Hang et al., 2004; Truscott et al.,
2001 ICP-MS 241Am
Varga, 2007; Zheng and Yamada, 2008
ICP-MS AMS241Am
241Am
2
122
(Prohaska et al., 2014) 241Am
27 4.2-1
, 2016 ICP-MS
ICP-MS
(m/ m=300) Pu Bi, Pb, Tl, Hg, Ir m/z = 241
241Am Yamamoto et al. 1983 0.032-0.263 mBq/g 241Am
DGA-N
Am
Am CaC2O4 DGA-N Am
Am
Am Am
SF-ICP-MS AmTEVA
Am
Am 6
4.2.1.1. 4.2-1 Aridus
Aspire PFA PFA
Aspire PFA
Aridus II 110 oC
PFAPTFE
PTFE
SF-ICP-MS Aridus II
PFA 50, 100 200 µL min-1
50 µL min-1 ICP-AES Activa-M
Na Mg K Fe Ca Al
Bi Pb Tl Hg Pt Hf REEs SF-ICP-MS Element
XR Thermo Scientific Bremen Germany Scott
4.2.1.2. Aridus-SF-ICP-MS Element XR
123
H27 Aridus
H27 4.2-6
Am H27 4.2.2.
4.2.1.3. IAEA-soil-6 and IAEA-375 NIST-4357, IAEA-385 and
IAEA-384 (NIST-4354) 241Am
JSAC-0471241Am
4.2.1.4. HCl, HNO3, HF, HCOOH, H2C2O4, NH4OH, NaNO2, Ca(NO3)2, , NH4SCN
HCl HNO3
Bi, Tl, Hg, Pb, U, Hf, Pt, In, Rh REEs Merck Millipore
Eichrom (DGA-N, UTEVA and TEVA,
50-100µm 2 mL ) 243Am Amersham International, UK
Milli-Q-Plus>18 MΩ cm-1
4.2.1.5.
(1) DGA-N
DGA-N HCl HNO3
Am U, Bi, Tl, Hg, Pb, Hf, Pt Dy 2 ng mL-1 HNO3 HCl 5mL DGA-N
REE Am Dy
Am DGA-N
HCl HNO3 5mL
HCl HNO3 5mL
U, Bi, Tl, Hg, Pb, Hf, Pt Dy SF-ICP-MSHNO3 0.01 8 M 0.01M 0.05M 0.1M 0.5M 1M 3M 5M 8M
HCl 0.01 M 9.5 M 0.01M 0.1M 0.25M 0.5M 1M 4M 9M 9.5 M
4.2-2 Am Dy
4.2-2 a b HNO3 c d HCl
yHNO3 HCl DGA-N
1
0 Tl HNO3
HCl DGA-N Hg HNO3
HCl DGA-N 8M HNO3 Bi
Horwitz 2005 0.01~4M HCl 0.01~8M HNO3 DGA-N Pb DGA-N 0.5 3M HNO3
124
Horwitz 2005 0.5-1M HNO3
0.25M HCl Pt DGA-N
Kd Pourmand and Dauphas, 2010 Hf HNO3 HCl
4M Hf DGA-N
HNO3<0.1M HCl<1.0M DGA-N :
Pu U UTEVA DGA-N
HNO 3 15mL 8M HNO 3 Pb Hg Pt ; 15mL 0.5M HNO3
Tl ; 15mL 0.1M HNO3 U Pt Hf
(3 HCl 10mL HCl Bi Tl Pb UTEVA DGA-N Am
(2)
Am
Qiao et al., 2009; Xu et al., 2014 Am Fe(OH)3 CaF2
CaC2O 4 3
JSAC-0471 5g
4.2-3 Mg Al Fe(OH)3 Mg
Al CaF2 Al Fe
30 CaC2O4
Na 10 Am
CaC2O4
(3) Am
UTEVA + DGA-N Am CaC2O4
SF-ICP-MS
JSAC-0471 5g
Na K Mg Ca Fe Al REEs
4.2-1 0.1 7.6 g mL-1
REEs 6 66 gmL-1 Am Am REEsREEs 90 CaC2O4
Dy DGA-N
REEs SF-ICP-MS
SF-ICP-MS REEs SF-ICP-MS
Maxwell (2010) DGA-N REEs 0.05M HNO3
4.2-4a REEs Am
125
DGA-N 0.05M HNO3 0.05M HNO3 La Ce
65 La 25 Ce 10mL 0.05M HNO3
REEs
TEVA 241Am
Thakur et al., 2011; Luisier et al., 2009REEs
4.2-4b Pr Nd Sm Eu 10
TEVA La Ce Pr Nd Sm Eu
DGA-N 0.05M HNO3 10mL TEVA
REEs 4.2-4b Am 95
Am REEs
4.2.1.6
(1)
Am 4.2-5
105ºC 24 802-20g 0.5 pg 243Am
450ºC 5
Am 120 mL
Savillex Corporation, Minnesota, USA 20-40 mL
160 C 4 Advantec filter100 mL 40mL 1M HNO3
Ca 100mg 2.5g
NH4OH pH 2.0 2.5 30
3000 rpm 20 1 5mL
15mL HNO3 8M
HNO3 20mL 0.2 g NaNO2 8M HNO3 UTEVAPu Pu IV
UTEVA + DGA-N Am 5mL 8M HNO3
UTEVA + DGA-N UTEVA
Am DGA-N DGA-N
(1)15mL 8M HNO 3 Pb Hg Pt
; (2)15mL 0.5M HNO3 Tl ; (3)15mL 0.1M HNO3 U Pt Hf(4)10 mL 0.05 M HNO3 La, Ce ; (5)10mL HCl Bi Tl
Pb
UTEVA + DGA-N Am DGA-N
Am 10mL 0.5M HCl 10mL 2M
NH4SCN-0.1M HCOOH TEVA Am REEs
5mL 2M NH4SCN-0.1M HCOOH TEVA Am10mL 2M NH4SCN-0.1M HCOOH 10mL 1M NH4SCN-0.1M
126
HCOOH TEVA REEs Am 10mL 4M HCl DGA-N
TEVA 4.2-6 Am TEVA
NH4SCN 8mL
SF-ICP-MS 1mL 4 HNO3
(2) Am Am
IAEA-soil-6 DF DF
Bi Tl Hg Pb U, Pu DF 3.5 10 4 2.4
10 4 1.5 10 4 1.2 105 3.6 106, 7 105
Am
IAEA-384 78 3 IAEA-385 77 1 IAEA-375 82 1 IAEA- -6 765 NIST- 4354 79 6 NIST-4357 79 7 80 3
LOD 3
1g 0.097 fg g-1 0.012 mBq g-1 LOD Pimpl and Higgy (2001)
0.03 mBq g-1 Jia (1997) 0.034 mBq g-1
LOD DF241Am
(3)
Am SF-ICP-MS
IAEA-soil-6 and IAEA-375 NIST-4357, IAEA-385 and IAEA-384
(NIST-4354)4.2-7
241Am
4.2.2. 241Am
4.2.2.1.
1620 241Am 241Am
Pu 239+240Pu 240Pu/239Pu
4.2.2.2
105ºC 24 80
5-10g 0.5 pg 243Am
450ºC 5 4.2.1.6241Am SF-ICP-MS 241Am
Pu 4.5.2.
4.2.2.3. Am Am
127
Am -
, Am 241Pu T1/2 = 14.4241Am T1/2 = 433 241Pu
241Am
16
20 241Am 239+240Pu240Pu/239Pu 4.2-2
241Am 241Am 239+240Pu0.136 0.219 mBq/g 0.219
mBq/g 20 241Am 0.100 ± 0.047 mBq/g241Am 241Am
Yamamoto 1983 1963 1976 15
30 15 2 1957
1980 15 241Am 241Am 0.030 0.337 mBq/g 1963
30 241Am 0.163 ± 0.085 mBq/g 1976
30 241Am 0.118 ± 0.078 mBq/g241Am
241Am 0.407 2.701 mBq/g
(Yamamoto et al., 1980) 239+240Pu 240Pu/239Pu 241Am/239+240Pu activity ratio 4.2-3
240Pu/239Pu 0.166 0.183
Kelley et al., 1999 Pu
20 3.6 20.2 4.2-2 Pu241Am (Ovsiannikova et al., 2010) 4.2-8A
241Am
4.2-8B C 241Am 239+240Pu 137Cs241Am 239+240Pu 137Cs 241Am
137Cs Pu 241Am/239+240Pu 0.34
0.43 ( 4.2-3)
(0.69 ± 0.08) Pu 241Am
241Am/239+240Pu 241Am
4.2-9 19 241Am/239+240Pu
0.39±0.02 4.2-9A 4.2-9B Yamamoto 1983241Am/239+240Pu (1955-1980) 4.2-9B
1957 1958 241Am / 239+240Pu 0.44 19610.30
128
241Pu
2
1952-1958 1961-1962
(Hisamatsu et al., 1978; Koide et al., 1981) 1 241Pu / 239+240Pu
2 4.2-9B 1957 1958241Am / 239+240Pu
241Pu/239+240Pu 1961 241Am / 239+240Pu
( 0.30) 4.2-9A
19 241Am/239+240Pu (0.39±0.02) Yamamoto (1983)
1960-1980 241Pu 1980241Am
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. .
131
Th 4.3.1.
Th Th -
TF Wang, et al., 2015ICP-MS
Th <1 – 100 mg kg-1 Yamasaki et al., 2001; Yoshida et al., 1998
Th 5.4
mg kg-1 (2.3 – 11 mg kg-1) 5.0 mg kg-1 (1.2 – 12 mg kg-1) Uchida et al. 2007a; Uchida et al.
2007b ThICP-MS Th 100 232
Ostapczuk et al., 2010; Sahoo et al., 2011 ICP-MS
Th
ng g-1 Uchida et al. 2007b
Th Th
Th-
Th Th
Feng et al., 1999 26
Th -
26 4.3.2.
Th
4.3.2.
GBW 1573a
26 27 20 27
10 Th
4.3.3.
(1)
30 50g
50mL
(2)
80˚C 3 500 10mL
4mL 80˚C 10 1mL
10
130˚C 1mL 0.5mL
40 1mL 20mL20mL 2
132
1/40 GBW 1573a
(3) ICP-MS
ICP-MS 2% 26 100027 500 Th
Th 0, 0.01, 0.1, 0.2 ng mL-1 ICP-MS
SF-ICP-MS
SF-ICP-MS: Element XR with Jet interface
RF Power: 1.3 kW : 16 L min-1
: 1.0 L min-1
: 0.85 L min-1
: Conical concentric
: m/ m = 300
: Run x pass 15x5 : 209Bi (0.1 ng mL-1) 232Th, 209 Bi
4.3.4.
Th GBW
NIST-1573a 4.3-1 GBW (n = 2) NIST-1573a (n = 3) Th 0.075 – 0.079 0.099 – 0.136 mg/kg
GBW (0.070) NIST-1573a information value (0.12)
Th
26 27 20 27
10 Th 4.3-2 20Th 1.4×10-5 6.7×10-4 mg/kg / 48
1.8 ×10-4 1.0 ×10-4 mg/kg 27
10 Th 7.7×10-5 4.7×10-4 mg/kg / 6
2.1×10-4 1.8×10-4 mg/kg
Th Th /
8 / 8Th
Th
Uchida (2007b) Th
40 6.4 ×10-4 mg/kg 37 5.5 ×10-4 mg/kg
20 10 Th 6 3 Uchida
ICP-MS - SF-ICP-MS
133
Th
Th Th -
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134
4.4.1.
-36 36Cl 30.1 35Cl
75.78
TF
2014
NAA
ICP-MSTF
TF
TMAH
2016
TMAH ICP
4.4.2. TMAH
H26 TMAH
2015
NAA Cl 26
NAA
100
mg Savillex 6 mL 25 TMAH Tama pureAA-1002 mL Milli-Q 1 mL 80 16
Milli-Q 50 mL 3000 rpm, 10 min.
0.45µm PTFE Millipore, ICP-MS
4.4.3
INAA TMAH 4.4-1
NAA TMAH4.4-2 Br I -ICP-MS 0.35±0.15 Br
135
0.97±0.13 I 0.83±0.09 3 1 TMAH
TMAH NAA
Yamada 1996
TMAH Takeda 2011Br I I
Tagami et al., 2010
4.4.3. TMAH ICP-MS
ICP-MS 8800 2
DL MS/MS + He 35 -> 35He MS/MS
2 35 Br I
ICP-MS
TMAH H2O2
1 TMAH Cl, Br, I5 mL PTFE , 30 mL H2O2 Tama pureAA-100
0.1 0.5 1.0 mL 100 2.5 4.4-3
13 mL PP 4.4-4
TMAH 0.45µm5mL PP 0.5mL H2O2 100 1
4.4.4. TF
80 RSDRSD 8
4.4-1
RSD 4.4-2
RSD
TF 4.4-3
Cl>Br>I Cl, Br, I 114 80 19 mg/kg
4540, 30, 0.14 mg/kg
TF 58 0.54 0.01
4.4-4
Tsukada and Nakamura 1998 Yuita 1983 TFTF Tsukada and Nakamura (1998) IAEA 2010
136
Yuita 1983
TF TF Yuita 1983
TF
4.4.5.
TMAH
35
TMAHH2O2 ICP-MS/MS
80 8%
Cl TF Cl
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137
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138
Pu - 4.5.1.
Bq / kg
TF ICRU, 2001 1994 IAEA TF
TRS-364 (IAEA TRS-364, 1994) IAEA TF
TRS 472 (IAEA TRS-472, 2010) TRS-472 Pu
TF
TF (Wang et al., 2015a)
TF 25 Pu 26
Pu 27
Pu - TF Pu
Pu
26 Pu 4 Pu- TF
4.5.2.
4.5.2.1.
Pu - TF
4 No.7 - No.10 4.5-1 PuIAEA Soil-6 JSAC-0471
4.5.2.2.
HCl, HNO3, HF, NaNO2, NH4I, H2O2, HBr, H3BO3, NH3, FeCl3, ascorbic
acid, TiCl3, Ca(NO3)2, La(NO3)3, NH2OHHCl, Iron (II) sulfamate
Bio-Rad 2 AG 1X8 100-200 mesh, Cl- form AG MP-1M 100-200 mesh, Cl- form Tama Chemicals
HNO3 SF-ICP-MS
Eichrom 3 TEVA UTEVA DGA 50 100 m
2mL 242Pu (CRM 130, plutonium spike
assay and isotopic standard, New Brunswick Laboratory, USA)
>18 MΩ cm-1 240Pu/239Pu 0.242 PuNBS-947
4.5.2.3. Pu
Pu ( 4.5-2 1-2.5 g
0.2 g 0.57 pg 242Pu
450 (Wang et al., 2015b) 5
139
120 mL Savillex Corporation, Minnesota, USA
10 mL 160˚C 4
50 mL Milli-Q
35mL 3.8M HNO3 100mg Ca 100mg La2mL 20 TiCl3 Pu IV Pu III 46 HF 7mL
15-20 3000rpm 15
H3BO3 0.5g 3M HNO3 20mL
Pu 0.3g NaNO2
Pu IV 40 0.510mL 3M HNO3 TEVA 10mL 3M HNO3
Ca Fe REEs 40mL 1M HNO3
U Pb Tl Pt 10mL 9M HCl Th Bi Hf Pu
3M HNO3 10mL UTEVA DGA TEVA
Pu IV Pu III TEVA Pu III 3M HNO3 - 0.1M
-0.02M Fe 2+ 25 20mL PuIII UTEVA DGA TEVA UTEVA
DGA U Tl Pb Pt Hf Fe DGA 30mL 0.1M
HNO3 DGA Pu 20mL 0.5M HCl-0.1M NH2OH HCl
4mL 200
1mL HNO3 4 HNO3 0.7mL
SF-ICPMS 26 Pu Pu
26 4.2.3.5
Pu SF-ICP-MS (Element XR) APEX-Q Zheng, 2015238U, 239Pu, 240Pu, 241Pu, 242Pu
10%
0.02 ng mL-1 Merck standard SF-ICP-MSSF-ICP-MS Pu 26 4.2-1
4.5.3.
4.5.3.1. Pu 239+240Pu 239Pu 240Pu/239Pu 4.5-1 4.5-1
27 1-6 Pu
1945 Pu (Yamamoto et al., 1983;
Saito-Kokubo et al., 2008) 60 (UNSCEAR, 1982;
Kelley et al., 1999) 2011 Pu (Zheng et al.,
2012) Pu 240Pu/239Pu
3 Pu 240Pu/239PuPu 240Pu/239Pu
140
7 240Pu/239Pu
0.160 0.182
Kelley et al., 1999 Pu
239+240Pu 0.204 0.919 mBq/g 239Pu 0.12
0.56 mBq/g Pu Yamamoto
1983 1963 1976 15 30
15 2 1957 1980
15 239+240Pu 239+240Pu 0.078 1.03
mBq/g 239+240Pu Yamamoto
Muramatsu et al., 2003
4.5.3.2. Pu
Pu Pu Pu
Pu
PuPu
20 30 ICP-MS 239Pu 240Pu240Pu
239Pu 4.5-2
4.5-2 , 239Pu 0.25× 10-5 – 1.9 × 10-5 mBq/g
8.5 × 10-6 mBq/g 5
4.5.3.3. Pu -
Pu - TF
27 239Pu
Pu-TF 4.5-2
Pu - TF 4.5×10-6 1.0×10-4
2.7×10-5 3.7×10-5
TF 1 2 Pu
4.5-3
239,240Pu Duffa 2002 Zhang 1989 238Pu
Adriano et al., 1981
TF - re-suspension(Wang et al., 2015a) Pu
TF re-suspension TF
Pu
Pu
Pu1 4 Baeza et al., 2006
141
(Guillen et al., 2016)
TF 1 2
TF
IAEA TRS-472 Pu - TF -TF 4.5-3 4.5-3 TRS-472
Pu-TF Pu-TF -
TF 9.5 10-6 N=105 IAEA TRS-472
- TF 2.7×10-5 (n = 10) Pu -
TF
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6 Pu, Am, Th Cl -
4.6.1.
2010 IAEA Technical Reports Series No. 472 Handbook of Parameter Values for the Prediction of
Radionuclides Transfer in Terrestrial and Freshwater Environments IAEA, 2010TF TRS-472 TF
Review paper
TRS-472
TECDOC-1616 TRS-472
TF Cs Sr
Th Pu Cl
Cu Ag Na W 100 IAEA, 2009
TRS-472 2007
TF 20072006-2007
Wang 2007 2014 TRS-472
4 Pu, Am, Th Cl TF
Wang et al. 2015
TF Pu Cl Am Th 2015 2016
TF
4.6.2.
8 2
Nie et al. (2010) Tuovinen et al. (2016) Matveyeva et al. (2015) Asaduzzaman et al. (2015) Hossen and
Ferdous 2015 Alsaffar et al. (2015) Chauhan and Kumar 2015 Alsaffar et al. (2016) Mostafa et al. (2016) Planinsek et al. (2016) Yan 2016 Th - TF
Todorov Djingova (2015) Li et al. (1994) Guillen (2016)
Am TF Guillen (2016) Pu 2
TF Froehlich 2016 AMS239Pu Pu 2 TF
Wang Wang 2015TF
144
GM AM GSD SD
N
GM
TF Th Am Pu Cl 4.6-1 4.6-3
4.6.3. IAEA TRS 472
4.6-1
Nie et al. 2010 U
Th U ICP-MS Th TFs
2.0 10-3 4.2 10-1 n 36 3.6 10-2 Yan 2016U N = 12 232Th Th TF
TF-Th 1 10-2 3.1 10-1 GM 1.1 10-1
Tuovinen (2016) TF U 0.5m3
Th ICP-MS
TF 1.0 10-2 5.8 10-1
Matveyeva et al. (2015) U232Th 228Th 230Th 232Th
TF 2.0 10-3 1.9 10-1 Nie 2010230Th TF 232Th 228Th
TF
Th TF Asaduzzaman
et al. (2015) Alsaffar et al. (2015) Alsaffar et al. (2016) 23, 3 4 Alsaffar et al. 2015
TF 4.0 10-3 1.4 10-2 Th
8 11 24 57 Th
Alsaffar et al. (2016) Th - TF232Th , 188 Bq/kg
Th TF1.1 10-2 Asaduzzaman et al. 2015
232Th Asaduzzaman TF 0.18 0.48
Hossen Ferdous 2015 10
TF TF 0.14 - 0.5 IAEA
4.6-1 2 Mostafa et al. (2016) 232Th
4TF TF-Th IAEA 0.14 1 Planinsek
et al. (2016) U U
TF 230Th 5.8 10-4 2.0 10-2
6.8 10-4 ~1.6 10-2 1.6 10-4 3~2.03 10-2 1.4 10-3~2.0 10-2
Th-TF 1.5 10-2
TF IAEA 1.2 10-3 1TF IAEA
145
IAEA TF232Th 228Ac 212Pb 208Tl
232Th 232Th228Ra 224Ra Th 228Ac
212Pb 208Tl Th ThTF Wang et al 2015
4.6-2 Li 1994 Todorov and Djingova 2015 Guillen 2016 Am-TF
Li (1994) 3241Am
TF 6.2 10-4 5.1 10-4
Todorov Djingova (2015) 5 Am- TF 241Am 2000-2500 Bq / kg
6 241Am
TF 9.0 10-5-9.3 10-3 Am
Guillen 2016 241Am
- TF Am-TF
4.8 0.2 IAEA 3.0 10-7 5.8 10-2
241Am 241Am
1 4 TF
Am-TF
(ICRP, 2010; Todorov and Djingova, 2015; Gomez and Brown, 2013,
Guillen et al. 2016)
Pu 4 4.6-3 Guillen (2016) 239Pu Pu-TF ( 1.5 0.046 )
IAEA 4.4 10-7 9.0 10-4 Froehlich
2016 2 - TF 1.5 10-3 4.7 10-3
TRS-472 1
TRS 472 Th Am Pu TF 4.6-1 4.6-3X TRS-472
4.6-1
Th-TF IAEA TF
IAEA TF
4.6-2 Todorov Djingov (2015) Li (1994) Guillen
(2016) Am-TF TRS-472 4.6-3Pu-TF IAEA
TRS-472
4.6-3 Pu-TF TRS-472
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4.7.1. Am Cl
4.7.1.1. Am
DGA-N TEVA Am / REEs3
SF-ICP-MS 2 20g 241Am
HNO3 CaC2O4
Am Na K Mg Al Fe UTEVA + DGA-N
Am TEVA REEs Aridus (II)-SF-ICP-MS241Am DF
Pu 7 105 241Am241Am ICP-MS 241Am
6 241Am241Am Am
76 82 LOD 0.012 mBq/g 241Am
16
20 241Am241Am
241Am 239+240Pu 0.136 0.219 mBq/g
4.7.1.2. TMAH
TMAH H2O2
ICP-MS/MS TF
4.7.2. Th
26 27 20 27
10 Th 20 Th 1.4×10-5 6.7×10-4 mg/kg
/ 48 1.8×10-4
1.0×10-4 mg/kg 27 10 Th 7.7×10-5
4.7×10-4 mg/kg / 6
2.1×10-4 1.8×10-4 mg/kg Th Th
/ 8
Th Th
Th -
4.7.3. Pu -
150
8 Pu Pu 240Pu/239Pu Pu Pu
Pu Pu - TF TF
4.5×10-6 1.0×10-4 2.7×10-5 TF-Pu
Pu TF Pu TF TF TF-Pu
151
152
4.2-1 CaC2O4 UTEVA + DGA-N Am 5g JSAC-0471 SF-ICP-MS 1mL
Matrix Na K Mg Ca Fe Al
Concentration ( g/mL) 1.5±0.2 7.6±1.1 0.1±0.0 1.9±1.6 2.2±0.2 1.7±0.4 REEs La Ce Nd Sm Dy
Concentration ( g/mL) 6±2 16±5 66±14 24±2 8±1
4.2-2 241Am
Organic matter 241Am activitySample code FAO-UNESCO Prefecture (%) mBq/g std
EF-SD-01 Andosol 18.0 0.067 0.017EF-SD-06 Fluvisol 8.5 0.154 0.011EF-SD-07 Andosol 8.4 0.084 0.012EF-SD-08 Cambisol 3.6 0.036 0.011EF-SD-09 Cambisol 5.4 0.089 0.014EF-SD-10 Andosol 17.0 0.122 0.015EF-SD-11 Fluvisol 7.0 0.060 0.010EF-SD-13 Fluvisol 7.1 0.110 0.014EF-SD-17 Fluvisol 20.0 0.058 0.015EF-SD-18 Andosol 14.2 0.113 0.013EF-SD-21 Fluvisol 6.5 0.104 0.015EF-SD-22 Cambisol 6.9 0.064 0.012EF-SD-23 Cambisol 6.6 0.037 0.010EF-SD-24 Fluvisol 6.3 0.058 0.011EF-SD-25 Fluvisol 8.1 0.099 0.010EF-SD-29 Cambisol 10.8 0.085 0.014EF-SD-30 Andosol 20.2 0.219 0.027EF-SD-35 Fluvisol 10.2 0.118 0.013EF-SD-36 Andosol 12.4 0.179 0.019EF-SD-37 Fluvisol 6.8 0.139 0.009
153
4.2-3 Pu 241Am/239+240Pu activity
4.3-1 Th
Th (mg/kg) std GBW-1 0.075 0.002 GBW-2 0.079 0.001 certified value 0.070 0.008 NIST-1573a-1 0.120 0.001 NIST-1573a-2 0.136 0.002 NIST-1573a-3 0.099 0.001 information value 0.12
239+240Pu activitySample code FAO-UNESCOPrefecture mBq/g std 240Pu/239Pu std 241Am/239+240Pu std
EF-SD-01 Andosol 0.182 0.001 0.182 0.015 0.37 0.09EF-SD-06 Fluvisol 0.384 0.007 0.166 0.016 0.40 0.03EF-SD-07 Andosol 0.207 0.002 0.169 0.014 0.41 0.06EF-SD-08 Cambisol 0.105 0.001 0.173 0.018 0.34 0.10EF-SD-09 Cambisol 0.227 0.002 0.182 0.015 0.39 0.06EF-SD-10 Andosol 0.339 0.005 0.172 0.017 0.36 0.04EF-SD-11 Fluvisol 0.161 0.001 0.175 0.012 0.37 0.06EF-SD-13 Fluvisol 0.256 0.003 0.172 0.016 0.43 0.05EF-SD-17 Fluvisol 0.159 0.001 0.183 0.019 0.37 0.10EF-SD-18 Andosol 0.290 0.003 0.182 0.013 0.39 0.04EF-SD-21 Fluvisol 0.283 0.002 0.170 0.008 0.37 0.05EF-SD-22 Cambisol 0.169 0.001 0.179 0.013 0.38 0.07EF-SD-23 Cambisol 0.100 0.000 0.180 0.012 0.37 0.10EF-SD-24 Fluvisol 0.145 0.001 0.183 0.014 0.40 0.08EF-SD-25 Fluvisol 0.254 0.001 0.174 0.008 0.39 0.04EF-SD-29 Cambisol 0.218 0.001 0.180 0.008 0.39 0.06EF-SD-30 Andosol 0.595 0.016 0.178 0.018 0.37 0.05EF-SD-35 Fluvisol 0.171 0.001 0.177 0.012 0.69 0.08EF-SD-36 Andosol 0.434 0.008 0.166 0.015 0.41 0.04EF-SD-37 Fluvisol 0.325 0.007 0.171 0.022 0.43 0.03
154
4.3-2 Th
Th (mg/kg) stdEP II-CF-1 6.7E-04 4.5E-05EP II-CF-2 NDEP II-CF-3 1.9E-04 1.9E-05EP II-CF-4 4.3E-05 2.0E-05EP II-CF-5 3.0E-05 1.1E-05EP II-CF-6 3.7E-05 1.5E-05EP II-CF-7 3.1E-05 1.1E-05EP II-CF-8 3.6E-04 2.8E-05EP II-CF-9 9.6E-05 2.5E-05EP II-CF-10 NDEP II-CF-11 3.7E-04 1.4E-05EP II-CF-12 3.0E-04 1.7E-05EP II-CF-13 2.8E-04 2.6E-05EP II-CF-14 5.1E-05 1.2E-05EP II-CF-15 2.7E-04 2.0E-05EP II-CF-16 NDEP II-CF-17 1.0E-04 1.4E-05EP II-CF-18 2.9E-05 5.6E-06EP II-CF-19 1.2E-04 2.5E-05EP II-CF-20 1.4E-05 7.0E-06Minimum 1.4E-05Maximum 6.7E-04Max./Min. 48Median 9.9E-05Arithmetric mean 1.8E-04Geometric mean 1.0E-04EP II-CF-11 2.9E-04 6.0E-06EP II-CF-12 2.5E-04 4.1E-05EP II-CF-13 4.7E-04 9.5E-06EP II-CF-14 1.4E-04 5.8E-06EP II-CF-15 2.0E-04 1.4E-05EP II-CF-16 7.9E-05 5.6E-06EP II-CF-17 1.7E-04 5.8E-06EP II-CF-18 7.7E-05 5.4E-06EP II-CF-19 2.3E-04 1.1E-05EP II-CF-20 1.5E-04 8.2E-06Minimum 7.7E-05Maximum 4.7E-04Max./Min. 6Median 1.9E-04Arithmetric mean 2.1E-04Geometric mean 1.8E-04
155
4.4-1 TMAH RSD(%)
*H27
4.4-2 RSD(%)
*H27
Code Cl mg/kg Br mg/kg I mg/kg
EFII Run-1 RSD Run-2 RSD Run-1 RSD Run-2 RSD Run-1 RSD Run-2 RSD
SD-1 51 18 29 11 7.3 1 7.2 5 1.9 17 1.8 7
SD-2 62 16 85 1 7.9 1 8.7 5 1.5 11 1.6 9
SD-3 90 15 76 5 113 2 115 3 30 0 29 4
SD-4 106 11 92 2 132 2 132 3 32 1 32 4
SD-5 99 5 88 5 110 1 110 3 32 2 31 4
SD-6 174 3 189 6 41 1 44 3 10 2 11 5
SD-7 222 3 210 4 158 1 161 3 21 1 22 4
SD-8 194 1 192 5 125 1 126 3 18 3 19 4
SD-9 37 18 32 10 54 0 53 5 30 2 29 4
SD-10 136 4 123 7 47 1 47 5 11 3 11 6
H27* RSD 78 (37-130) 2 (0-5) 2 (1-4)
Code Cl mg/kg Br mg/kg I mg/kg
EFII Run-1 RSD Run-2 RSD Run-1 RSD Run-2 RSD Run-1 RSD Run-2 RSD
CF-1 2530 2 2760 4 8.2 5 8.9 7 - - 0.026 21
CF-2 6380 2 6310 5 9.1 4 9.0 8 0.033 45 0.026 37
CF-3 1110 5 1060 4 10.4 6 10.0 5 0.037 44 0.022 71
CF-4 4770 4 4530 5 113 6 108 6 0.137 17 0.124 10
CF-5 5180 4 4890 6 46 5 44 7 0.290 9 0.357 5
CF-6 11900 7 11300 5 15.3 7 15.0 6 0.098 22 0.070 41
CF-7 2630 7 2500 4 29 7 28 4 0.104 20 0.101 33
CF-8 2110 6 2030 3 9.3 6 9.3 3 0.128 15 0.189 14
CF-9 5050 10 4720 5 51 8 50 5 0.347 11 0.360 9
CF-10 4760 9 4320 5 12.7 7 13.6 5 0.140 15 0.160 14
H27* RSD 7 (1-35) 2 (1-10) 19 (4-33)
156
4.4-3 TF
4.4-4.
Reference Cl Br I
58 (11 – 141) 0.54 (0.07 – 1.2) 0.010 (0.001 – 0.019)
2016 42 (9 – 138) 0.69 (0.05 – 3.2) 0.011 (0.002 – 0.038)
Tsukada and Nakamura, 1998
15 44 0.36 1.7 0.005, 0.015
Yuita, 1983 127 (10-265) 0.79 (0.36-1.8) 0.011 (0.005-0.028)
TRS-472 (IAEA, 2010)
26 (14 – 48) - 0.0065
Code Cl Br I
EFII- Crop Soil TF Crop Soil TF Crop Soil TF
CF-1 2640±120 40±10 66 8.6±0.7 7.3±0.4 1.2 0.026 1.8±0.3 0.014
CF-2 6340±330 73±10 87 9.0±0.8 8.3±0.4 1.1 0.029±0.018 1.6±0.2 0.019
CF-3 1090±70 83±14 13 10.2±0.9 114±4 0.09 0.029±0.022 29.4±1.1 0.001
CF-4 4650±280 99±11 47 110±9 132±5 0.83 0.130±0.026 31.8±1.3 0.004
CF-5 5030±350 94±7 54 45±4 110±3 0.41 0.324±0.033 31.4±1.4 0.010
CF-6 11600±980 181±12 64 15.1±1.4 43±2 0.35 0.084±0.036 10.6±0.5 0.008
CF-7 2560±200 216±11 12 28±3 160±5 0.18 0.103±0.040 21.3±1.0 0.005
CF-8 2070±150 193±11 11 9.3±0.6 125±4 0.07 0.159±0.032 18.7±0.9 0.009
CF-9 4880±550 35±7 141 50±5 54±3 0.93 0.353±0.049 29.3±1.4 0.012
CF-10 4540±490 129±10 35 13.1±1.1 47±3 0.28 0.150±0.031 10.7±0.7 0.014
157
4.5-1 Pu 240Pu/239Pu 1-6, 27 7-10, 28
Sample ID
Prefecture 239Pu activity (mBq/g)
239+240Pu activity(mBq/g)
240Pu/239Pu atom ratio
1 Akita 5.55 ± 0.15 × 10-1 8.85 ± 0.30 × 10-1 0.162 ± 0.008
2 Niigata 2.78 ± 0.09 × 10-1 4.48 ± 0.02 × 10-1 0.166 ± 0.010
3 Toyama 2.20 ± 0.09 × 10-1 3.57 ± 0.10 × 10-1 0.171 ± 0.008
4 Gifu 3.62 ± 0.15 × 10-1 6.04 ± 0.31 × 10-1 0.182 ± 0.013
5 Nagasaki 1.47 ± 0.06 × 10-1 2.34 ± 0.11 × 10-1 0.160 ± 0.011
6 Fukushima 2.36 ± 0.12 × 10-1 3.93 ± 0.30 × 10-1 0.167 ± 0.012
7 Chiba 2.32 ± 0.11 × 10-1 3.87 ± 0.29 × 10-1 0.181 ± 0.013
8 Toyama 2.44 ± 0.08 × 10-1 3.92 ± 0.73 × 10-1 0.165 ± 0.012
9 Gifu 5.52 ± 0.33 × 10-1 9.19 ± 0.07 × 10-1 0.180 ± 0.014
10 Nara 1.23 ± 0.03 × 10-1 2.04 ± 0.23 × 10-1 0.179 ± 0.006
158
4.5-2 239Pu Pu -
4.5-3 Pu -
Sample ID Sampling location 239Pu in rice (mBq/g) std 239Pu in soil (mBq/g) std TF7 (EF-SD-40) Chiba 5.3E-06 1.5E-06 2.3E-01 1.1E-02 2.3E-058 (EF-SD-42) Toyama 4.9E-06 1.7E-06 2.4E-01 8.4E-03 2.0E-059 (EF-SD-43) Gifu 2.5E-06 8.9E-07 5.5E-01 3.3E-02 4.5E-0610 (EF-SD-45) Nara 1.3E-05 1.1E-06 1.2E-01 2.9E-03 1.0E-041 (EP-SD-64) Akita 1.9E-05 1.7E-05 5.6E-01 1.5E-02 3.5E-052 (EP-SD-65) Niigata 8.0E-06 2.9E-06 2.8E-01 9.0E-03 2.9E-053 (EP-SD-66) Toyama 4.5E-06 1.7E-06 2.2E-01 9.0E-03 2.0E-054 (EP-SD-67) Gifu 9.0E-06 2.2E-06 3.6E-01 1.5E-02 2.5E-055 (EP-SD-68) Nagasaki 1.2E-05 6.5E-06 1.5E-01 6.0E-03 8.2E-05
6 (OK-K2) Fukushima 6.6E-06 2.5E-06 2.4E-01 1.2E-02 2.8E-05RemarksThe 240Pu/239Pu atom ratio of EF-SD-45 was determined to be 0.195 ± 0.049, indicating global fallout sourceRange of TF of Pu for rice 4.5E-06 - 1.0E-04Minimum 4.5E-06Maximum 1.0E-04Max./Min. 22.7Median 2.6E-05Arithmetric mean (AM) of TF 3.7E-05Geometric mean (GM) of TF 2.7E-05
159
4.6-
120
08-2
016
Th−
a:
Und
er n
atur
al fi
eld
cond
ition
s, TF
s wer
e ob
tain
ed b
y ex
amin
ing
232 Th
con
cent
ratio
ns in
the
plan
t and
cor
resp
ondi
ng so
il sa
mpl
es.
b: In
an
aban
done
d ur
aniu
m m
ine,
TFs
wer
e ob
tain
ed b
y ex
amin
ing
230 Th
(or 23
2 Th) c
once
ntra
tions
in th
e pl
ant a
nd c
orre
spon
ding
soil
sam
ples
. c:
In U
-mill
taili
ng d
ispo
sal s
ites,
TFs w
ere
obta
ined
by
exam
inin
g 23
0 Th c
once
ntra
tions
in th
e pl
ant a
nd c
orre
spon
ding
soil
sam
ples
.
Plan
t Gro
up
N
AM
SD
G
M
GSD
M
in.
Max
. TR
S 47
2 G
M
Ref
. No.
R
emar
k
Gra
ss
183
1.3×
10-1
1.
4×10
-1
6.0×
10-2
4.
4 2.
0×10
-3
9.0×
10-1
4.
2×10
-2
e Ref
(Gra
ss)
Nat
ural
fiel
d TF
sa U
min
e ta
iling
TFs
c 20
16 d
ata
entri
es: 1
2 Le
afy
Veg
etab
le
25
1.1×
10-1
1.
5×10
-1
1.5×
10-2
22
5.
8×10
-4
3.4×
10-1
1.
2×10
-3
Hos
sen,
201
5 Pl
anin
sek,
201
6 N
atur
al fi
eld
TFsa
Ura
nium
min
e TF
sb 20
16 d
ata
entri
es: 1
5 Fr
uit
edib
le p
art
ined
ible
par
t
18
7
1.5×
10-1
1.2×
10-1
4.5×
10-1
7.7×
10-2
6.0×
10-2
9.2×
10-2
7.0
6.3
2.5×
10-4
1.0×
10-3
1.3
0.7
f R
ef (F
ruit)
N
atur
al fi
eld
TFsa
Nat
ural
fiel
d TF
sa N
on-le
afy
Veg
etab
le
edib
le p
art
ined
ible
par
t
43
11
2.3×
10-1
3.4×
10-1
3.7×
10-1
2.7×
10-1
2.6×
10-2
2.4×
10-1
13
3.7
1.9×
10-4
3.8×
10-2
1.7
9.1×
10-1
7.8×
10-4
2.2×
10-3
g Ref
(N
on-L
eafy
V
eget
able
)
Nat
ural
fiel
d TF
sa N
atur
al fi
eld
TFsa
Cer
eal
(e
xcep
t ric
e)
38
5.5×
10-1
3.
3×10
-1
3.5×
10-1
12
3.
6×10
-4
1.0×
100
2.1×
10-3
j Ref
(Cer
eal)
Nat
ural
fiel
d TF
sa U
rani
um m
ine
TFsb
2016
dat
a en
tries
: 30
Ric
e ed
ible
par
t in
edib
le p
art
44
3
5.1×
10-2
3.0×
10-3
1.0×
10-1
2.0×
10-3
1.5×
10-2
2.5×
10-3
7.7
2.0
3.1×
10-5
1.0×
10-3
4.8×
10-1
5.0×
10-3
1.6×
10-4
h R
ef (R
ice)
N
atur
al fi
eld
TFsa
Pot e
xper
imen
t TFs
i 20
16 d
ata
entri
es: 4
Tu
ber
edib
le p
art
ined
ible
par
t
14
10
1.1×
10-1
3.6×
10-2
2.5×
10-1
2.9×
10-2
1.4×
10-2
2.9×
10-2
47
14
1.4×
10-3
1.3×
10-2
1.9×
10-1
1.2×
10-1
2.0×
10-4
1.9×
10-2
Asa
duzz
aman
, 20
14,
Kha
n 20
10;
C
hauh
an, 2
015
Plan
inse
k, 2
016
Nat
ural
fiel
d TF
sa
Ura
nium
min
e TF
sb 20
16 d
ata
entri
es: 5
Roo
t cro
p 6
5.9×
10-1
5.
5×10
-1
4.6×
10-1
2.
4 2.
8×10
-1
1.7
8.0×
10-4
A
sadu
zzam
an, 2
014
Shan
thi,
2012
N
atur
al fi
eld
TFsa
Tree
17
1.
5×10
-2
2.5×
10-2
2.
8×10
-3
12
4.6×
10-5
1.
0×10
-1
R
odrig
uez,
20
10;
Popi
c, 2
011;
Zh
ang,
198
9
Ura
nium
min
e TF
sb C
onta
min
ated
ar
ea
TFsd
160
d: In
a w
etla
nd si
te c
onta
min
ated
by
radi
oact
ive
was
te d
isch
arge
d fr
om a
nuc
lear
rese
arch
faci
lity,
TFs
for 23
2 Th w
ere
dete
rmin
ed.
e R
ef (G
rass
): N
ie, e
t al.,
201
0; T
uovi
nen,
et a
l., 2
016;
Mat
veye
va, e
t al.,
201
5; IC
RP,
200
9; A
lhar
bi a
nd E
l-Tah
er.,
2013
; Kris
tsan
anuw
at e
t al.,
201
4; C
erne
et a
l.,
2010
; Dra
govi
c et
al.,
201
0; K
han
et a
l., 2
011;
Ouf
ni e
t al.,
201
1; P
alla
vici
ni, 2
011;
Sm
odis
et a
l., 2
012;
Cha
krab
orty
et a
l., 2
013;
Stro
k an
d S
mod
is 2
013.
Yan
, 20
16.
f Ref
(Fru
it): A
lhar
bi a
nd E
l-Tah
er, 2
013;
Kris
tsan
auw
at e
t al.,
201
4; K
umar
et a
l., 2
008;
Sha
nthi
et a
l., 2
012
g Ref
(Non
-Lea
fy v
eget
able
): K
rists
anau
wat
et a
l., 2
014;
Zha
ng e
t al.,
201
1; S
hant
hi e
t al.,
201
2; A
swoo
d et
al.,
201
3; M
heem
eed
et a
l., 2
014.
h R
ef (R
ice)
: Asa
duzz
aman
, et a
l., 2
015;
Als
affa
r, et
al.,
201
5; K
rists
anau
wat
et a
l., 2
014;
Sha
nthi
et a
l., 2
012;
Sae
ed e
t al.,
201
2. A
lsaf
far,
et a
l., 2
016.
i:
In a
pot
exp
erim
ent u
sing
nat
ural
soil,
TFs
wer
e ob
tain
ed b
y ex
amin
ing
232 Th
con
cent
ratio
ns in
gra
in a
nd so
il sa
mpl
es.
j Ref
(Cer
eal):
Kha
n 20
10; M
ihay
lova
, el a
l.,
2013
; Alh
arbi
, et a
l., 2
013;
Mos
tafa
, et a
., 20
16.
4.
6-2
2008
-201
6A
m−
a:
In a
dun
e ad
jace
nt to
Sel
lafie
ld a
nd a
low
leve
l was
te d
ispo
sal s
ite, T
Fs fo
r 241 A
m w
ere
dete
rmin
ed.
b: In
lysi
met
ers s
pike
d w
ith 24
1 Am
, TFs
for A
m w
ere
obta
ined
by
exam
inin
g th
e 24
1 Am
con
cent
ratio
n in
pla
nt a
nd so
il sa
mpl
es.
c: In
nat
ural
con
ditio
ns, a
ggre
gate
d TF
s wer
e ob
tain
ed b
y ex
amin
ing
241 A
m c
once
ntra
tions
in th
e pl
ant a
nd c
orre
spon
ding
soil
sam
ples
. d:
In n
atur
al c
ondi
tions
, TFs
wer
e ob
tain
ed b
y ex
amin
ing
241 A
m c
once
ntra
tions
in th
e pl
ant a
nd c
orre
spon
ding
soil
sam
ples
. Pl
ant G
roup
N
A
M
SD
GM
G
SD
Min
. M
ax.
TRS
472
GM
R
ef. N
o.
Rem
ark
Gra
ss
28
0.24
0.
57
2.6×
10-3
10
3 9.
0×10
-5
1.4
3.3×
10-2
IC
RP,
2009
To
doro
v, 2
015
Con
tam
inat
ed a
rea
TFsa
241 A
m sp
iked
stud
y TF
sb Le
afy
Veg
etab
le
4 1.
2×10
-3
2.4×
10-3
6.
3×10
-5
19
3.6×
10-6
4.
9×10
-3
2.7×
10-4
G
omez
, 20
13,
Li, 1
994
241 A
m
spik
ed
stud
y TF
sb N
atur
al fi
eld
TFsd
Non
-leaf
y V
eget
able
edib
le p
art
ined
ible
par
t
7 3
1.4×
10-3
3.7×
10-4
1.4×
10-3
1.5×
10-4
6.9×
10-4
3.4×
10-4
11
1.5
9.0×
10-5
2.0×
10-4
3.7×
10-3
5.0×
10-4
3.6×
10-4
Leht
o, 2
013,
Li
, 199
4
Nat
ural
fiel
d TF
sc
Nat
ural
fiel
d TF
sd
Tube
r 3
1.1×
10-5
2.
3×10
-6
1.0×
10-5
1.
2 8.
4×10
-6
1.3×
10-5
2.
1×10
-4
Gom
ez, 2
013,
24
1 Am
spik
ed st
udy
TFsb
Roo
t cro
p 4
1.3×
10-3
2.
5×10
-3
6.2×
10-5
22
6.
9×10
-6
5.1×
10-3
6.
7×10
-4
Gom
ez,
2013
, Li
, 199
4
241 A
m
spik
ed
stud
y TF
sb N
atur
al fi
eld
TFsd
Cer
eal
ined
ible
par
t 2
2.5×
100
3.3×
100
2.0×
10-1
4.
8×10
0 7.
9×10
–5
Gui
llen,
2016
241 A
m sp
iked
stud
y TF
sb 20
16 d
ata
entri
es: 2
161
4.
6-3
2008
-201
6Pu
−
a: In
a d
une
adja
cent
to S
ella
field
and
a lo
w le
vel w
aste
dis
posa
l site
, TFs
was
det
erm
ined
by
exam
inin
g th
e 23
9,24
0 Pu c
once
ntra
tions
in p
lant
and
soil
b:
In a
con
tam
inat
ed a
rea
near
a d
ecom
mis
sion
ed n
ucle
ar fa
cilit
y, P
u TF
s wer
e de
term
ined
. c:
In n
atur
al e
nviro
nmen
t, TF
s wer
e de
term
ined
by
exam
inin
g 23
9 Pu c
once
ntra
tions
in th
e pl
ant a
nd c
orre
spon
ding
soil
sam
ples
d:
In ly
sim
eter
s con
tam
inat
ed w
ith 23
9,24
0 Pu, T
Fs fo
r Pu
wer
e ob
tain
ed b
y ex
amin
ing
the
239,
240 Pu
con
cent
ratio
n in
pla
nt a
nd so
il sa
mpl
es.
e: In
nat
ural
con
ditio
ns, a
ggre
gate
d TF
s wer
e ob
tain
ed b
y ex
amin
ing
239,
240 Pu
con
cent
ratio
ns in
the
plan
t and
cor
resp
ondi
ng so
il sa
mpl
es.
f: In
lysi
met
ers c
onta
min
ated
with
239 Pu
, TFs
for P
u w
ere
obta
ined
by
exam
inin
g th
e 23
9 Pu c
once
ntra
tion
in p
lant
and
soil
sam
ples
. Pl
ant G
roup
N
A
M
SD
GM
G
SD
Min
. M
ax.
TRS
472
GM
R
ef. N
o.
Rem
ark
Gra
ss
20
2.5×
10-2
7.
8×10
-2
2.3×
10-4
44
1.
1×10
-6
3.3×
10-1
1.
6×10
-4
ICR
P,20
09 X
u,
2009
, Li,
2011
Fr
oehl
ich,
201
5
Con
tam
inat
ed a
rea
TFsa
Con
tam
inat
ed a
rea
TFsb
Nat
ural
fiel
d TF
sc
Leaf
y V
eget
able
3
1.9×
10-5
1.
7×10
-5
1.5×
10-5
2.
0 7.
9×10
-6
1.1×
10-5
8.
3×10
-5
Gom
eze,
201
3,
Lysi
met
er st
udy
TFsd
Non
-leaf
y V
eget
able
ed
ible
par
t in
edib
le p
art
1 3
3.0×
10-5
1.9×
10-4
1.2×
10-4
1.5×
10-4
2.0
6.0×
10-5
3.0×
10-4
6.5×
10-5
Leht
o, 2
013
Leht
o, 2
013
Nat
ural
fiel
d TF
se
Nat
ural
fiel
d TF
se Tu
ber
3 1.
4×10
-5
3.1×
10-6
1.
3×10
-5
1.2
1.1×
10-5
1.
7×10
-5
1.1×
10-4
G
omez
e, 2
013,
Ly
sim
eter
stud
y TF
sd R
oot c
rop
3 2.
2×10
-5
1.7×
10-5
1.
6×10
-5
2.4
5.1×
10-6
3.
9×10
-5
3.9×
10-4
G
omez
e, 2
013,
Ly
sim
eter
stud
y TF
sd C
erea
l
ined
ible
par
t 2
7.7×
10-1
1.
0×10
0
4.
6×10
-2
1.5×
100
4.4×
10–5
G
uille
n,20
16
Lysi
met
er st
udy
TFsf
2016
dat
a en
tries
: 2
162
4.2-1 Aridus II SF-ICP-MS (Element XR)
4.2-2 DGA-N
163
4.2-3 Fe(OH)3 CaC2O4 CaF2 n = 3
4.2-4 DGN 0.05M HNO3 Am REE (a) TEVA Am REE (b)
164
4.2-5 SF-ICP-MS Am
4.2-6 DGA-N 0.5M HCl TEVA 4M HCl Am
165
4.2-7 IAEA-soil-6 IAEA-375 NIST-4357, IAEA-385 IAEA-384 (NIST-4354) 241Am
166
4.2-8 241Am 239+240Pu 137Cs
167
4.2-9 241Am/239+240Pu 241Am 241Am/239+240Pu
168
4.4-1 NAA TMAH -ICP-MS
4.4-2 TMAH
169
4.4-3 1 TMAH 100
4.4-4 1 TMAH 100
170
4.5-1
(1-6, 27 7-10, )
171
4.5-2 Pu HNO3 -
172
4.5-3 Pu - IAEA TRS-472
4.6-1 2008 2016 Th - IAEA TRS-472 ( TF
2015-2016.2 2016.2-2016.12)
173
4.6-2 2008 2016 Am - IAEA TRS-472TF
2015-2016.2 2016.2-2016.12
4.6-3 2008 2016 Pu - IAEA TRS-472TF
2015-2016.2 2016.2-2016.12
174
14C
Pu, Am, Th Cl
TF Kd
Pu, Am, Th Cl
3
175
TF Kd
TF Kd
—TF Cs - Kd
135Cs
Cs
5.2.1. TF
TF
90Sr 137Cs
Ni, Sr, Mo Pb
Ni 3
5 Co, Zn, Cu, As, Cd
5.2.2. − TF
28 10 5 5
10 5 5
26 3
1520 TF
TF 26 28
14-18
26-28
176
5.2.3. TF
Na, Mg, Al, Si, P, K, Ca, Cr, M, Fe, Co, Ni, Cu, Zn, Sr, Cd, Ba 14-18
TF
18.4 25.3 7 TF Fe, Zn, p<0.01
Pinson 2015
TF
7 TF
37 Na, Mg, Al, Si, P, K, Ca, Sc, Ti, V, Cr, Mn, Fe,
Co, Ni, Cu, Zn, Se, Rb, Sr, Y, Zr, Nb, Mo, Cd, Sn, Sb, Cs, Ba, La, Ce, Sm, Eu, Gd, Pb, Th, UTF
20
5.2.4. Kd
20 30 Kd
10 23 Kd Kd 10 3.88×103
20 2.34×103 30 1.91×103 Kd
10 Kd 1000
30
5.2.5. Cs
27-28 Tag 5.3×10-5
1.6×10-4 m2 kg-1
137Cs
Tag 3.4×10-3 m2 kg-1 5.5×10-3 m2 kg-1 3.8×10-3 m2 kg-1 Cs
177
Tag 137Cs
137Cs 137Cs137Cs 137Cs
13C 15N
TF Tag Kd
178
14C14C 14C
14C14C
14C14C
5.3.1. 14C 14C 14C TRU
[1,2-14C] 0.5 g
4.2 × 105 Bq 14C 14C14C 4.2 × 103
Bq/mL 14C 14C14C
14C 25˚C 30˚C14C 14C
14C
5.3.2.
7
7
14CO2
14C
4 3
14C
1
5.3.3. 14C
179
14C
-
180
Pu, Am, Th Cl
14 18− TF - Kd
Pu, Am, Th Cl
Pu, Am, Th
TF
5.4.1. Am Cl 5.4.1.1. Am
DGA-N TEVA Am REEs
3SF-ICP-MS 2 20g 241Am
Am HNO3 CaC2O4 Am
Na K Mg Al Fe UTEVA + DGA-N Am
TEVA REEs Aridus (II)-SF-ICP-MS241Am Pu DF
7 105 241Am241Am ICP-MS 241Am
6241Am Am
76 82 LOD
0.012 mBq/g 241Am
16
20 241Am 241Am 239+240Pu 0.136
0.219 mBq/g
5.4.1.2. TF TMAH
TMAH H2O2 ICP-MS/MS
TF
5.4.2. -
181
26 27 20 27
10 Th 20 Th 1.4×10-5 6.7×10-4 mg/kg
/ 48 1.8×10-4
1.0×10-4 mg/kg 27 10 Th 7.7×10-5 4.7×10-4
mg/kg / 6 2.1×10-4
1.8×10-4 mg/kg Th Th /
8
Th Th Th
-
8 Pu Pu 240Pu/239Pu Pu Pu
Pu Pu - TF TF
7.0×10-6 1.1×10-4 3.1×10-5 TF-Pu
Pu TF TF-Pu
182
183
184
185
186
RI
Pu
187