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  • Surface resonant states and superlensing in acoustic metamaterials

    Muralidhar Ambati, Nicholas Fang, Cheng Sun, and Xiang Zhang*Center for Scalable and Integrated Nanomanufacturing (SINAM), University of California, Berkeley, California 94720, USA

    Received 19 April 2007; published 31 May 2007

    We report that the negative material responses of acoustic metamaterials can lead to a plethora of surfaceresonant states. We determine that negative effective-mass density is the necessary condition for the existenceof surface states on acoustic metamaterials. We offer the microscopic picture of these unique surface states; inaddition, we find that these surface excitations enhance the transmission of evanescent pressure fields acrossthe metamaterial. The evanescent pressure fields scattered from an object can be resonantly coupled andenhanced at the surface of the acoustic metamaterial, resulting in an image with resolution below the diffrac-tion limit. This concept of acoustic superlens opens exciting opportunities to design acoustic metamaterials forultrasonic imaging.

    DOI: 10.1103/PhysRevB.75.195447 PACS numbers: 43.20.g, 43.35.d, 46.40.Ff

    I. INTRODUCTION

    Advances in electromagnetic metamaterials1,2 offer excel-lent opportunities to realize new and exotic phenomena, suchas negative refraction3 and artificial magnetism.4,5 Its acous-tic counterpart with negative material properties has beenrecently explored.69 Acoustic metamaterials with locallyresonant elements can be designed to display anomalous re-sponse at selected frequencies so that effective dynamic ma-terial properties can be negative. It should be noted that theeffective negative properties of the metamaterials are dy-namic and highly dispersive. Such acoustic metamaterialsoffer a possible route to the realization of intriguing phenom-ena; negative refraction was reported earlier in double nega-tive acoustic metamaterials.8

    Recent work on phononic crystalsperiodic modulationof density and modulusalso showed that negative refrac-tion and focusing of acoustic waves1012 can be obtainedfrom band-folding effects due to Bragg scattering. Phononiccrystals require that the spatial modulation of impedance isof the same order as the acoustic wavelength.1319 Metama-terials provide a major step toward an effective-medium de-scription, as the spatial periodic modulation of impedance ismuch smaller than the wavelength. Acoustic metamaterials,also referred as sonic crystals, have been considered as spec-tral gap materials6,2022 and refractory acoustic devices.23,24Metamaterials broaden the range of material responses foundin nature, which can be especially useful in realizing newphenomena and in designing novel devices. Yet to the best ofour knowledge, there has been very limited investigation inthis direction. In this paper, we report a surface resonance onan acoustic metamaterial and examine its unique character-istics. As a result of this surface resonance, we propose andnumerically demonstrate an acoustic superlensanalogousto Pendrys perfect lens25for sub-diffraction-limited acous-tic imaging.

    II. SURFACE STATES ON ANACOUSTIC METAMATERIAL

    We consider a plane harmonic longitudinal wave analysisat a boundary between a fluid half-space and an acoustic

    metamaterial half-space Fig. 1a. Medium I is consideredas a fluid, with positive mass density and bulk modulus,whereas medium II is taken as an acoustic metamaterial. In ahomogeneous medium with mass density and bulk modu-lus B, the equilibrium equation and mass continuity equationare written in the index notation to relate the pressure P andvelocity field vi at any given point,

    kiP vi = 0, kivi PB

    = 0, 1

    where ki and are the wave vector and angular frequency ofthe plane wave.

    Let us consider the necessary and sufficient conditionsthat allow the existence of surface states at the interface be-tween a fluid and an acoustic metamaterial, the latter beingmodeled as a structured isotropic fluid. Structured fluid con-sists of the same fluid as medium I as the matrix with acous-tic resonators in it. The surface states represent elastic per-turbations with pressuremaximum at the interface andexponentially decaying in the direction perpendicular to theinterfaceschematically shown in Fig. 1a. By matchingpressure and normal velocity fields at the interface z=0, weobtain the relation between the normal components of wavevectors:

    kzI

    I+

    kzII

    II= 0. 2

    The necessary condition for a bound state to exist at theinterface requires that both kzs have positive imaginaryparts, which implies that the mass density of the acousticmetamaterial should be negative II0. Negative densityimplies that the response of fluidaccelerationis out ofphase with the dynamic pressure gradient, and it is obtainedwhen such negative responses of the oscillators constitutingthe acoustic metamaterial dominate the background. The dy-namic effective-mass density of the metamaterials can besignificantly different from the volume averaged massdensity,26,27 as the multiple scattering is treated in an averagesense.26 Negative effective-mass density is reported for fluid-solid composites, e.g., soft rubber spheres in water.8 In gen-eral, acoustic metamaterial can be modeled as a set of har-

    PHYSICAL REVIEW B 75, 195447 2007

    1098-0121/2007/7519/1954475 2007 The American Physical Society195447-1

  • monic oscillators. Here, surface resonance corresponds to theoscillation of harmonic oscillators such that there is constantslipping at the interface. Given effective negative mass den-sity, the slip arises due to the difference in tangential veloci-ties that changes the direction across the interface. By calcu-lating the components of the velocities along the y and z axesby Eq. 1, we obtain that the velocity components areshifted in phase by /2. Therefore, the trajectories of theparticle motions are ellipses with major axes parallel to theinterface, and the elliptical rotation of the particles near theinterface remains the same in both the media Fig. 1a. Incontrast to this surface state, the particle trajectories in theRayleigh wave are elliptical with major axis perpendicular tothe interface and the rotation changing with depth. In addi-tion, the pattern of the displacements in the unique surfacestate is illustrated Fig. 1b.

    III. DISPERSION RELATION OF THE SURFACE STATES

    We derive the surface-state dispersion between the angu-lar frequency of the surface states and the wave vector kyby combining Eq. 2 with the dispersion relations of mediaI and II, ky

    2I,II+ kz2I,II=2 /BI,II, The tangential wave

    vector ky is required to be continuous across the interface,resulting in the dispersion relation of surface states,

    ky2

    = 2III

    II2 I2IIBI

    I

    BII . 3In addition to the necessary condition II0, surfacebound states require that ky

    2k02=2I /BI. This inequality

    and Eq. 3 are used to determine the conditions on the prop-erties of acoustic metamaterial that support the surface states.In the case III, the bulk modulus of the acousticmetamaterial should be either positive, BII0, or negativesatisfying the inequality BIIIIBI /I. On the other hand, forthe case III, the bulk modulus of the acoustic metama-terial should be negative and BIIIIBI /I.

    We find that when the bulk moduli of two media are thesame B, the dispersion relation of surface states reduces to

    ky2

    =

    2

    B III

    I + II . 4

    Similar to the surface-plasmon resonance in electromagnet-ics, negative mass density in acoustic metamaterials signifi-cantly broadens the surface resonant band of ky in the limitof II I. This broadening is represented by the flatdispersion curve that is wave vector independent Fig. 2.The bulk modulus of both the media is taken to be the same,BII=BI. The effective-mass density of medium IIa struc-tured fluidis taken in Lorentz form.7 Linear-response func-tions such as mass density take the Lorentz form 1/ o

    2

    2, in the case where a wave of angular frequency in-teracts with a medium consisting of localized resonator withresonant frequency o.6 Here, we consider only the fre-quency interval in which the surface state exists: effective-mass density of medium II is negative and greater in magni-tude than medium I, II0 and III. Dispersioncurve for the surface resonance is shown in red, and thelinear dispersion curve of medium I is shown in blue. It isevident that the wave vector of the surface wave is alwaysgreater than that of the bulk wave in medium I.

    IV. CHARACTERISTICS OF THE SURFACE STATES

    We consider a thin slab of acoustic metamaterial whoseeffective-mass density is negative in the near field of an ob-ject. We find that the evanescent pressure fields, scatteredfrom the object, can be resonantly coupled onto the surfacestates and transmitted through the slab with enhanced ampli-tude. Evanescent pressure fields are in which the pressureand velocity fluctuations are shifted in phase by /2, andthey exist in near field decaying exponentially away from theobject. Transmission enhancement is due to the bound stateson the surface acting as an energy reservoir, wherein thesurface states take energy from the source and enhance the

    FIG. 1. Color online. Schematic of the surface state at aninterface separating two semi-infinite media. Medium I is consid-ered to have positive material properties mass density and bulkmodulus B, whereas medium II is taken as an acoustic metamate-rial with generic material properties. All the physical quantities per-taining to the medium are designated by the respective mediumsuperscript. a Schematic of the pressure profile of surface boundstates; it is maximum at the interface and decaying exponentiallyperpendicular to the interface. The motion trajectory of the materialpoints is an ellipse; the elliptical rotation of the particles near theinterface is the same in both media shown clockwise. The eccen-tricity of the ellipses depends on the wave vector of the surface statewith major axes parallel to the interface. b The pattern of thedisplacements of the surface wave is illustrated top view. Theschematic shows that the displacements in y and z directions are 90out of phase, with slipping at the interface.

    AMBATI et al. PHYSICAL REVIEW B 75, 195447 2007

    195447-2

  • amplitude of evanescent waves. The degree of enhancementacross a finite slab of acoustic metamaterial depends on thethickness of acoustic metamaterial, which, in turn, deter-mines the resonant coupling of surface states at the two in-terfaces.

    Given an acoustic metamaterial II of finite thickness dplaced in a medium I, the overall transmission coefficientTratio of pressure fieldsacross the acoustic metamaterialcan be computed by taking account of multiple scatteringevents similar to the electromagnetic case.25

    Tky,d =tt expikz

    IId1 + rr expi2kz

    IId, 5

    where

    r =

    kzI

    I

    kzII

    II

    kzI

    I+

    kzII

    II

    , r = r, t = 1 + r, t = 1 + r.

    t and t are the pressure transmission coefficients at the in-terface of I / II and II/ I, respectively. Similarly, r and r arethe corresponding pressure reflection coefficients. The expo-nential growth of overall transmission for evanescent pres-sure fields is valid when rr1. This inequality implies adiverging reflectivity on either surface, that is, kz

    I /I+kzII /II

    0, which is exactly the condition we obtain for surfaceresonance in Eq. 2. Figure 3 displays the overall transmis-

    sion of a wide range of wave vectors across the acousticmetamaterial of different thicknesses. It clearly demonstratesthe enhancement of evanescent waves ky /k01, a key fea-ture of the surface resonance. However, there is no exponen-tial growth in the case of nonzero losses. In these calcula-tions, we consider acoustic metamaterialmedium IItohave complex effective-mass density with negative real partand positive imaginary part.7 The positive imaginary part ofeffective-mass density corresponds to the loss in the metama-terial, which is a dynamic average of various microscopicrelaxation phenomenaleading to bulk viscosityin theconstituent materials of the metamaterial. The demonstratedenhancement of evanescent waves in acoustic metamaterialFig. 3 gives rise to the possibility of restoring the amplitudeof the wide range of evanescent components, and thus lead-ing to sub-diffraction-limited imaging, i.e., superlensing.

    V. ACOUSTIC SUPERLENS

    We propose a perfect acoustic lens analogous to Pendrysperfect lens25 in two different ways. The first prospect is anacoustic metamaterial whose effective material propertiesmass density and bulk modulusare simultaneously nega-tive and perfectly matched, impedancewise, to the surround-ing medium. The second one is an acoustic metamaterial thathas negative mass density and positive bulk moduluswhich are equal in magnitude to those of the surroundingmediumwith thickness smaller than the acoustic wave-

    FIG. 2. Color online Dispersion curve of the surface state atthe interface between two semi-infinite media with mass densitiesof opposite signs. The effective-mass density of the medium IIanacoustic metamaterialis taken in Lorentz form, and the frequencyinterval is considered in which the surface states exist, II0and III. The bulk modulus of both media is taken to besame, BII=BI. Dispersion curve for the surface resonance is shownin, and it is clear that in the limit of III, the dispersioncurve asymptotically reaches infinity. Also, the linear dispersioncurve of medium I is shown in blue. The vertical lines in the figuredepict the x intercepts wave vectors at a given frequency, and it isclear that the wave vector of the surface wave is always greater thanthat of the bulk wave in medium I.

    0 2 4 6 8 10 120

    4

    8

    12

    16

    20

    TransmissionCoefficient

    Wave Vector

    d = /4d = /5d = /6

    ky/k0

    ()

    ,y

    Tkd

    FIG. 3. Color online. Enhanced transmission of evanescentpressure waves across an acoustic metamaterial, a slab of negativeeffective-mass density. Different thicknesses d of the acousticmetamaterials are considered, and in each case the effective-massdensity of the acoustic metamaterial is taken as II= 1+0.01iI.The bulk modulus is assumed to be same as that of the surroundingmedium, BII=BI. Tky ,d is the ratio of amplitude of pressurefields across the metamaterial. Enhanced transmittivitythe wave-vector range over which the evanescent waves are transmitted withincreased amplitudeis a strong function of the thickness of theslab d, as the thickness determines the coupling of surface statesat the two interfaces.

    SURFACE RESONANT STATES AND SUPERLENSING IN PHYSICAL REVIEW B 75, 195447 2007

    195447-3

  • length. We find that in the quasistatic limit, the dependenceon modulus is eliminated and only mass densities are rel-evant for pressure fields. We consider such an acousticmetamaterial slab with effective negative mass density as asuperlens in acoustics, which offers highly localized surfaceacoustic waves over a broad evanescent wave-vector spec-trum. However, the loss in the acoustic metamaterial and theunit-cell dimensions of metamaterial impose practical limita-tions on imaging resolution. The loss in acoustic metamate-rial depends on the structure of metamaterial, the losses inthe constituent materials of metamaterial, and the frequencyof operation. In addition to the loss in acoustic metamaterial,the unit-cell dimensions of the acoustic metamaterial a af-fects the resolution. This limitation occurs as the evanescentwaves of large lateral wave vector ky interact with the inho-mogeneity of the acoustic metamaterials, and the averageover the metamaterialeffective medium descriptiondoesnot hold for evanescent waves whose ky is comparable to2 /a.

    We use numerical simulations to demonstrate the acousticsuperlens effect with a thin slab of lossy homogenized ma-

    terial of positive bulk modulus and negative mass density.The wave equation, 1/P2P /c2=0, is solvedin computational domain displayed in Fig. 4a usingFEMLAB,28 where c is the speed of acoustic wave. Twosources width /20, separated by a distance of /4, emanat-ing from waveguides are taken as the object. The boundaryconditions are as follows: the walls of the waveguides arerigid and pressure waves are only interacting with the sur-rounding medium at the exit. In addition, the boundaries ofthe computational domain are taken as nonreflecting. Pres-sure field distribution in the presence of the slab of negativemass density, thickness /5, is plotted in Fig. 4a. It isclearly evident that the presence of the slab offers enoughcontrast to resolve the two sources. Since the image is pri-marily formed by evanescent waves, there is no fixed focalplane. The best contrast is at the interface between media IIand I; therefore, it is considered as the image plane. Theresolving power of the slabacting as an acousticsuperlensis obtained from the transfer function, ratio of theimage pressure fields to object pressure fields. It is calculatedfrom Eq. 5, accounting for the additional decay from the

    FIG. 4. Color online Acoustic superlensing with a slab of effective negative mass density. a The configuration considered is asfollows: a= /4, d= /5, u= /20, and II= 1+0.01iI. A slab of negative mass density of thickness d is placed in medium I. Two sourcesseparated by a are placed at a distance u from the slab. The pressure field amplitude distribution after finite element analysis shown at theright resolves the two sources. b The transfer functionthe modulus of image pressure field normalized by object pressure field inwave-vector spaceshows that the evanescent waves in the interval 1.3k0 ,4.8k0 are enhanced. Image plane is taken at the interfaceseparating media II and I. c The amplitude of evanescent pressure field ky =2k0 normalized to the amplitude in object plane clearly showsthe enhancement with local maximum at each of the interfaces red. The blue line is the control without the superlens, which shows anexponential decay of the amplitude of the evanescent pressure field. The abscissa is the z coordinate normalized to the wavelength. d Thepressure field amplitude in the image plane with red and without blue the acoustic superlens. The presence of acoustic superlens offersenough contrast to resolve the object.

    AMBATI et al. PHYSICAL REVIEW B 75, 195447 2007

    195447-4

  • object to the lens. Figure 4b illustrates that a range of eva-nescent waves in the interval 1.3k0 ,4.8k0 can be enhancedand recovered in the image plane. Figure 4c shows theenhancement of an evanescent pressure wave ky =2k0coupled to the surface bound states. Calculations show thatthere is a local maximum on the surfaces of the slab and anet enhancement from the object plane to the image plane. InFig. 4d, we plot the pressure amplitude distribution in theimage planetransfer function Tu ,ky ,d convoluted withobject wave-vector spectrumwith and without the slab ofnegative mass density. Negative mass density slab offershigh contrast at the image plane by enhancing the evanescentpressure fieldsthat carry finer details of the objectand atthe same time damping the propagating pressure fields. It isnumerically demonstrated that a flat slab of negative massdensity can be used as an acoustic lens for subwavelengthimaging. Such a slab of material acts as a superlens whichcan overcome the limitation of traditional lens performance.In contrast to the superlens discussed, there exists a modewhere the Lamb wavescoupled Rayleigh surface wavesare highly localized.29 The coupled wave-vector spectrumwith Lamb waves at this frequency provides an improved

    signal-to-noise ratio but does not overlap with evanescentwave-vector spectrum, and hence there is no super-resolution.

    VI. CONCLUSIONS

    In conclusion, we propose a different surface resonancephenomenon in acoustics. Unlike in electromagnetics, wherenegative permittivity and permeability control P and S polar-ized surface states, respectively, it is proved here that onlynegative mass density is necessary for the surface resonancein acoustics. These surface resonant states and superlensingare likely to stimulate research in the design of acousticmetamaterials and devices.

    ACKNOWLEDGMENTS

    Financial support from the ONR Grant No.N000140710626 and ONR/DARPA Multidisciplinary Uni-versity Research Initiative MURI Grant No. N00014-01-1-0803 is acknowledged. The authors also acknowledgehelpful discussions with J. Sau and D. K. Gramotnev.

    *Author to whom correspondence should be addressed. Email ad-dress: [email protected]

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