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Nucleate Boiling Heat Transfer Enhancement with Electrowetting

AritraSur,YiLu,CarmenPascentePaulRuchhoeftandDongLiu

UniversityofHouston,Houston,TX77204USA

Outline q  Introduction q  Electrowetting q  Experimental design and measurements q  Electrowetting modulated nucleate boiling q  Conclusions

2

Introduction

3

q  Nucleate boiling – liquid-vapor phase change

o  One of the most efficient modes of heat transfer

ü  Transfers enormous amount of heat with small driving temperature difference

o  Widely applied in energy conversion, power generation and thermal management

o  Current limitations ü  Low boiling heat transfer coefficient (BHTC) ü  Highest critical heat flux (CHF) is only around 10% of

theoretical maximum ü  An increase in CHF by 30% alone will increase the power

density of pressurized water reactors by 20%

Boiling 101

4

Fig. 1 A typical boiling curve.Wall superheat ΔTsat = (Tw -Tsat)

Heat flux q’’

ΔTONB

CHF Film boiling

Single-phase

Transition boiling

ExcursionONB W

all h

eat f

lux

q”

q Goals for boiling heat transfer enhancement o  Onset of nucleate boiling (ONB) at low wall superheat o  Steeper boiling curve – high HTC o  Extremely high CHF

Wall superheat ΔTsat = (Tw -Tsat)

Hea

t flu

x q’

ΔTONB

CHF Film boiling

Single-phase

Transition boiling

Excursion

Wall superheat ΔTsat = (Tw -Tsat)

Hea

t flu

x q’

ΔTONB

Single-phase

Nuc

leat

e bo

iling

Fig. 1 Boiling curves: (a) a typical boiling curve; and (b) an ideal boilingcurve.

(a) (b)

Effects of Surface Wettability q  Surface wettability plays a critical role in nucleate boiling

o  Hydrophobic surfaces have lower energy barrier for nucleation and promotes ONB

o  High HTC depends on: nucleation site density, bubble departure size/frequency, and contact line motion, etc.

o  Higher CHF can be obtained if the surface remains wetted by liquid and the vapor phase boundary is restricted

q  A dilemma: On one hand, hydrophobicity promotes

ONB; on the other hand, hydrophilicity enhances CHF

5

6

Effects of Surface Wettability

Better boiling heat transfer!

CHF ONB ONB

CHF

Jo H. et al. 2011. IJHMT. ‘ A study of nucleate boiling on hydrophilic, hydrophobic and heterogeneous wetting surfaces

How can we harness the benefits of

both hydrophobicity and

hydrophilicity?

Current Enhancement Technology

7

q  Surfaces with hybrid wettability

q  Surfaces with hierarchical micro/nanoscale structures

8

Hybrid surface

Current Enhancement Technology

q  It is working! q  But …

o  Complicated to fabricate o  Multiple parameters

affecting boiling process o  Difficult to optimize o  Wettability

distribution fixed once fabricated

Can we actively control the

spatiotemporally dynamic boiling

process?

Outline q  Introduction q  Electrowetting q  Experimental design and measurements q  Electrowetting modulated nucleate boiling q  Conclusions

9

q  Electrowetting (EW): Modification of surface wettability with an applied electric field, also termed “electrowetting on dielectric” (EWOD)

q  EW is represented by the change of contact angle θ

o  Hydrophilic surface: θ < 90°

o  Hydrophobic surface: θ > 90° (Superhydrophobic: θ > 120°)

Electrowetting

Electrode Dielectric layer Teflon layer

Silicon substrate

EW of water droplet on Teflon-coated surface

10

θ0 θa

θ0 èθa

Electrowetting Theory

cosθa = cosθ0 +

ε0εd

2dσ LV

V 2

11

Contact angle saturation

Water on Teflon θ0 = 120° d = 1 µm d = 500 nm

θ0: inherent contact angle;

θa: apparent contact angle

ε0: permittivity in vacuum;

εd: relative permittivity

d: dielectric layer thickness;

V: applied voltage

σLV: liquid surface tension

where

q  EW theory was first developed by Gabriel Lippmann in 1875, known as the Young-Lippmann equation

q  DC electrowetting

q  AC electrowetting

Electrowetting - Droplets

12

P2 mode (V = 32 V, f = 28 Hz)

P4 mode (V = 32 V, f = 79 Hz)

Visualization Simulation

Electrowetting - Bubbles

13

Zhao Y. and Cho S.K., 2006, Lab Chip, “Micro air bubble manipulation by electrowetting on dielectric”

q  Contact angle variation is significant enough to reverse the surface wettability

q  Under AC EW, interfacial oscillation generates strong streaming flow around the bubble

Ko et al., 2009, App Phy Lett, “A synthetic jet produced by electrowetting-driven bubble oscillation in aqueous solutions”

It is possible to modulate/enhance

nucleate boiling with EW!

Outline q  Introduction q  Electrowetting q  Experimental design and measurements q  Electrowetting modulated nucleate boiling q  Conclusions

14

Experimental Setup

15

Test Device

16

n  Coating material: DuPont™ Teflon® (AF1600) dissolved in FC40 (2%)

n  Adhesion promoter: Fluorosyl™ FCL-52 in fluorosolvent FSM660-4 (0.4%)

n  Fabrication method o  Dip coat Fluorosyl solution

o  Spin coat Teflon

!

!!

!

Measurement Parameters q Optical imaging

o  Nucleate bubble dynamics o  Boiling regime identification

q  IR thermography o  Boiling surface wall temperature o  Heat flux

q Data acquisition o  Power supply to heater o  Liquid pool temperature

17

Synchronous

Wall Temperature and Heat Flux

18

IR Image

Wall temperature Heat flux

Electrowetting Signals

19

. . / 2r m sV a=

. .r m sV a=

. . / 3r m sV a=

2 2. .r m s DCV a V= +

a

a

a

0

0

0

0

with DC offset

a

VDC

a

- a

a

- a

a

- a

Time

Outline q  Introduction q  Electrowetting of droplets vs. bubbles q  Experimental design and measurements q  Electrowetting modulated nucleate boiling q  Conclusions

20

Onset of Nucleate Boiling

21

Hydrophobic Surface q” = 3.7 kW/m2

EW modulated (Vr.m.s = 78 V, f = 10 Hz)

q” = 6.8 kW/m2

Onset of Nucleate Boiling

22

q Change in bubble geometry o  Absence of vapor patch upon departure

q Delayed ONB o  Hydrophobic surface = 3.7 kW/m2

o  EW modulated = 6.8 kW/m2

q Shorter bubble departure time o  Hydrophobic surface = 1.5 sec o  EW modulated = 430.25 ms

q Decreased bubble footprint size o  Hydrophobic surface, radius = 3 mm o  EW modulated, radius = 2.75 mm

q Reduced contact angle o  Hydrophobic surface ~ 104 – 118 ° o  EW modulated ~ 80 °

Hydrophobic surface

EW modulation

0 200 400 600 800 1000 1200 1400 16000.0

0.5

1.0

1.5

2.0

2.5

3.0

3.5

Rad

iusofbubblefootp

rint(m

m)

T ime(ms )

Hydrophobic s urfac e

0 200 400 600 800 1000 1200 1400 1600100

102

104

106

108

110

112

114

116

118

120Hydrophobic s urfac e

Contactangle(Deg

rees

)

T ime(ms )

0 50 100 150 200 250 300 350 400 45040

50

60

70

80

90

100

110

120

Contactangle(Deg

rees

)

T ime(ms )

E Wmodulated(Vr.m.s .= 78V,f= 10Hz )

0 50 100 150 200 250 300 350 400 450 5000.0

0.5

1.0

1.5

2.0

2.5

3.0

3.5E Wmodulated (V

r.m.s .= 78V ,f= 10Hz )

Rad

iusofbubblefootp

rint(m

m)

T ime(ms )

100 ms

Fully-Developed Nucleate Boiling

23

Hydrophobic surface q” = 62.6 kW/m2

EW modulated q” = 62.6 kW/m2

Fully-Developed Nucleate Boiling

24

0.0 0.5 1.0 1.5 2.0 2.5 3.0 3.5 4.0 4.5 5.0104.5

105.0

105.5

106.0

106.5

107.0

107.5

108.0

Walltem

per

ature

(°C

)

T ime(s ec )

Hydrophobic s urfac eE Wmodulated(V

r.m.s= 78V,f= 10Hz )

0.0 0.5 1.0 1.5 2.0 2.5 3.0 3.5 4.0 4.5 5.0

398

400

402

404

406

408

410

412

414

416

Wallh

eatflux(kW

/m2 )

T ime(s ec )

Hydrophobic s urfac eE Wmodulated(V

r.m.s= 78V,f= 10Hz )

Average wall temperature Average boiling heat flux

q  Effect of AC EW

o  Decrease in average wall temperature by 1.5ºC

o  Increase in boiling heat flux by 10 kW/m2

Film Boiling to Nucleate Boiling Transition

25

Applied heat flux = 82 kW/m2

EW waveform applied

Wall Temperature Variation

26

0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0 2.2 2.4105

110

115

120

125

130

135

140

145

Tem

per

ature

(°C

)

T ime(s )

S patiallyaverag edwalltemperature

E W s ig na lapplied

0.74s ec

CHF Enhancement q  Wall heat flux = 86.9 kW/m2

q  EW effect on boiling regime o  Absence of vapor film o  Surface exposed to bulk fluid o  Delayed onset of film boiling o  Higher departure frequency o  Smaller departure size

q  EW effect on wall temperature o  Lower wall temperature

o  Hydrophobic surface > 200 °C o  EW modulated ~ 110 °C

o  Enhanced HTC o  Enhanced wall heat flux

27

Hydrophobic surface

EW modulation

EW-Enhanced Boiling Heat Transfer

Boiling curve Boiling heat transfer coefficient

q  Delayed onset of film boiling q  CHF is enhanced under the influence of EW q  Overall enhancement of boiling HTC

0 10 20 30 40 50 60 70 800

20

40

60

80

100

120

140

160

Wallh

eatflux(kW

/m2 )

Walls uperheat(°C )

Hydrophobic s urfac e

E W-modulated(Vr.m.s = 78V,f= 10Hz )

Onset of film boiling

28

0 20 40 60 80 100 120 140 160 180 2000

1

2

3

4

5

6

7

8

9

10

Boilinghea

ttran

sfer

coefficien

t(kW

/m2 -K)

Wallheatflux (kW/m2)

Hydrophobic s urfac eE W-modulated(V

r.m.s= 78V,f= 10Hz )

Enhancement Mechanisms

q  Nucleate boiling regime o  Altering the bubble dynamics o  Enhancing microcovection in the liquid o  Re-creating the microlayer o  Augmenting the quenching heat transfer

q  Filmwise transition boiling o  Destabilizing the liquid-vapor interface

29

Conclusions q  We have demonstrated that the bubble dynamics can be

effectively controlled by EW and nucleate boiling heat transfer can be favorably improved over the entire range of boiling regimes.

q  We have developed experiments and are developing theoretical/numerical models to understand the physical mechanisms of EW-enhancement of nucleate boiling.

30

31

Acknowledgements q  Financial support from

o  National Science Foundation (NSF) o  University of Houston

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