center for electronic correlations and magnetism ... · 4/17/2013 · interaction between...
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Surprising effects of the interaction between electrons in solids
Dieter Vollhardt
Center for Electronic Correlations and Magnetism University of Augsburg
Inauguration Symposium of the Wolfgang Pauli Centre DESY Hamburg; April 17, 2013
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• “Physics of dirt” (Pauli)
• Peculiarities of quantum many-particle systems
• Electronic correlations in solids
• Dynamical Mean-Field Theory: Models vs. materials
• Developments & Perspectives
Outline:
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Example: Magnetite (Fe3O4)
Macroscopic view:
Solids
quantum many-particle problem
Microscopic view: O(1023) interacting electrons + ions
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• “Die Festkörperphysik ist eine Schmutzphysik” (Pauli) • “One shouldn‘t wallow in dirt” (Pauli to Peierls)
… but “dirt physics” can be fundamental and universal Fe3O4
T>TK (high energies) Asymptotically free local moment
) )( (1/ FJ N EK FT E e− Λ
T<TK (low energies) Screening of moment (confinement)
J
Prototypical interaction problem with “running coupling constant” J(Λ) QED, QCD
Magnetic impurity in a host of non-interacting (itinerant) electrons
“Kondo effect”
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Peculiarities of Interacting Many-Particle Systems
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Interacting many-particle systems
Elementary (“bare”) particles + fundamental interactions effective (“quasi”) particles + effective interactions
↓ N →∞# particles
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1
2Spin = Fermion
Fermi-Dirac statistics
Fermi body/surface
⇓
Non-interacting electrons
⇓Pauli exclusion principle (Hamburg, 1925) N →∞
Ground state:
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Fermi gas: Ground state
kx
ky
kz
Fermi surface 22
2F FE km
=
0 0FermiFermi pressure3 2 0
5 5F FE E NE P EN V V
∂= ⇒ = − = >
∂
Incompressibility of ordinary matter due to Pauli principle + uncertainty relation
kF
Fermi sphere
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kx
ky
kz
Fermi gas: Excited state
Switch on repulsive interaction
k-eigenstates: infinite life time
Particle
Hole
Fermi sphere
Fermi surface
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Fermi liquid
kx
ky
kz
Well-defined k-states ("quasiparticles") with - finite life time - effective mass - effective interaction
(Quasi-) Particle
(Quasi-) Hole
Landau (1956/58)
1-1 correspondence between one-particle states (k,σ)
= elementary excitation
“Standard model of condensed matter physics“
Fermi sphere
Fermi surface
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Simple metals
Potassium
T2 (K2)
C/T
(mJ/
mol
e K2
)
CeCu2Si2, UBe13: very heavy quasiparticles:
Kondo impurity physics
"Heavy Fermions"
* 1000 m m≈
Steglich et al. (1979)
Stewart et al. (1983)
C/T
(mJ/
mol
e K2
) T2 (K2)
*m m≈
Result of elementary excitations
(quasiparticles)
0im *l V
T
mm
cT
γ→
= ∝
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Interacting many-particle systems
Q
e
r Qr
Coulomb potential
Vacuum
Elementary (“bare”) particles + fundamental interactions effective (“quasi”) particles + effective interactions
↓ N →∞# particles
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r /rQ e
rξ−
Effective Yukawa potential
Electron gas: Screening Simplest approximation: Thomas-Fermi
Q
e
Interacting many-particle systems
Elementary (“bare”) particles + fundamental interactions effective (“quasi”) particles + effective interactions
↓ N →∞# particles
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r
3 cos(2 )FQ k rr
Friedel oscillations
Electron gas: Screening Better approximation: Lindhard
Q
e
Interacting many-particle systems
Elementary (“bare”) particles + fundamental interactions effective (“quasi”) particles + effective interactions
↓ N →∞# particles
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Electrons in real solids
“Strong effective interaction” of electrons in localized orbitals
Interacting many-particle systems
Hel
d (2
004)
Q
e
r
Elementary (“bare”) particles + fundamental interactions effective (“quasi”) particles + effective interactions
↓ N →∞# particles
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Entirely new phenomena, e.g., phase transitions
Interacting many-particle systems
↓Unpredicted behavior “emerges”
↓ N →∞# particles
We used to think that if we knew one, we knew two, because one and one are two. We are finding out that we must learn a great deal more about 'and'. Eddington (1882-1944)
“More is different” Anderson (1972)
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Entirely new phenomena, e.g., phase transitions
Interacting many-particle systems
↓Unpredicted behavior “emerges”
↓ N →∞# particles
Examples: Superconductivity Magnetism Metal-insulator transition
Traffic Weather Stock market
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Entirely new phenomena, e.g., phase transitions
Interacting many-particle systems
↓ N →∞# particles
Metal-insulator transition
Fe3O4
Electrons interact by strong effective repulsion
Why?
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Correlations
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Correlations in mathematics, natural sciences:
AB A B≠
2( ) ( ') ( ) ( ')n n n n n≠ =r r r r
e.g., densities:
The Fermi gas (1,..., )Nψ = A1
( )i
N
iiνψ
=∏ is uncorrelated,
but is spatially correlated due to the Fermi statistics (“Pauli hole”)
Correlations (I): Effects beyond factorization approximations (e.g., Hartree-Fock)
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Time/space average insufficient
Temporal/spatial correlations in everyday life
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Electronic Correlations in Solids
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Narrow d,f-orbitals/bands strong electronic correlations
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Correlated electron materials have unusual properties
} How to study correlated systems theoretically?
• sensors, switches, Mottronics • spintronics • thermoelectrics • high-Tc superconductors
With potential for technological applications:
• functional materials: oxide heterostructures …
•huge resistivity changes •gigantic volume anomalies •colossal magnetoresistance •high-Tc superconductivity •metallic behavior at interfaces of insulators
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material realistic model Þ modeling
“The fundamental laws necessary for the mathematical treatment of a large part of physics and the whole of chemistry are thus completely known, and the difficulty lies only in the fact that application of these laws leads to equations that are too complex to be solved.” Dirac (1929)
quantum many-particle problem
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material realistic model Þ modeling
maximal reduction: Hubbard model Þ U
time
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†
, ,σ σ
σ↑ ↓= +− ∑ ∑H c c n nt Ui j i i
i j i
Hubbard model Gutzwiller, 1963 Hubbard, 1963 Kanamori, 1963
time
Dimension of Hilbert space L: # lattice sites
Computational time for N2 molecule: ca. 1 year with 50.000 compute nodes
n n n n↑ ↓ ↑ ↓≠i i i i
Static (Hartree-Fock-type) mean-field theories generally insufficient
(4 )LO
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†
, ,σ σ
σ↑ ↓= +− ∑ ∑H c c n nt Ui j i i
i j i
Theoretical challenge of many-fermion problems: Construct reliable, comprehensive non-perturbative approximation schemes
Hubbard model Gutzwiller, 1963 Hubbard, 1963 Kanamori, 1963
time
n n n n↑ ↓ ↑ ↓≠i i i i
Static (Hartree-Fock-type) mean-field theories generally insufficient
Purely numerical approaches (d=2,3): hopeless
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Dynamical Mean-Field Theory (DMFT) of Correlated Electrons
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Metzner, Vollhardt (1989)
,d Z→∞→
Z=12
time
dynamical mean-field
Theory of correlated electrons
Hubbard model
Face-centered cubic lattice (d=3)
Georges, Kotliar (1992))
Self-consistent single-impurity Anderson model
†
, ,σ σ
σ↑ ↓= +− ∑ ∑H c c n nt Ui j i i
i j i
Strong simplifications
Solve with an „impurity solver“, e.g., QMC, NRG, ED,...
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Exact time resolved treatment of local electronic interactions
Dynamical mean-field theory (DMFT) of correlated electrons
U
U
Spec
tral
fun
ctio
n
Experimentally detectable ?
Correlations (II): Transfer of spectral weight
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Correlated Electron Materials
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Hel
d (2
004)
Electronic correlations
Many-body theory
: unrealistic
Material-specific input Density functional theory
(LDA/GGA) or GW
time
Comprehensive, non-perturbative approximation scheme needed
?
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: unrealistic
Hel
d (2
004)
Electronic correlations
Many-body theory (DMFT)
Material-specific input Density functional theory
(LDA/GGA) or GW
time
LDA+DMFT
+ ⇓
Anisimov et al. (1997) Lichtenstein, Katsnelson (1998)
Comprehensive, non-perturbative approximation scheme needed
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Application of LDA+DMFT
(Sr,Ca)VO3: 3d1 system
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Theory Electronic structure
180V VO∠ − − = °
162V VO∠ − − ≈ °
No correlation effects/spectral transfer
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LDA+DMFT results
k-in
tegr
ated
spe
ctra
l fun
ctio
n
constrained LDA: U=5.55 eV, J=1.0 eV
CaVO3
Osaka – Augsburg – Ekaterinburg collaboration: Sekiyama et al. (2004)
/
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3-peak structure detected
Osaka – Augsburg – Ekaterinburg collaboration, (2004, 2005)
Bulk sensitive photoemission spectroscopy
occupied states
Comparison with experiment
X-ray absorption spectroscopy unoccupied states
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GGA+DMFT phonon dispersion at 1.2 TC
Lattice dynamics of paramagnetic bcc iron Leonov et al. (2012)
Exp.: Neuhaus, Petry, Krimmel (1997)
State-of-the-art LDA+DMFT: Correlation-induced structural transformations
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Phase diagram of light actinide series
Tem
pera
ture
(0 C
) Explain and predict properties of complex correlated materials
Perspective of the LDA+DMFT approach
Phase diagram connecting individual binary alloy diagrams Black: two-phase regions; Brown : details unknown
Boring, Smith (2000)
Ac Th Pa U Np Pu Am Cm
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Developments & Perspectives
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Real-time evolution of correlation phenomena, e.g., time-resolved photoemission spectroscopy
Required: Theory of non-equilibrium in correlated bulk materials
1. Correlated electrons in non-equilibrium
Perfetti et al. (2006)
±∞
metal insulator
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Freericks, Turkowski (2006)
Eckstein, Kollar, Werner (2009) Quench in Hubbard model from U=0 to U>0
time after quench
Thermalization
Non-equilibrium DMFT
Momentum distribution (U=3.3)
Extension, e.g. • time resolved PES • pump-probe experiments
1. Correlated electrons in non-equilibrium
Eckstein (2009)
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Bosonic/fermionic atoms in optical lattices: Exp. realization of models
2. Correlated cold atoms in optical lattices
Observation of Fermi surface (40K atoms) Köhl, Esslinger (2006)
High degree of tunability: “quantum simulator”
Greiner et al. (2002)
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Jaksch et al. (1998) Hubbard model with ultracold atoms
Atomic total angular momentum Ltot = F N=2F+1 hyperfine states
2. Correlated cold atoms in optical lattices
SU(N) Hubbard models N=3, e.g. 6Li, U<0: Color superconductivity, “baryon formation (QCD)” Rapp et al. (2006)
Cooper pairs
“Baryons“
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Correlated many-particle systems: More fascinating than ever
±∞
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(L. Mathey) (M. Potthoff)
(M. Thorwart)
(D. Pfannkuche)
(M. Eckstein) (A. I. Lichtenstein)
(F. Lechermann)
•••
•
•••