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Theory of Domain-Wall Magnetoresistance in Metallic Antiferromagnets Jun-Hui Zheng, 1 Arne Brataas, 1 Mathias Kl¨ aui, 2, 1 and Alireza Qaiumzadeh 1 1 Center for Quantum Spintronics, Department of Physics, Norwegian University of Science and Technology, NO-7491 Trondheim, Norway 2 Institute for Physics, Johannes Gutenberg-University Mainz, 55128 Mainz, Germany (Dated: October 26, 2020) We develop a theory to compute the domain-wall magnetoresistance (DWMR) in antiferromag- netic (AFM) metals with different spin structures. In the diffusive transport regime, the DWMR can be either negative or positive depending on the domain-wall orientation and spin structure. In contrast, when the transport is in the ballistic regime, the DWMR is always positive, and the magnitude depends on the width and orientation of the domain wall. Our results pave the way of using electrical measurements for probing the internal spin structure in antiferromagnetic metals. I. INTRODUCTION Antiferromagnetic (AFM) materials are promising can- didates for next-generation spintronic nanodevices with advantages of low-power consumption, fast spin dynam- ics, and small size [1, 2]. In AFM memory devices, the data are stored in domains separated by domain walls (DWs) [3]. Highly efficient manipulation and accurate detection of AFM spin structures are essential for fur- ther developing the frontier of this field [1, 4]. The most extensively explored mechanisms for writing magnetic states in AFM metals so far are spin-transfer torques and spin-orbit torques [1, 4]. The magnetic state in a single domain can be electrically read out by measuring the anisotropic magnetoresistance (AMR) [5], the tun- neling magnetoresistance (MR) [6] in AFM spin valves, and the tunneling AMR [7, 8]. The comprehensive interplay between charge or spin currents and DWs brings diverse interesting phenomena and opens new opportunities for spintronic applications. The spin dynamics of DWs have been systemically stud- ied in the presence of charge and spin currents in both ferromagnetic (FM) and AFM systems [934]. These studies greatly enrich the methods of electrically manip- ulating the magnetic texture. Conversely, how itiner- ant electrons scatter off a DW conveys magnetic texture information. Charge and spin currents scattering from FM DWs [3545] and spin currents scattering from AFM DWs [3032, 46, 47] have also been explored extensively. Yet how charge currents are scattered by AFM DWs and the associated DWMR remain unexplored theoretically. Related studies could provide useful means for the detec- tion of AFM domain structures. In FM metals, a DW usually acts as an effective mag- netic barrier and increases the MR [3540]. Negative DWMR might appear in special cases when either the DW enhances the electron decoherence and reduces the weak localization in disordered systems [36] or the re- laxation time is spin dependent [48]. AFM metals, on the other hand, have more complex magnetic textures than FM metals [49]. Consequently, the AFM DWMR may exhibit more exotic properties [50]. Recently, an ex- perimental study on charge transport in the AFM metal FIG. 1. A-type, C-type, and G-type AFM structures. The black vectors show the direction of the charge current jx. In parallel (P) and staggered (S) configurations, spins are paral- lel and antiparallel for neighbors in the direction of current, respectively. The DW is perpendicular to the current direc- tion Mn 2 Au has reported a surprising AMR with the opposite sign to the typical AMR in FM systems and furthermore AFM DWMR signatures where found that are not under- stood on a theoretical level so far [51, 52]. This clearly calls for a study to fill the gap of a missing theory of AFM DWMR to complete the understanding of DWMR in systems with different magnetic orderings and symme- tries. In this paper, we formulate a framework to explore the DWMR in AFM metals in cubic lattices with A-type, C- type, or G-type AFM spin structure as shown in Fig. 1. Our formalism is general and can be used for other AFM lattices. Assuming that the DW is pinned, we investi- gate the charge transport in the direction perpendicular to the DW. The local magnetic moments of the neighbors in the charge current direction may be ordered in parallel (ferromagnetically) or in antiparallel (antiferromagneti- cally). We name these two configurations as parallel (P) and staggered (S) configuration, respectively, see Fig. 1. Assuming that the Fermi wavelength l F is much smaller than the DW width w, we treat the transport problem in the diffusive regime and the ballistic regime, separately. The two regimes correspond to different cases that the arXiv:2004.07154v2 [cond-mat.mes-hall] 23 Oct 2020

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Page 1: Domain-Wall Magnetoresistance in Antiferromagnetic Metals · 16/04/2020  · Domain-Wall Magnetoresistance in Antiferromagnetic Metals Jun-Hui Zheng, 1Arne Brataas, Mathias Kl aui,2,1

Theory of Domain-Wall Magnetoresistance in Metallic Antiferromagnets

Jun-Hui Zheng,1 Arne Brataas,1 Mathias Klaui,2, 1 and Alireza Qaiumzadeh1

1Center for Quantum Spintronics, Department of Physics,Norwegian University of Science and Technology, NO-7491 Trondheim, Norway

2Institute for Physics, Johannes Gutenberg-University Mainz, 55128 Mainz, Germany(Dated: October 26, 2020)

We develop a theory to compute the domain-wall magnetoresistance (DWMR) in antiferromag-netic (AFM) metals with different spin structures. In the diffusive transport regime, the DWMRcan be either negative or positive depending on the domain-wall orientation and spin structure.In contrast, when the transport is in the ballistic regime, the DWMR is always positive, and themagnitude depends on the width and orientation of the domain wall. Our results pave the way ofusing electrical measurements for probing the internal spin structure in antiferromagnetic metals.

I. INTRODUCTION

Antiferromagnetic (AFM) materials are promising can-didates for next-generation spintronic nanodevices withadvantages of low-power consumption, fast spin dynam-ics, and small size [1, 2]. In AFM memory devices, thedata are stored in domains separated by domain walls(DWs) [3]. Highly efficient manipulation and accuratedetection of AFM spin structures are essential for fur-ther developing the frontier of this field [1, 4]. The mostextensively explored mechanisms for writing magneticstates in AFM metals so far are spin-transfer torquesand spin-orbit torques [1, 4]. The magnetic state in asingle domain can be electrically read out by measuringthe anisotropic magnetoresistance (AMR) [5], the tun-neling magnetoresistance (MR) [6] in AFM spin valves,and the tunneling AMR [7, 8].

The comprehensive interplay between charge or spincurrents and DWs brings diverse interesting phenomenaand opens new opportunities for spintronic applications.The spin dynamics of DWs have been systemically stud-ied in the presence of charge and spin currents in bothferromagnetic (FM) and AFM systems [9–34]. Thesestudies greatly enrich the methods of electrically manip-ulating the magnetic texture. Conversely, how itiner-ant electrons scatter off a DW conveys magnetic textureinformation. Charge and spin currents scattering fromFM DWs [35–45] and spin currents scattering from AFMDWs [30–32, 46, 47] have also been explored extensively.Yet how charge currents are scattered by AFM DWs andthe associated DWMR remain unexplored theoretically.Related studies could provide useful means for the detec-tion of AFM domain structures.

In FM metals, a DW usually acts as an effective mag-netic barrier and increases the MR [35–40]. NegativeDWMR might appear in special cases when either theDW enhances the electron decoherence and reduces theweak localization in disordered systems [36] or the re-laxation time is spin dependent [48]. AFM metals, onthe other hand, have more complex magnetic texturesthan FM metals [49]. Consequently, the AFM DWMRmay exhibit more exotic properties [50]. Recently, an ex-perimental study on charge transport in the AFM metal

FIG. 1. A-type, C-type, and G-type AFM structures. Theblack vectors show the direction of the charge current jx. Inparallel (P) and staggered (S) configurations, spins are paral-lel and antiparallel for neighbors in the direction of current,respectively. The DW is perpendicular to the current direc-tion

Mn2Au has reported a surprising AMR with the oppositesign to the typical AMR in FM systems and furthermoreAFM DWMR signatures where found that are not under-stood on a theoretical level so far [51, 52]. This clearlycalls for a study to fill the gap of a missing theory ofAFM DWMR to complete the understanding of DWMRin systems with different magnetic orderings and symme-tries.

In this paper, we formulate a framework to explore theDWMR in AFM metals in cubic lattices with A-type, C-type, or G-type AFM spin structure as shown in Fig. 1.Our formalism is general and can be used for other AFMlattices. Assuming that the DW is pinned, we investi-gate the charge transport in the direction perpendicularto the DW. The local magnetic moments of the neighborsin the charge current direction may be ordered in parallel(ferromagnetically) or in antiparallel (antiferromagneti-cally). We name these two configurations as parallel (P)and staggered (S) configuration, respectively, see Fig. 1.Assuming that the Fermi wavelength lF is much smallerthan the DW width w, we treat the transport problem inthe diffusive regime and the ballistic regime, separately.The two regimes correspond to different cases that the

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FIG. 2. Domain-wall magnetoresistance (DWMR) Rw as afunction of DW width w. In P-configurations, the DWMRis positive. In S-configurations, it depends on the ratio be-tween the domain wall width and the mean free path of elec-trons lMFP. In the diffusive regime, the DWMR is negative inmost cases while in the ballistic regime the DWMR is positive.Here, lF is the Fermi wavevector.

mean free path of the itinerant electrons is significantlysmaller than the DW width, lMFP � w, and oppositelylMFP � w.

In Fig. 2, we schematically present our main result.We find that the DWMR is always positive in the P-configurations. In addition, its magnitude is proportionalto 1/w in the diffusive regime and 1/w2 in the ballisticregime. These behaviors are very similar to the DWMRin FM metals [40]. In contrast, the DWMR in the S-configurations strongly depends on ratio between the DWwidth and the mean free path as well as doping level. Inthis case, the DWMR is negative in the diffusive regimefor most doping levels. The DW promotes rather thanhinders the electron mobility. This is because the DWcan effectively suppress the magnetic staggering stiffnessand thus enhance the electron mobility. On the otherhand, in the ballistic regime, the DWMR becomes pos-itive. It is proportional to 1/w near-half filling (aboutone electron per cubic cell) and vanishes in the low filling.Consequently, the DWMR changes its sign when the DWwidth becomes comparable to the mean free path for theintermediate electron filling case in the S-configurations.

The rest of this paper is structured as follows. In Sec.II, we introduce the generic Hamiltonian and its symme-try. In Sec. III and IV, we develop the diffusive transporttheory and the ballistic transport theory separately andcalculate the DWMR. In Sec. V, we give a short conclu-sion.

II. HAMILTONIAN

We model the itinerant electrons in two-sublatticeAFM metals, containing antiferromagnetically coupled Aand B sublattices, with the following generic Hamiltonian

H = −Jn(x) · στz + h1(k)σ0τx + h2(k)σ0τ0, (1)

where k is the electron wavevector and J is the strengthof the s-d exchange interaction between the itinerant elec-trons and the staggered local magnetization n [1, 53].Without loss of generality, we consider a Neel-type DWperpendicular to the x axis. The local magnetization isparameterized as

n(x) = (sin θ cosφ, sin θ sinφ, cos θ), (2)

where φ is the azimuthal angle, which is a constant inNeel DWs, and θ is the polar angle, which depends onthe position along the x direction. The Pauli matrices τand σ act on the two-sublattice subspace and the spinsubspace, respectively. The structure factor

h1(k) = −t∑d

cos (k · d), (3)

describes inter-sublattice hopping between the antiferro-magnetically ordered nearest-neighbor (A-B sites) withconnection bonds d. The structure factor

h2(k) = −t∑b

cos (k · b), (4)

governs intra-sublattice hopping between ferromagneti-cally ordered nearest-neighbor (A-A or B-B sites) withconnection bonds b, if such hoppings exists, e.g., for theG-type AFM structure, this term is zero. The explicitform of h1 and h2 for each AFM spin structure is shownin Table I.

Since the Hamiltonian is spatially dependent along thex direction, we replace the wavevector k with the opera-

tor k = (−i∂x, ky, kz), where the components ky and kzremain good quantum numbers. Next, we apply a gaugetransformation

R(x) = exp

[− iφσz

2

]exp

[− iθ(x)σy

2

], (5)

which makes the exchange term spatially uniform [36],i.e.,

R−1[n(x) · σ]R = σz. (6)

Simultaneously, the operator −i∂x in the hopping termsh1 and h2 also becomes

R−1[−i∂x]R = −i∂x −λ(x)σy

2, (7)

where λ(x) = dθ/dx describes the spatial gradient of theDW texture. The DW now induces a non-Abelian gaugepotential λ(x)σy/2 inside the hopping terms, which van-ishes far from the DW. To make the matrix representa-tion of the Hamiltonian more elegant, we further applya global rotation transformation

T = exp

[− iσxπ

4

]exp

[− iτyπ

4

]. (8)

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TABLE I. Hamiltonian H and the spin-spiral spectrum Esζ

TypeH = −Jn · στz + h1(k)σ0τx + h2(k)σ0τ0

and spectrum Esζ with s, ζ = ±1

As

h1 = −2t cos kx

h2 = −2t(cos ky + cos kz)

Esζ = −2t cos ky − 2t cos kz

+ 2ζt sin λ2

sin kx + s√

4t2 cos2 λ2

cos2 kx + J2

Ap

h1 = −2t cos ky

h2 = −2t(cos kx + cos kz)

Esζ = −2t cos λ2

cos kx − 2t cos kz

+ s√

4t2(cos ky − ζ sin λ2

sin kx)2 + J2

Cs

h1 = −2t(cos kx + cos ky)

h2 = −2t cos kz

Esζ = −2t cos kz + 2ζt sin λ2

sin kx

+ s√

4t2[cos λ2

cos kx + cos ky]2 + J2

Cp

h1 = −2t(cos ky + cos kz)

h2 = −2t cos kx

Esζ = −2t cos λ2

cos kx

+ s√

4t2(cos ky + cos kz − ζ sin λ2

sin kx)2 + J2

Gs

h1 = −2t(cos kx + cos ky + cos kz)

h2 = 0

Esζ = 2ζt sin λ2

sin kx

+ s√

4t2[cos λ2

cos kx + cos ky + cos kz]2 + J2

Finally, the Hamiltonian in the rotated basis becomes

Hr = [R(x)T ]−1HR(x)T

= Jσyτx + h1(k +λσz

2ex)τz + h2(k +

λσz2ex),(9)

where ex = (1, 0, 0). As well as the charge conserva-tion, the rotated Hamiltonian has pseudospin conserva-tion, since [ζ,Hr] = 0, where ζ = σzτz is the pseudospinoperator. The matrix form of Hr is block diagonal. Thespin-spiral spectrum of Hr with a constant λ are shownin Table I.

In the following, we compute the DWMR in both diffu-sive and ballistic regimes using this rotated Hamiltonian.The lattice constant is set to be a = 1 for simplicity. Wewill assume that the DW texture is modelled by [30, 31]

cos θ = tanh(πxw

). (10)

Then, the gradient of the DW texture is maximum at theDW center, |λ|max = π/w.

III. DIFFUSIVE TRANSPORT THEORY

When the mean free path is significantly shorter thanthe DW width w, electrons move diffusively. Thecorresponding DWMR in FM systems has previouslybeen evaluated using perturbative quantum field theory

FIG. 3. The equivalent resistor circuit of an AFM system inthe diffusive regime.

[36, 40] and Boltzmann transport theory [37]. To circum-vent the complicated evaluation of Feynman diagrams inquantum field theory, we provide a new and consider-ably simpler method for computing the diffusive trans-port when the DW is wide w � lF and λ(x) varies slowly.

As shown in Fig. 3, we divide the system into a se-ries of small spin-spiral segments with length ∆xi. Eachsegmemt has a constant spin-spiral gradient λi = λ(xi),where xi is the center position of the i-th segment. Inthe diffusive regime, Ohm’s law applies. Since the pseu-dospin is conserved, the two pseudospin flavors ζ = ±1function as parallel resistor circuits. For each pseudospinflavor ζ, the resistance of a series resistor circuit is givenby the sum of resistances of infinitesimal resistor elements

Rζ =∑i

∆xiσζ(λi)S

=

∫ L/2

−L/2

dx

σζ(λ)S, (11)

where σζ(λi) is the conductivity of the i-th spin-spiralsegment with pseudospin ζ, L is the system length alongthe x-axis, and S is the cross-section. The total resistanceof the system R consists of the two pseudospin flavorsin parallel, 1/R = 1/R+ + 1/R−. The DWMR is thedifference between the total MR in the presence and inthe absence of a DW,

Rw = R−R0 ' −σ−20 S−1

∫ L/2

−L/2δσdx, (12)

where R0 = L/Sσ0 is the MR of a single AFM domain,

σ(λ) = σ+(λ) + σ−(λ) (13)

is the total conductivity in a spin-spiral segment, σ0 =σ(0), and δσ = σ(λ) − σ0. In Eq. (12), we have usedthat in a uniform domain σ+(0) = σ−(0). Now, theproblem of DWMR has been reduced to the calculationof the conductivity σζ(λ) in a spin-spiral segment. Notethat depending on specific materials, the system can havedifferent electron filling per cubic cell.

In a low-filling regime, where only the low energy statesare occupied, the chemical potential µ is close to the bandbottom at −6t. The low-energy eigenvalues of Hr for aspin-spiral segment with a constant λ becomes especiallysimple. From the spectrum shown in Table I, up to thesecond order in λ and kα, we find

E ' δE +(kx − kc)2

2m∗x+

k2y

2m∗y+

k2z

2m∗z+ const. (14)

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Here, the anisotropic effective mass of electrons is m∗α =gκ/2t

2 or 1/2t, when the spins are staggered or paral-lel for neighbors along the α axis. The numerator isdefined as gκ =

√t2 + J2/4κ2, where κ = 1, 2, 3 for

A-type, C-type, and G-type AFM structures, respec-tively. A finite spin-spiral gradient leads to a shift inthe momentum kc ∝ λ and the energy δE = Zκλ2/m∗x,where Zκ = J2/(32g2

κκ2) for P-configurations and Zκ =

−J2/(32t2κ2) for S-configurations respectively. Thespectrum (14) is similar to the sepectrum of a free elec-tron model and thus we can use the Drude formula forconductivity. The Drude conductivity along the x direc-tion is given by

σ(λ) = e2nτ/|m∗x|, (15)

where n = kxF kyF k

zF /3π

2 is the electron density, kαF isthe anisotropic Fermi wavevector, and τ is the electronlifetime. Using Eq. (12), we find that the relative changein the MR due to the DW becomes

RwR0

= 6πZκ ·(lxF )2

Lw, (16)

where lαF = 1/kαF is the anisotropic Fermi wavelength.Equation (16) shows that in P-configurations, Ap and

Cp cases, the DWMR is positive similar to FM systems.In contrast, in S-configurations, As, Cs, and Gs cases,the DWMR becomes negative, because the coefficientZκ is negative. The counter intuitive phenomena thatthese DWs reduce the MR, can be interpreted from theDrude’s formula. In S-configurations, since the energyshift induced by a spin-spiral is negative, the local elec-tron density and also the local conductivity inside theDW are enhanced. In other words, the DWs soften theeffects of the staggered field.

Next, we consider a general case with arbitrary elec-tron filling. Note that for a spin-spiral with a constantgradient λ, the momentum kx becomes a good quantumnumber in Hr. Using the Kubo formalism [54], we provethat the conductivity for each pseudospin becomes

σζ(λ) = e2τ∑s

∫BZ

d3k

(2π)3(vζsx )2δ(Esζ − µ), (17)

where vζsx = ∂Esζ/∂kx is the group velocity of electronsin the s-th band of pseudospin ζ. The relative DWMRcan be shown to be Rw/R0 ∝ 1/w. Technical detailscan be found in the Appendix. In the low-filling limit,Eq. (17) is consistent with the Drude conductivity (15).We can also rewrite the conductivity (17) as σζ(λ) =

e2τv2xρµζ , where ρζ(µ) is the density of states (DOS) and√

v2x is the average velocity along the x-direction at the

chemical potential µ for pseudospin ζ. This expressionclearly shows that the conductivity can be enhanced byincreasing either the DOS or the average velocity.

In Fig. 4-a), we plot the relative DWMR as a func-tion of chemical potential for a DW with λmax = 0.3/a.

FIG. 4. The relative DWMR Rw/R0 as a function of thechemical potential µ. The DW width is w ' 10.5a and we setJ = t. We show the results for negative chemical potential.The part with positive chemical potential is symmetric withthe negative part. Here, L is the length of the system and ais the lattice constant.

The DW width is w ' 10.5a. The result shows thatfor different chemical potentials, the DWMR usually isnegative in S-configurations and always is positive in P-configurationa. To understand this phenomena, in Fig. 5,we confirm that the ratios of the conductivity of uniform

domains (λ = 0) for different AFM types, σAs0 /σAp0 and

σCs0 /σCp0 , are significantly smaller than one. Since thesingle AFM domains of As-type and Ap-type, or Cs-typeand Cp-type, share a common DOS, the ratio less thanone means that the electron mobility (or the averagedvelocity) is suppressed in the direction that neighboringmagnetic moments are staggered. We interpret that inS-configurations a spin spiral can effectively suppress themagnetic staggering stiffness and thus enhances the elec-tron mobility. This explains the formation of negativeDWMR in S-configurations. In Fig. 4-a), we also find inseveral energy regions in S-configurations, the DWMRbecomes positive. These phenomena usually accompanywith significant suppression of DOS (corresponding tothe conducting channels) due to the spin spiral as shownin Fig. 6.

IV. BALLISTIC TRANSPORT THEORY

When the electron’s mean free path is much larger thanthe DW width, by using the Landauer approach, the con-

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FIG. 5. The ratio of diffusive conductivity in a single AFMdomain with S-configuration and P-configuration. The ratiois significantly less than one.

FIG. 6. Density of states (DOS) for As, Cs and Gs cases

ductance in the x-direction at zero temperature is

G = e2S∑ζs

∫ vζsx >0

BZ

d3k

(2π)3vζsx |λ=0Tζs,kxδ(E

sζ |λ=0 − µ),

(18)where Tζs,kx is the transmission coefficient for each chan-nel [55]. Since λ(x) varies slowly, the adiabatic approxi-mation can be applied. In other words, we can treat themotion of electrons classically by using Hamilton’s equa-tions, x = ∂kxE

sζ (λ(x), kx) and kx = −∂xEsζ (λ(x), kx).

The two variables ky and kz are hidden since they areconserved during the evolution. The transmission coeffi-cient becomes Tkx = 1 for open channels and Tkx = 0 forclosed channels. The DWMR is determined by how manychannels become closed due to the DW. Note that theelectrons’ motion follows the law of conservation of en-ergy. The DW, as an aisle, only allows injecting electronswithin the energy window

[min(Esζ ), max(Esζ )

]λ=λmax

for fixed ky and kz set by the DW to pass through. Tech-nically, for an injecting electron with E = Esζ (λ = 0, k0

x),

the channel is open if there is a solution of kx near to k0x

for the equation E = Esζ (λmax, kx).

In the low filling limit, using the low energy spectrum(14), we obtain the resistance of a single AFM domain,R0 = (4π2~/e2)(lyF l

zF /S). For all S-configurations, the

DWs are transparent and cause no additional resistance,since all low-energy channels are open due to the negativeenergy shift δE. However, for P-configurations, δE is

positive, we obtain the relative DWMR

RwR0

=(πlxF )2

w2· 2Zκ. (19)

The situation differs in the moderate filling case. Forinstance, in the As case, the local dispersion with gradi-ent λ is

E±ζ = −2t(cos ky + cos kz) + 2ζt sin(λ/2) sin kx

±√

4t2 cos2(λ/2) cos2 kx + J2. (20)

We rewrite the energy in the form

E±ζ (λ, kx) = E±ζ (λ = 0, kx) + Veff[λ(x), kx]. (21)

Different models can use a similar decomposition. Herewe find near kx = π/2 (which can not be occupied in thelow filling limit), the effective potential Veff ∼ ±2tλ(x)/2for a small λ. This quantity tunes the energy windowin the DW. In S-configurations, the leading order of tun-ing the window is ∝ λmax and thus δRr ∝ 1/w. Similardiscussion works for P-configurations. However, the lead-ing order of tuning the window becomes proportional toλ2

max, resulting in δRr ∝ 1/w2 as the low-filling case.In Fig. 4-b), we plot the relative DWMR for a 180◦

DW with λmax = 0.3/a. We see in S-configurations itvanishes for a low filling case, but becomes significantlylarger than that in P-configurations in a moderate fillingcase.

V. CONCLUDING REMARKS

We have developed a formalism to compute the MRfrom magnetic textures in AFM metals in diffusive andballistic regimes. In AFM systems, the DWMR exhibitsa more complex behavior as compared to FMs. TheAFM DWMR can be negative in the diffusive regimeeven in the absence of spin-dependent relaxation timeand spin-orbit couplings, which contrasts the FM case.This unique feature arises because DWs soften the effectsof the staggered magnetic moments in AFM metals.

Our results stimulate further DWMR measurementsto reveal the properties of AFM metals. In the diffu-sive regime, since the sign of DWMR is sensitive to spinconfigurations, measuring the MR provides informationon the configuration along the current direction. Thequalitative dependence of the DWMR on DW proper-ties is measurable by varying the DW width through me-chanical strains or magnetic fields in conjunction withmagnetic imaging using X-ray magnetic linear dichroismcontrast [46, 51].

ACKNOWLEDGMENTS

The authors thank O. Gomonay and M. Jourdan fordiscussions. This work was supported by the European

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Research Council via an Advanced Grant (no. 669442“Insulatronics”), the Research Council of Norwaythrough its Centres of Excellence funding scheme (projectno. 262633, “QuSpin”), the Norwegian Financial Mech-anism 2014-2021 (Project No. 2019/34/H/ST3/00515,“2Dtronics”), and the German Research Foundation(SFB TRR 173 Spin+X, projects A01 and B02).

Appendix A: Charge conductivity in the spin-spiralsegment

The pseudospin ζ is a conserved in our systems. Be-low we focus on each subspace with ζ = ±1. For thesimplicity of notation, we hide the index ζ in the follow-ing. For a spin-spiral segment with a constant gradientλ, the momentum kx in the rotated Hamiltonian Hr be-comes a good quantum number. Correspondingly, the

current operator in the rotated basis (c†k,s) is

jx =∑k,s,s′

c†k,sJss′(k)ck,s′ , (A1)

where J (k) = ∂kxHr(k) and s represents the internaldegree of freedom besides the pseudospin ζ.

Next, we introduce a unitary transformation Uk to

diagonalize the Hamiltonian, Hr(k) = U†kΛkUk, whereΛk = diag{E+(k), E−(k)} is a diagonal matrix. In the

eigenbasis of the Hamiltonian, dk = Ukck, the currentoperator becomes

jx =∑k,s,s′

d†k,sJk;ss′ dk,s′ , (A2)

where Jk = UkJ (k)U†k.The conductivity in the Kubo formalism is [54]

σ = limω→0

{ Im[π(iωn → ω + iδ)]

ω

}, (A3)

where the current-current correlation is

π(iωn) =1

V

∫ β

0

dteiωnt〈Ttjx(t)jx(0)〉

=1

β

∑p

∫d3k

(2π)3Tr[JkGk(ip+ iω)JkGk(ip)

].

(A4)

The single particle Green’s function Gk(ip) is a diagonalmatrix. In the Lehmann representation, we have

Gk;s,s′(ipn) = δs,s′

∫dε

As(k, ε)

ipn − ε+ µ, (A5)

where the spectral density is

As(k, ε) =2∆k

(Es − ε)2 + ∆2k

. (A6)

In above, s = ±, ∆k = 1/2τk, where τk is the lifetime ofthe quasiparticle.

Using these formula and using the same techniques de-veloped in Section 8.1 of Mahan’s book [54], we can di-rectly obtain the conductivity,

σ =∑s,s′

∫d3k

(2π)3

4πJk;s,s′Jk;s′,sAs(k, ε)As′(k, ε)δ(ε−µ).

(A7)Note that for a large τk (i.e., a small ∆k), we have

As(k, ε)As′(k, ε) ' 4πδ(ε− Es)τk, (A8)

when Es = Es′

[54], and

As(k, ε)As′(k, ε) = 0, (A9)

when Es 6= Es′. On the other hand, using the fact that

Jk = UkJ (k)U†k = Uk[∂kx(U†kΛkUk)]U†k, (A10)

we obtain

Jk = Uk(∂kxU†k)Λk + ∂kxΛk + Λk(∂kxUk)U†k. (A11)

Thus, for Es = Es′, we have

Jk,s,s′ = [Uk(∂kxU†k) + (∂kxUk)U†k]s,s′E

s′

k + δs,s′∂kxEs′

k

= δs,s′∂kxEsk. (A12)

We further assume that τk = τ and finally obtain

σ = e2τ∑s

∫d3k

(2π)3(vsx)2δ(Es − µ), (A13)

where vsx = ∂kxEsk. We have added the factor e2, which

is set to 1 in the above derivation.By expanding Eq. (A13) as a function of the gradient

λ, the correction from spin-spiral is of the order of λ2.The relative DWMR becomes

RwR0

=πCdiffuse

Lw, (A14)

where

Cdiffuse = −e2τ

σ0

∑ζ,s

∫BZ

d3k

(2π)3F2[Esζ ]δ(Esζ |λ=0 − µ),

(A15)and

F2[E] =[E′E′ − 2EE′′ − EE′′ + E′′′

E′E2

−E′′2

E′2E2 +

2E′′

E′EE′

]∣∣∣λ=0

. (A16)

We have used the convention that E = ∂λE and E′ =∂kxE. Eq. (A14) demonstrates that in the diffusive trans-port regime, the DWMR is inversely proportional to theDW width. The following calculation is the detail for theexpansion.

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7

Appendix B: Expansion of Eq. (A13)

We start from the integral

I =

∫BZ

d3k

(2π)3v2δ(E − µ), (B1)

where E(k, λ) and v(k, λ) = E′ = ∂kxE are functions of

k and λ. Using the convention E = ∂λE, we expand thevelocity v and the δ-function around λ = 0,

v2δ(E−µ) =(v0+v0λ+

1

2v0λ

2)2(

δ0+δ0λ+1

2δ0λ

2), (B2)

where v0 = v|λ=0 and δ0 = δ(E|λ=0−µ). Order by orderexpanding the function v2δ(E−µ), we obtain coefficientsfor λi as following,

λ0 : v20δ0 (B3a)

λ1 : 2v0v0δ0 + v20 δ0 (B3b)

λ2 : v0v0δ0 + v0v0δ0 +1

2v0v0δ0 + 2v0v0δ0. (B3c)

For simplicity, we will omit the foot index 0 but keep inmind λ→ 0. Note that δ = E∂Eδ = Eδ′/v and

δ =∂

∂λ(E∂Eδ) = E∂Eδ + E

∂λ(∂Eδ)

= E∂Eδ + E2(∂2Eδ) =

E

vδ′ + E2 1

v

∂kx

(1

vδ′)

=E

vδ′ + E2 1

v2δ′′ − E2 v

v3δ′. (B4)

Substituting these expansions into the integral (B1), In-tegration by parts shows that these coefficients become

λ1 :[(E′E′ − E′′E)

]∣∣λ=0

δ(E|λ=0 − µ), (B5)

λ2 :[1

2E′E′ − EE′′ − 1

2EE′′ +

1

2

E′′′

E′E2

−1

2

E′′2

E′2E2 +

E′′

E′EE′

]∣∣∣λ=0

δ(E|λ=0 − µ).(B6)

As a result, for both ζ, we obtain

δσ = e2τ∑ζ,s

∫BZ

d3k

(2π)3

{λF1[Esζ ]

+λ2

2F2[Esζ ]

}δ(Esζ |λ=0 − µ), (B7)

where F1[E] =[E′E′ − E′′E

]∣∣λ=0

. In our models, theparity symmetry of the functions under kx → −kx, deter-mines that the integral of F1 vanishes. Thus, the DWMRbecomes

Rw =Cdiffuse

σ0S

∫ L/2

−L/2

λ2

2dx =

π

w

Cdiffuse

σ0S. (B8)

Using R0 = L/σ0S, we finally obtain Eq. (A14).

[1] V. Baltz, A. Manchon, M. Tsoi, T. Moriyama, T. Ono,and Y. Tserkovnyak, Rev. Mod. Phys. 90, 015005 (2018).

[2] R. Lebrun, A. Ross, S. A. Bender, A. Qaiumzadeh,L. Baldrati, J. Cramer, A. Brataas, R. A. Duine, andM. Klaui, Nature (London) 561, 222 (2018).

[3] M. Foerster, O. Boulle, S. Esefelder, R. Mattheis, andM. Klaui, “Domain wall memory device,” in Handbookof Spintronics, edited by Y. Xu, D. D. Awschalom, andJ. Nitta (Springer Netherlands, Dordrecht, 2014) pp. 1–46.

[4] T. Jungwirth, X. Marti, P. Wadley, and J. Wun-derlich, Nature Nanotechnology 11, 231 (2016),arXiv:1509.05296 [cond-mat.mtrl-sci].

[5] X. Marti, I. Fina, C. Frontera, J. Liu, P. Wadley, Q. He,R. J. Paull, J. D. Clarkson, J. Kudrnovsky, I. Turek,J. Kunes, D. Yi, J. H. Chu, C. T. Nelson, L. You,E. Arenholz, S. Salahuddin, J. Fontcuberta, T. Jung-wirth, and R. Ramesh, Nature Materials 13, 367 (2014),arXiv:1503.05604 [cond-mat.mtrl-sci].

[6] Y. Wang, C. Song, G. Wang, J. Miao, F. Zeng, andF. Pan, Advanced Functional Materials 24, 6806 (2014),https://onlinelibrary.wiley.com/doi/pdf/10.1002/adfm.201401659.

[7] B. Park, J. Wunderlich, X. Martı, V. Holy, Y. Kurosaki,M. Yamada, H. Yamamoto, A. Nishide, J. Hayakawa,H. Takahashi, A. Shick, and T. Jungwirth, Nature ma-

terials 10, 347—351 (2011).[8] R. Duine, Nature Materials 10, 344 (2011).[9] L. Berger, Journal of Applied Physics 55, 1954 (1984).

[10] G. Tatara and H. Kohno, Phys. Rev. Lett. 92, 086601(2004).

[11] S. Zhang and Z. Li, Phys. Rev. Lett. 93, 127204 (2004).[12] A. Thiaville, Y. Nakatani, J. Miltat, and Y. Suzuki,

Europhysics Letters (EPL) 69, 990 (2005).[13] G. Tatara, T. Takayama, H. Kohno, J. Shi-

bata, Y. Nakatani, and H. Fukuyama, Journal ofthe Physical Society of Japan 75, 064708 (2006),https://doi.org/10.1143/JPSJ.75.064708.

[14] A. Mougin, M. Cormier, J. P. Adam, P. J. Metaxas, andJ. Ferre, Europhysics Letters (EPL) 78, 57007 (2007).

[15] S.-W. Jung, W. Kim, T.-D. Lee, K.-J. Lee, and H.-W. Lee, Applied Physics Letters 92, 202508 (2008),arXiv:0804.3864 [cond-mat.mes-hall].

[16] G. Tatara, H. Kohno, and J. Shibata, Physics Reports468, 213 (2008).

[17] J. Ryu, S.-B. Choe, and H.-W. Lee, Phys. Rev. B 84,075469 (2011).

[18] C. H. Marrows, Advances in Physics 54, 585 (2005),https://doi.org/10.1080/00018730500442209.

[19] O. Boulle, G. Malinowski, and M. Klaui, Materials Sci-ence and Engineering: R: Reports 72, 159 (2011).

Page 8: Domain-Wall Magnetoresistance in Antiferromagnetic Metals · 16/04/2020  · Domain-Wall Magnetoresistance in Antiferromagnetic Metals Jun-Hui Zheng, 1Arne Brataas, Mathias Kl aui,2,1

8

[20] F. G. Aliev, R. Schad, A. Volodin, K. Temst, C. V. Hae-sendonck, Y. Bruynseraede, I. Vavra, V. K. Dugaev, andR. Villar, Europhysics Letters (EPL) 63, 888 (2003).

[21] M. Yamanouchi, D. Chiba, F. Matsukura, and H. Ohno,Nature 428, 539 (2004).

[22] M. Yamanouchi, D. Chiba, F. Matsukura, T. Dietl, andH. Ohno, Phys. Rev. Lett. 96, 096601 (2006).

[23] M. Yamanouchi, J. Ieda, F. Matsukura, S. E. Barnes,S. Maekawa, and H. Ohno, Science 317, 1726 (2007),https://science.sciencemag.org/content/317/5845/1726.full.pdf.

[24] K.-J. Kim, J. Ryu, G.-H. Gim, J.-C. Lee, K.-H. Shin, H.-W. Lee, and S.-B. Choe, Phys. Rev. Lett. 107, 217205(2011).

[25] D. Hinzke and U. Nowak, Phys. Rev. Lett. 107, 027205(2011).

[26] T. Shiino, S.-H. Oh, P. M. Haney, S.-W. Lee, G. Go, B.-G. Park, and K.-J. Lee, Phys. Rev. Lett. 117, 087203(2016).

[27] O. Gomonay, T. Jungwirth, and J. Sinova, Phys. Rev.Lett. 117, 017202 (2016).

[28] A. C. Swaving and R. A. Duine, Journal of Physics: Con-densed Matter 24, 024223 (2011).

[29] E. G. Tveten, A. Qaiumzadeh, O. A. Tretiakov, andA. Brataas, Phys. Rev. Lett. 110, 127208 (2013).

[30] A. Qaiumzadeh, L. A. Kristiansen, and A. Brataas,Phys. Rev. B 97, 020402 (R) (2018).

[31] E. G. Tveten, A. Qaiumzadeh, and A. Brataas, Phys.Rev. Lett. 112, 147204 (2014).

[32] S. K. Kim, Y. Tserkovnyak, and O. Tchernyshyov, Phys.Rev. B 90, 104406 (2014).

[33] H.-J. Park, Y. Jeong, S.-H. Oh, G. Go, J. H.Oh, K.-W. Kim, H.-W. Lee, and K.-J. Lee, arXive-prints , arXiv:2001.07351 (2020), arXiv:2001.07351[cond-mat.mes-hall].

[34] J. Shi, V. Lopez-Dominguez, F. Garesci, C. Wang, H. Al-masi, M. Grayson, G. Finocchio, and P. Khalili Amiri,Nat. Electron. 3, 92 (2020).

[35] G. G. Cabrera and L. M. Falicov, phys-ica status solidi (b) 61, 539 (1974),https://onlinelibrary.wiley.com/doi/pdf/10.1002/pssb.2220610219.

[36] G. Tatara and H. Fukuyama, Phys. Rev. Lett. 78, 3773(1997).

[37] P. M. Levy and S. Zhang, Phys. Rev. Lett. 79, 5110(1997).

[38] Y. Lyanda-Geller, I. L. Aleiner, and P. M. Goldbart,Phys. Rev. Lett. 81, 3215 (1998).

[39] J. B. A. N. van Hoof, K. M. Schep, A. Brataas, G. E. W.Bauer, and P. J. Kelly, Phys. Rev. B 59, 138 (1999).

[40] A. Brataas, G. Tatara, and G. E. W. Bauer, Phys. Rev.B 60, 3406 (1999).

[41] U. Ebels, A. Radulescu, Y. Henry, L. Piraux, andK. Ounadjela, Phys. Rev. Lett. 84, 983 (2000).

[42] E. Simanek, Phys. Rev. B 63, 224412 (2001).[43] A. D. Kent, J. Yu, U. Rudiger, and S. S. P. Parkin,

Journal of Physics Condensed Matter 13, R461 (2001).[44] P. Yan and G. E. W. Bauer, Phys. Rev. Lett. 109, 087202

(2012).[45] A. von Bieren, A. K. Patra, S. Krzyk, J. Rhensius,

R. M. Reeve, L. J. Heyderman, R. Hoffmann-Vogel, andM. Klaui, Phys. Rev. Lett. 110, 067203 (2013).

[46] A. Ross, R. Lebrun, O. Gomonay, D. A. Grave, A. Kay,L. Baldrati, S. Becker, A. Qaiumzadeh, C. Ulloa,G. Jakob, F. Kronast, J. Sinova, R. Duine, A. Brataas,A. Rothschild, and M. Klaui, Nano Lett. 20, 306 (2020),arXiv:1907.02751 [cond-mat.mtrl-sci].

[47] P. Shen, Y. Tserkovnyak, and S. K. Kim, arXive-prints , arXiv:2002.11777 (2020), arXiv:2002.11777[cond-mat.mes-hall].

[48] R. P. van Gorkom, A. Brataas, and G. E. W. Bauer,Phys. Rev. Lett. 83, 4401 (1999).

[49] J. Lan, W. Yu, and J. Xiao, Nature Communications 8,178 (2017), arXiv:1706.01617 [cond-mat.other].

[50] R. Jaramillo, T. F. Rosenbaum, E. D. Isaacs, O. G. Sh-pyrko, P. G. Evans, G. Aeppli, and Z. Cai, Phys. Rev.Lett. 98, 117206 (2007).

[51] S. Y. Bodnar, Y. Skourski, O. Gomonay, J. Sinova,M. Klaui, and M. Jourdan, Phys. Rev. Applied 14,014004 (2020).

[52] S. Y. Bodnar, L. Smejkal, I. Turek, T. Jungwirth,O. Gomonay, J. Sinova, A. A. Sapozhnik, H. J. Elmers,M. Klaui, and M. Jourdan, Nature Communications 9,348 (2018), arXiv:1706.02482 [cond-mat.mtrl-sci].

[53] R. Cheng and Q. Niu, Phys. Rev. B 86, 245118 (2012).[54] G. D. Mahan, Many Particle Physics, Third Edition

(Plenum, New York, 2000).[55] Y. V. Nazarov and Y. M. Blanter, Quantum Trans-

port: Introduction to Nanoscience (Cambridge Univer-sity Press, 2009).