manipulating light with single nanowires - for physics · manipulating light with single nanowires....
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Manipulating Light with Single Nanowires
Sino-UK Workshop on Nanophotonics and Metamaterials, Peking Univ
Limin TongState Key Laboratory of Modern Optical Instrumentation Department of Optical Engineering, Zhejiang University
2012-12-07
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OutlineOutline
1. Introduction — Nanowire Photonics
2. Nanowire Light Manipulation2.1 Light Generation
2.2 Light Propagation
2.3 Light Modulation
2.4 Light Detection
3. Summary & Outlook
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OutlineOutline
1. Introduction — Nanowire Photonics
2. Nanowire Light Manipulation2.1 Light Generation
2.2 Light Propagation
2.3 Light Modulation
2.4 Light Detection
3. Summary & Outlook
![Page 4: Manipulating Light with Single Nanowires - For physics · Manipulating Light with Single Nanowires. ... Au-Nanorod-doped nanofiber plasmonics. P. Wang et al., Nano Lett. 12, 3145](https://reader031.vdocuments.net/reader031/viewer/2022022018/5b8edd1809d3f28c298b9c0c/html5/thumbnails/4.jpg)
1.Introduction
4
▪
Nanowire
ZnO nanowire Ag nanowire
1-D structure large aspect ratiodiameter 100-102 nm
Glass nanofiber
L. M. Tong et al., Nature 426, 816 (2003)
X. Guo et al., Nano Lett. 9, 4515 (2009)
Semiconductor Metal
Dielectric
close to or below the wavelength of visible light
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1.Introduction
Manipulating light on a nanometer scale with high flexibility
Wrapping light around a human hair
low loss
tight optical confinement
strong evanescent fields
abnormal waveguide dispersion
…
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Favorable properties of nanowires for photonics
Sub-wavelength dimension
Tight optical confinement
Large surface-to-volume ratio
Engineerable surface states
Strong evanescent fields
Free-standing and low-mass
High mechanical strength
Optically visible
▪
Why it is attractive to Photonics ?
Small footprint devicesLow-threshold nonlinear effects
Bandgap
engineering for light absorption, conversion, emission
Strong near-field interaction
Sensitivity to light momentum
Easy micro/nanomanipulation
1.Introduction
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▪
Why it is attractive to Photonics ?
7
Nanowire
Electrons, photons, phonons, atoms, polaritons
on the subwavelength or nanometer scale
Fascinating 1-D structure for manipulating
Fundamental study and technological applications
Intrigue a variety of opportunities for
1.Introduction
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1.IntroductionJ. Giles, Nature 441, 265 (2006)
Nanowire
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1.IntroductionJ. Giles, Nature 441, 265 (2006)
Nanowire
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Nanowires
Nanowires studied in our group
Glass nanofibers e.g., Silica, phosphate
Polymer nanofibers e.g., PMMA, PS
Semiconductor nanowires e.g., ZnO, CdSe
Metal nanowires e.g., Silver, gold
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NanowiresGlass nanofibers e.g., Silica, phosphate
Polymer nanofibers e.g., PMMA, PS
Semiconductor nanowires e.g., ZnO, CdSe
Metal nanowires e.g., Silver, gold
OpticsNear-field optics Guide wave optics OptoelectronicsNonlinear opticsPlasmonicsQuantum opticsOptomechanics
Plenty of opportunities for manipulating light with nanowires
Nanowires studied in our group
+
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Semiconductor
Glass
Polymer
20032004
20052006
20072008
20092010
2011
Low-loss optical nanofiber
Nature 426, 816 (2003)
Nanofiber opticsOpt. Express 12, 1025 (2004)
Nanowire photon- plasmon near-field
couplingNano. Lett. 9, 4515 (2009)
Microfiber laserAPL 89, 143513 (2006)
Microfiber dye laserAPL 90, 233501 (2007)
Nanofiber MZI Opt. Lett. 33, 303 (2008)
Polymer single- nanofiber optical sensor
Nano. Lett. 8, 2757 (2008)
Single-nanowire single-mode lasers
Nano. Lett. 11, 1122 (2011)
Quantum-dot- activated nanofibers
Adv. Mater. 23, 3770 (2011)
Roadmap of Our Nanowire Photonics ResearchSince 2003
Nanofiber couplerNano Lett. 5, 259 (2005)
Metal
Carbon
Bandgap-engineered nanowires
JACS 133, 2037 (2011)Nano. Lett.11, 5058 (2011)
Microfiber- microfluidic
optical sensors Lab Chip 11, 3720 (2011)
2012
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Semiconductor
Glass
Polymer
20032004
20052006
20072008
20092010
2011
Low-loss optical nanofiber
Nature 426, 816 (2003)
Nanofiber opticsOpt. Express 12, 1025 (2004)
Nanowire photon- plasmon near-field
couplingNano. Lett. 9, 4515 (2009)
Microfiber laserAPL 89, 143513 (2006)
Microfiber dye laserAPL 90, 233501 (2007)
Nanofiber MZI Opt. Lett. 33, 303 (2008)
Polymer single- nanofiber optical sensor
Nano. Lett. 8, 2757 (2008)
Single-nanowire single-mode lasers
Nano. Lett. 11, 1122 (2011)
Quantum-dot- activated nanofibers
Adv. Mater. 23, 3770 (2011)
Roadmap of Our Nanowire Photonics ResearchSince 2003
Nanofiber couplerNano Lett. 5, 259 (2005)
Metal
Carbon
Bandgap-engineered nanowires
JACS 133, 2037 (2011)Nano. Lett.11, 5058 (2011)
Microfiber- microfluidic
optical sensors Lab Chip 11, 3720 (2011)
2012
Light Manipulation
generation, propagation, modulation and detection of light with single nanowires
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Contributed by many colleagues and students of our Nanophotonics Research Group
Nanophotonics Research Group @ ZJU www.nanophotonics.zju.edu.cn
Group photo 2012-06
Faculty 4, PhD student 11, MSc student 10
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This talk ──
our recent research in
Nanowire Light Manipulation
1 Light Generation — Nanowire lasing
2 Light Propagation— Nanowire waveguiding
3 Light Modulation— Nanowire optical modulation
4 Light Detection — Nanowire photodetection
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OutlineOutline
1. Introduction — Nanowire Photonics
2. Nanowire Light Manipulation2.1 Light Generation
2.2 Light Propagation
2.3 Light Modulation
2.4 Light Detection
3. Summary & Outlook
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OutlineOutline
1. Introduction — Nanowire Photonics
2. Nanowire Light Manipulation2.1 Light Generation
2.2 Light Propagation
2.3 Light Modulation
2.4 Light Detection
3. Summary & Outlook
![Page 18: Manipulating Light with Single Nanowires - For physics · Manipulating Light with Single Nanowires. ... Au-Nanorod-doped nanofiber plasmonics. P. Wang et al., Nano Lett. 12, 3145](https://reader031.vdocuments.net/reader031/viewer/2022022018/5b8edd1809d3f28c298b9c0c/html5/thumbnails/18.jpg)
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2.1 Nanowire Light Generation
One of the simplest approach –— optically or electrically pumping an active nanowire (e.g., a semiconductor nanowire)
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2.1 Nanowire Light Generation
One of the simplest approach –— optically or electrically pumping an active nanowire (e.g., a semiconductor nanowire)
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Y. Xiao et al., (Submitted)
However ─
this kind of laser
multimode
single cavityhigh threshold
low endface reflectivity (1%)
2.1 Nanowire Light Generation
One of the simplest approach –— optically or electrically pumping an active nanowire (e.g., a semiconductor nanowire)
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S. S. Wang et al., Opt. Express 17, 10881 (2009)
3D-FDTD
211
nn
R << e.g., ZnO nanowire (D=300nm)
R ~ 0.01 @633nm
Low quality of the F-P cavity
High threshold for nanowire lasing
Endface reflectivity
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2 2
2
(1 2 ) (1 ) exp( 2 )4 (1 )(1 ) exp( 2 )
T K lR K K l
S. S. Wang et al., Opt. Lett. 34, 253 (2009)
Recently, relying on strong near-field coupling of nanowires, we proposed to create high-reflectivity Sagnac loop mirrors in a single nanowire
— a technique learnt from fiber optics
Y. Xiao et al., Nano Lett. 11, 1122 (2011)
Fold a nanowire into loop mirrors at both ends increase the reflectivtiy and create additional cavities
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4-cavity coupling Mode selection via Vernier effect Single-mode low-threshold nanowire laser
Y. Xiao et al., Nano Lett. 11, 1122 (2011)
One cavity, R ~ 1%
4 coupled cavitiesR > 30 %
2.1 Nanowire Light Generation
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Y. Xiao et al., Nano Lett. 11, 1122 (2011)
CdSe Nanowire200-nm diameter75-um length
Pumping light: 532-nm pulses(5 kHz repetition rate, 15 ns pulse width)
2.1 Nanowire Light Generation
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Y. Xiao et al., Nano Lett. 11, 1122 (2011)
97 μJ/cm259.7 μJ/cm234.4 μJ/cm2
Single-mode low-threshold nanowire laser
2.1 Nanowire Light Generation
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OutlineOutline
1. Introduction — Nanowire Photonics
2. Nanowire Light Manipulation2.1 Light Generation
2.2 Light Propagation
2.3 Light Modulation
2.4 Light Detection
3. Summary & Outlook
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Less than /5Confinement
Loss
Photonic v.s. PlasmonicBetter than /10
Low Very high
2.2 Nanowire Light Propagation
For dielectric nanowire waveguides, optical confinement is limited by optical diffraction
Optical micrograph of 650-nm light guiding through a silica (D=500 nm), a ZnO (D=300 nm) and a silver (D=100 nm) nanowires in cascade
X. Guo et al., Laser Photon. Rev. (In press)
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2.2 Nanowire Light Propagation
Chemically grown metal nanowire is one of the most attractive candidates owing to its unparallel uniformities and sidewall smoothness low scattering loss
SEM image of a 290-nm- diameter Ag nanowire
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However, there are great challenges for using tightly confined palsmonic nanowires
e.g., efficient coupling light into plasmons in single nanowires
2.2 Nanowire Light Propagation
Lens-focusingPrism-coupling
A. W. Sanders et al., Nano Lett. 6, 1822 (2006)
conventionally using bulk components with low efficiency
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ZnO nanowire Ag nanowire
Relying on tight confinement & strong near-field interaction of nanowire waveguides, we proposed directly coupling a dielectric and a metal nanowire by highly localized near-field interaction
2.2 Nanowire Light Propagation
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Silica nanofiberSilver nanowire
300-nm silica nanofiber
80-nm silver nanowire
@633-nm wavelength
Coupling a 633-nm light from a 500-nm-diameter silica nanofiber to a 200-nm-diameter silver nanowire
Simulation
Experimental
Which was confirmed by both numerical simulation and experimental result
2.2 Nanowire Light Propagation
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After optimization of the geometric parameters, coupling efficiency can go typically higher than 50%
Fractional output from the Ag nanowire: 49%
Coupling efficiency ~75%Silica nanofiber: D=500 nm
Ag nanowire: D=240 nm L=12µm
Deducting the guiding loss:
Ag about 0.43 dB/µm ZnO lower than 0.001dB/µm
Nanowire Coupling
X. Guo et al., Nano Lett. 9, 4515 (2009)
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Coupling length ~220 nm
270-nm-diameter ZnO nanowire
240-nm-diameter Ag nanowire
Branch coupling of photonic and plasmonic nanowires
Nanowire Coupling
X. Guo et al., Nano Lett. 9, 4515 (2009)
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Branch coupling of photonic and plasmonic nanowires
Nanowire Coupling
X. Guo et al., Nano Lett. 9, 4515 (2009)
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Fractional output from the Ag nanowire:
488nm —— 4%
532nm —— 8%
650nm —— 64%
Coupling efficiency ~82%
Deducting the guiding loss:
Ag about 0.43 dB/µm ZnO lower than 0.001dB/µm
Branch coupling of photonic and plasmonic nanowires
Nanowire Coupling
X. Guo et al., Nano Lett. 9, 4515 (2009)
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Mach-Zehnder InterferometerHybrid “Photon-Plasmon” circuits and devices
Applications
X. Guo et al., Nano Lett. 9, 4515 (2009)
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(1) Mach-Zehnder Interferometer
3-2. Hybrid “Photon-Plasmon” circuits and devices
As-assembled MZI
ZnO Nanowire: D 330 nm, L 89 µm
Ag Nanowire: D 120 nm, L 6.5 µm
X. Guo et al., Nano Lett. 9, 4515 (2009)
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Mach-Zehnder Interferometer
Hybrid “Photon-Plasmon” circuits and devices
ZnO Nanowire: D 330 nm, L89 µm
Ag Nanowire: D 120 nm, L 6.5 µm
FSR = 2.75 nm @710 nm
Potential applications: sensors, modulators etc.X. Guo et al., Nano Lett. 9, 4515 (2009)
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Au nanorods doped polymer nanowires
For tighter confinement with higher localization
Au nanorods : 20 nm dimeter, 100 nm length
P. Wang et al., Nano Lett. 12, 3145 (2012)
2.2 Nanowire Light Propagation
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Au-Nanorod-doped nanofiber plasmonics
Au nanorods doped PS nanofibers
P. Wang et al., Nano Lett. 12, 3145 (2012)
SPP resonance spectra of Au nanorods doped in PAM polymer nanowires
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For guided light with wavelength of 785 nm (coincided with the L-SPR peak), the photon-LSPR-conversion efficiency goes up to 70% for a single nanorod.
Single nanorod excitation
Potentials: optical sensing, nonlinear optics …
P. Wang et al., Nano Lett. 12, 3145 (2012)
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Humidity sensing
Fast response, high sensitivity, no photo-bleaching
Au-Nanorod-doped nanofiber plasmonics
P. Wang et al., Nano Lett. 12, 3145 (2012)
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OutlineOutline
1. Introduction — Nanowire Photonics
2. Nanowire Light Manipulation2.1 Light Generation
2.2 Light Propagation
2.3 Light Modulation
2.4 Light Detection
3. Summary & Outlook
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2.4 Nanowire Light Detection
In conventional photodetection scheme, light was irradiated on the nanowire.
Relying on the tight confinement of a nanowire waveguide, we tried a waveguiding detection of light in single nanowires.
using NW length (~100 um) rather than the thickness (~ 0.5 um) for light capture
greatly enhance the light-matter interaction
F. X. Gu et al., Nanotechnology 22, 425201 (2011)
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• Sub-bandgap photoconductivity, infrared optical quenching
Enhanced Sub- bandgap effects
Make it possible for light detection with sub-bandgap effects
F. X. Gu et al., Nanotechnology 22, 425201 (2011)
2.4 Nanowire Light Detection
CdS bandgap: 2.46 eV
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Extrinsic photoconductivity
Compared with irradiation scheme, waveguiding detection offer anenhancement factor of ~105
CdS nanowire photodetection
@ 593 nm
Make it possible for light detection with sub-bandgap effects
2.4 Nanowire Light Detection
F. X. Gu et al., Nanotechnology 22, 425201 (2011)
Extend the spectral response to longer
wavelength with high sensitivity
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To further extend the spectral range, we developed a source-moving VLS growth technique, and obtained bandgap-engineered nanowires
2.4 Nanowire Light Detection
CdSSe nanowire with gradient lattices and compositions along the length of the nanowire
F. X. Gu, et al., J. Am. Chem. Soc. 133, 2037(2011)
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To further extend the spectral range, we developed a source-moving VLS growth technique, and obtained bandgap-engineered nanowires
2.4 Nanowire Light Detection
CdSSe nanowire with gradient lattices and compositions along the length of the nanowire
with bandgap continuously engineered from 500 to 700 nm
F. X. Gu, et al., J. Am. Chem. Soc. 133, 2037(2011)
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Using a bandgap-engineered CdSSe nanowire for light detection, and incorporated with infrared quenching effect
2.4 Nanowire Light Detection
F. X. Gu et al., Appl. Phys. Lett. 99, 181111 (2011)
we have successfully covered the spectral range from 400 to 1600 nm using a single nanowire
Infrared quenching of photoconductivityin a 350 nm diameter CdSSe NW.Ib is established by 532 nm light at constant Pin of 10 nW is quenched upon the addition of 1550 nm signal light
Infrared quench
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OutlineOutline
1. Introduction — Nanowire Photonics
2. Nanowire Light Manipulation2.1 Light Generation
2.2 Light Propagation
2.3 Light Modulation
2.4 Light Detection
3. Summary & Outlook
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Summary
▪
Manipulating light with single nanowires have brought new opportunities for light generation, propagation, modulation and detection.
▪
Waveguiding photonic nanowires offer favorable properties for manipulating light on the nanoscale.
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For light manipulation
Outlook
How far can we go ? ─ depends on ─
How well can we confine and guide the light
What’s the next ?
Dielectric Semiconductor Plasmonic
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0.1 nm 1 nm 10 nm 100 nm 1000 nm 10 um
Atomic wire Nanowire Microwire
Nanotube/NanowireMetal AW
Quantum confinement Metal NW
Optical confinement
Semiconductor NW
Glass NW
Nanowire Optics Guide wave opticsNear-field optics
Nanowire + New Physics
Nonlinear opticsQuantum optics
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54
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Optics in an optical nanofiber
▫
Introduction
as has been envisioned in glass optical nanofibers in recent years L. Tong et al., Opt. Commun. 285, 4641 (2012)
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Zhejiang University (China)Min Qiu
University of Houston (USA)Jiming Bao
Harvard University (USA) Eric Mazur
Peking University (China)Qihuang Gong, Ying Gu, Lun Dai
Hunan University (China)Anlian Pan
Gatech (USA)Younan Xia
Collaborators
Fudan University (China)Weitao Liu
Acknowledgement
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National Science Foundation of China(NSFC)
National Basic Research Program (973) of China
Ministry of Education, China
National Science Foundation of USA (NSF)
etc.
Acknowledgement
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Thank you
Acknowledgement