Nucleation MechanismMost common model:Methane solvation shell is dodecahedral hydrate cageNucleation occurs by aggregation of dodecahedral water cages

Other models based on long-range ordering of methane molecules

Mechanism: Long Lived Fragments

Cluster GrowthLarge, rapid variations in cluster sizeNot dependent on clustering distance

Chart2

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15105105

87979

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67171

106565

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85656

12101107

95252

76565

123535

94748

127679

108284

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107071

137478

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125151

87575

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56666

1068110

11142143

115455

67777

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108080

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76262

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124848

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86262

67980

135257

11104105

76868

77273

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197778

76868

7106106

197070

85252

297070

116969

226466

128185

87474

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8129133

125454

127676

990119

184646

216871

57779

106767

96565

158081

87073

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8104117

107273

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164949

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106868

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109393

12125125

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67575

115860

127476

108989

65656

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57373

108485

127676

108688

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75255

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8111111

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129797

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105153

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87070

266060

106060

97272

137171

128282

76666

137575

9138139

106363

178989

107477

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13103109

157878

7135135

119292

118080

9111116

95456

96969

98787

139395

139395

2.75 A

3.3 A

3.5 A

t / ns

number of hydrate waters

Size of Biggest Cluster

3.5A

0.00225

0.00323

0.00420

0.00519

0.00625

0.00714

0.00816

0.00918

0.0121

0.01128

0.01215

0.01318

0.01419

0.01518

0.01625

0.01727

0.01820

0.01923

0.0224

0.02116

0.02221

0.02318

0.02430

0.02519

0.02622

0.02731

0.02823

0.02919

0.0328

0.03123

0.03227

0.03337

0.03424

0.03520

0.03626

0.03719

0.03828

0.03918

0.0426

0.04122

0.04232

0.04322

0.04428

0.04521

0.04631

0.04736

0.04832

0.04923

0.0524

0.05131

0.05215

0.05322

0.05423

0.05528

0.05617

0.05723

0.05833

0.05924

0.0623

0.06123

0.06223

0.06327

0.06418

0.06514

0.06621

0.06729

0.06823

0.06923

0.0720

0.07122

0.07227

0.07313

0.07420

0.07525

0.07623

0.07719

0.07816

0.07927

0.0828

0.08139

0.08233

0.08328

0.08421

0.08523

0.08625

0.08733

0.08835

0.08925

0.0916

0.09112

0.09227

0.09311

0.09425

0.09538

0.09621

0.09738

0.09824

0.09918

0.116

0.10113

0.10229

0.10333

0.10429

0.10535

0.10628

0.10716

0.10838

0.10924

0.1121

0.11116

0.11224

0.11321

0.11424

0.11537

0.11619

0.11714

0.11815

0.11936

0.1228

0.12126

0.12228

0.12324

0.12442

0.12526

0.12631

0.12729

0.12828

0.12926

0.1323

0.13120

0.13218

0.13324

0.13427

0.13523

0.13622

0.13714

0.13823

0.13934

0.1420

0.14113

0.14226

0.14320

0.14424

0.14519

0.14642

0.14731

0.14821

0.14927

0.1522

0.15131

0.15225

0.15325

0.15431

0.15524

0.15634

0.15738

0.15835

0.15928

0.1626

0.16128

0.16248

0.16343

0.16434

0.16535

0.16617

0.16736

0.16827

0.16931

0.1724

0.17123

0.17221

0.17332

0.17422

0.17540

0.17624

0.17728

0.17826

0.17932

0.1820

0.18123

0.18243

0.18349

0.18423

0.18526

0.18616

0.18731

0.18836

0.18927

0.1934

0.19142

0.19225

0.19346

0.19420

0.19533

0.19647

0.19741

0.19818

0.19940

0.231

0.20136

0.20245

0.20327

0.20443

0.20552

0.20646

0.20738

0.20839

0.20948

0.2134

0.21135

0.21239

0.21323

0.21433

0.21532

0.21640

0.21730

0.21844

0.21940

0.2234

0.22155

0.22242

0.22343

0.22441

0.22540

0.22647

0.22748

0.22841

0.22940

0.2344

0.23159

0.23268

0.23339

0.23453

0.23539

0.23635

0.23764

0.23853

0.23981

0.2453

0.24137

0.24257

0.24339

0.24445

0.24556

0.24649

0.24750

0.24857

0.24942

0.2549

0.25163

0.25250

0.25345

0.25452

0.25578

0.25645

0.25738

0.25858

0.25966

0.2646

0.26159

0.26256

0.26358

0.26447

0.26547

0.26646

0.26750

0.26851

0.26949

0.2735

0.27177

0.27232

0.27357

0.27443

0.27547

0.27652

0.27752

0.27857

0.27960

0.2851

0.28164

0.28264

0.28349

0.28448

0.28550

0.28642

0.28735

0.28858

0.28967

0.2954

0.29165

0.29254

0.29350

0.29457

0.29555

0.29635

0.29751

0.29845

0.29956

0.356

0.30156

0.30343

0.30455

0.30564

0.30654

0.30746

0.30874

0.30954

0.3157

0.31159

0.31235

0.31352

0.31467

0.31537

0.31630

0.31744

0.31858

0.31942

0.3258

0.32153

0.32257

0.32367

0.32458

0.32561

0.32673

0.32752

0.32847

0.32954

0.3352

0.33160

0.33247

0.33355

0.33448

0.33590

0.33652

0.33763

0.33855

0.33942

0.3456

0.34154

0.34239

0.34357

0.34459

0.34543

0.34656

0.34763

0.34840

0.34943

0.3553

0.35152

0.35248

0.35344

0.35445

0.35546

0.35657

0.35747

0.35861

0.35974

0.3651

0.36149

0.36259

0.36362

0.36450

0.36548

0.36647

0.36770

0.36879

0.36976

0.3735

0.37166

0.37255

0.37390

0.37482

0.37549

0.37675

0.37761

0.37890

0.37956

0.3868

0.38154

0.38263

0.38355

0.38476

0.38576

0.38690

0.38745

0.38872

0.38990

0.3968

0.39143

0.39252

0.39349

0.39457

0.39562

0.39666

0.39750

0.39867

0.39953

0.444

0.40189

0.40242

0.40394

0.40457

0.40561

0.40646

0.40757

0.40847

0.40948

0.4157

0.41144

0.41254

0.41344

0.41453

0.41547

0.41641

0.41738

0.41852

0.41935

0.4242

0.42170

0.42298

0.42358

0.42460

0.42565

0.42659

0.42748

0.42860

0.42939

0.4350

0.43148

0.43253

0.43359

0.43473

0.43546

0.43672

0.43743

0.43872

0.43955

0.4443

0.44137

0.44288

0.44322

0.44460

0.44539

0.44686

0.44756

0.44851

0.44948

0.4552

0.45139

0.45248

0.45333

0.45457

0.45556

0.45643

0.45754

0.458105

0.45957

0.4673

0.46167

0.46265

0.46349

0.46485

0.46599

0.466100

0.46761

0.46874

0.46981

0.4781

0.47177

0.47280

0.47353

0.47454

0.47566

0.47670

0.47768

0.47883

0.47965

0.4848

0.48186

0.48237

0.48391

0.48483

0.48568

0.48673

0.48794

0.48852

0.489104

0.4948

0.49141

0.49227

0.49394

0.49447

0.49549

0.49645

0.49732

0.49842

0.49982

0.553

0.50172

0.50276

0.50387

0.50436

0.50554

0.50675

0.50764

0.50850

0.50947

0.5137

0.51155

0.51271

0.51396

0.51467

0.51574

0.51654

0.51782

0.51864

0.51968

0.5271

0.52178

0.52286

0.52360

0.52458

0.52560

0.52677

0.52751

0.52855

0.52949

0.53100

0.53189

0.53284

0.53345

0.53486

0.53562

0.53648

0.53770

0.53880

0.53989

0.5447

0.54169

0.54246

0.54374

0.54469

0.54582

0.54680

0.54788

0.54891

0.54981

0.5570

0.55177

0.55260

0.55333

0.55488

0.55538

0.55679

0.55771

0.55847

0.55954

0.5655

0.56153

0.56256

0.56393

0.56450

0.56592

0.56674

0.567117

0.56892

0.56970

0.5796

0.57163

0.57267

0.57355

0.57457

0.57560

0.57674

0.57778

0.57868

0.57980

0.5857

0.58162

0.58297

0.58359

0.58481

0.58579

0.586105

0.58747

0.58864

0.58984

0.59107

0.59146

0.59274

0.59369

0.59495

0.59564

0.59669

0.59769

0.59866

0.59978

0.663

0.60158

0.60258

0.60467

0.60555

0.60674

0.60750

0.60887

0.60969

0.6195

0.61198

0.61251

0.61344

0.61442

0.61588

0.61650

0.61748

0.61880

0.61949

0.6288

0.62143

0.62244

0.62381

0.62469

0.62544

0.62663

0.62766

0.62858

0.62944

0.6375

0.63151

0.632103

0.63371

0.63446

0.63569

0.63659

0.63762

0.63860

0.63980

0.6491

0.64176

0.64274

0.64350

0.64464

0.64585

0.646107

0.64769

0.64884

0.64991

0.6599

0.65185

0.65289

0.65353

0.65465

0.65569

0.65654

0.65770

0.65866

0.65973

0.6673

0.66178

0.66271

0.66361

0.66465

0.66587

0.66682

0.66758

0.66868

0.66958

0.6773

0.671106

0.67273

0.67347

0.67479

0.67589

0.67671

0.67793

0.67883

0.67976

0.6864

0.681100

0.68293

0.68387

0.68465

0.685121

0.686127

0.68790

0.68867

0.68959

0.6986

0.69161

0.692101

0.69357

0.69493

0.69572

0.69658

0.69777

0.69872

0.69985

0.758

0.70181

0.70267

0.70358

0.70477

0.70578

0.70684

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