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OFFICE OF CIVILIAN RADIOACTIVE WASTE MANAGEMENT 1A: QA SPECIAL INSTRUCTION SHEET Page: 1 of: I Conpete Only AppEcable Items This Is a placeholder page for records ihst cannot be scanned or microfilmed 2. Record Date 3. Accsslon Nurnber 09t23/1999 .MOL.19990928.0234 4. Aunhor Namels) 6. Aur Organization ABDELI ASEED NJA 6. Title SIMULATING OF THE EFFECT ON CRITICALITY OF SIMULTANOUS MATRDC DEGRADATION AND ASSEMBLY COLLAPSE FOR THE 21 PWR WASTE PACAKGE 7. Document Numberls) S. ersion CAL-EBS-NU-M00D2 REV. 00 S. Docurnent Type 10. Medium DISKETTE - De--,;3n Doemment D4+0 vis />p+;c 11. Access Control Code PUB 12. Traceabillty Designator CAL-EBS-NU-000002 13. Comments g. OAKDISKETTE -hus Secial rrocezs Ccadtchrven1.4L) CAN BE LOCATED THROUGH THE RECORDS PROCESSING CENTER AP-17.1Q.1 Rev. 0613011999

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Page 1: OFFICE OF CIVILIAN RADIOACTIVE WASTE SPECIALDocument Identifier, CA-EBS-NU0002 REV 00 Page 6 of 30 hZN'g. Sw t Mflu. O w (L100J0 .0000 . W100) aim WI000 MM000W. .10000 giuFe 1 5 1o

OFFICE OF CIVILIAN RADIOACTIVE WASTE MANAGEMENT 1A: QASPECIAL INSTRUCTION SHEET Page: 1 of: I

Conpete Only AppEcable Items

This Is a placeholder page for records ihst cannot be scanned or microfilmed2. Record Date 3. Accsslon Nurnber

09t23/1999 .MOL.19990928.0234

4. Aunhor Namels) 6. Aur Organization

ABDELI ASEED NJA

6. TitleSIMULATING OF THE EFFECT ON CRITICALITY OF SIMULTANOUS MATRDC DEGRADATION AND ASSEMBLYCOLLAPSE FOR THE 21 PWR WASTE PACAKGE

7. Document Numberls) S. ersion

CAL-EBS-NU-M00D2 REV. 00

S. Docurnent Type 10. Medium

DISKETTE - De--,;3n Doemment D4+0 vis />p+;c11. Access Control CodePUB

12. Traceabillty DesignatorCAL-EBS-NU-000002

13. Comments g.OAKDISKETTE -hus Secial rrocezs Ccadtchrven1.4L)

CAN BE LOCATED THROUGH THERECORDS PROCESSING CENTER

AP-17.1Q.1 Rev. 0613011999

Page 2: OFFICE OF CIVILIAN RADIOACTIVE WASTE SPECIALDocument Identifier, CA-EBS-NU0002 REV 00 Page 6 of 30 hZN'g. Sw t Mflu. O w (L100J0 .0000 . W100) aim WI000 MM000W. .10000 giuFe 1 5 1o

II

M{OL. 19990928.6234 MO L.19990928 .0234

OFFICE OF CMIVAN RADIOACTIVE WASTE MANAGEMENT. CA QA

CALCULATION COVER SHEET Page: I Of. 30

2. Calctulton TitleSimulating the Effect on Citicality of'Simultaneous Matrix Degradation and Assembly Collapse for the 21 PWR Waste Package

3. Docurment Idenrffir Pincludfn Revision Nurnber)CAL-EBS-NU40W0 REV 00

4. Totat Attachments I. AttAchment Numbers- Nwnber of paGes In each2 V ________1-3,CDROM_

Pft Nare Sinpue Date

6. odgintor Abdelhalim A. Alsaed z /2 /T7

7. Checkar Laeta Angers 4 A __3_*_ _

S.~~~ ~ ~ ~ .L.a_

S. Lead Peter Gottlieb 4Z4

E. Remarks

Revision Nstory

10. Revsion No. I1. Oescri4Won of Revision

00 Initial Issue

A'41ZRe. 03119

Ar-s4.1 ZCl Rev. 06J3011E99

Page 3: OFFICE OF CIVILIAN RADIOACTIVE WASTE SPECIALDocument Identifier, CA-EBS-NU0002 REV 00 Page 6 of 30 hZN'g. Sw t Mflu. O w (L100J0 .0000 . W100) aim WI000 MM000W. .10000 giuFe 1 5 1o

Waste Package Operations CalculationTitle: Simulating the Effect on Criticality of Simultaneous Mtr Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier CAL-EBS-NU 000002 REV 00 Page 2 of 30

CONTENTS

Page

1. PRPOSE_.__........_.._.__...... _ ._ 5

2. METHOD _..... ....... n... ... ...... 5.....n........ _ ..... 5

3. ASSUMPTIONS 6

4. USE OF COMPUTER SOFTWARE AND MODELS_. ........ 8

4.1 SOFTWARE APPROVED FOR QUALIrT ASSURANcE (QA) WORK ............................. ..... 842 SOFFvARE ROurIEs.. . ......... ..................4 4 . o m 3 .. ...... M........DEL...S...................... ........ ...............

S. CALLATIN 9 . ...

5.1.1 SpentFuelAssenblyParameters .. 95.1.2 lact Waste Package Geometry Parameters .. 115.1.3 Material Propertes .. 115.1.4 Fuel Isotopic Concentratons.. 145.1.5 BasketadFuelDegradationProdut Compositions .............................................. , 1

5.2 CALcuAToN OF NUmBER DENSTES FOR DECIDED BASKET MATEnAL...... .... 165.3 CALCAnoNoFNumBERDEmfmEsFoRFuELREOioN .............................. 175.4 MCNP CASE DEscpnON .... . ............ .... 17

6. RESULTS i....................n.. .... _ .. _....n_...n.n. 187. ATACHMENTS .~._. -.................... __. .. 24

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Wats P~kaP n--4:n"* &M-1l1-t2 -TV ;35C A %VMI A "*VJD .i UA

Title: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier CAL-EBS-NU-000002 REV 00 Page 3 of 30

FIGURES

Page

2-1. Degraded 21 PWR Fuel Waste Package with Unifonn Corrosion Product Distibution ....... 6

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Waste Patkage Operations CalculationTitle: Simulating the Effect on Criticality of Simultaneous Matrix Degrdation and AssemblyCollapse for the 21 PWR Waste PackageDocment Identlfier. CAL-EBS-NU-0 02 REV 00 Page 4 of 30

TABLES

Page

3-1. Principal Long-Term Bumup Credit Isotopes ............................................................. 75-1. Mechanical Parameters ofB&W IS 15 Fuel Assembly .................................................. 105-2. Fuel Region Node eigs and Volumes .... . ............ 105-3. Waste Pacige Dimensions .. ........ . ................. 1154. Densities ofNon-Fuel Materials ..... ... ........... -... . 11S-S. Atomic Weights &nole) ............ ................ . .............. . ...... . ....... 135-6. Chemical Compositions of WP and Fuel Assembly Alloys Modeled ............ .................... 145-7. Corrosion Products Remaining Following Basket Degradation ................................. ...... 155-8. Effects of Fuel Degradation on Principal Isotope Inventoy ..................... ... 166-1. Reactivity Evaluation of Simultaneous Matrix Degradation and Assembly Copse......... 196-2. Reactivity Evaluation of Simultaneous Matrix Degradation and Assembly Collapse..... 206-3. Regression Results of Ak as a Function of Fission Product Loss and Assembly Collapse.. 237-1. List of Attachments ....... . ..... . ;...... 247-2. List of Files in Attachnent II ..... ........ . ....... ...................... 24

Page 6: OFFICE OF CIVILIAN RADIOACTIVE WASTE SPECIALDocument Identifier, CA-EBS-NU0002 REV 00 Page 6 of 30 hZN'g. Sw t Mflu. O w (L100J0 .0000 . W100) aim WI000 MM000W. .10000 giuFe 1 5 1o

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Waste PAckage Operations CalculationTitle: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier: CAL-EBS-NU-000002 REV 00 Page 5 of 30

1. PURPOSE

The purpose of this calculation s to evaluate the effects of fission products loss on the rctivityof commercial pressurized water reactor (PWR) spent nuclear fuel (SNF) in 21 PR wastepackages (VPs) in the event of simultaneous fuel matrix degradation and assembly collapse.ibis is in support of the work outlined in Reference 1.

Referencing in this calculation refers to the input document number appearing in column 2a ofthe Document Input Reference Sheets (DIRS), Attachment I hereto.

.2. METHOD

The Commercial PWR assembly design is based on the Babcock and Wilcox (B&W) 15 x 15Mark B assembly (see Assunption 3.3) In this calculation, multiplication factor (kw) values arecalculated for various degraded WP configurations using the Monte Carlo N-Particle transportcode system version 4B2 (MCNP4B2; CSCI: 30033; Ref. 2). For each combination ofenrichment and burnup evaluated, 18 axial fuel nodes are utilized to allow the effects ofdifferences in burnup along the assembly length to be considered. Fuel region number densitiesused in this criticality evaluation were extracted from the MCNP cases from Reference 3 for aparticular fuel node and decay time.

This calculation considers the waste package with uniform corrosion product distribution Sixfuel configurations, which are based on varying the rod pitch, will be considered for eachcombination of enriciment and bumup. Considering a conservative early breach of the wastepackage, this calculation assumes that the waste package will be full of uniform corrosionproducts at 10,000 years. For the first set of cases the reactivity of the waste package isevaluated for an intact fuel matrix at the nominal rod pitch with funl fission product inventory.At 45,000 years the fuel matrix is considered completely collapsed such that the rods aretouching and all the fission products released Four intermediate cases are also evaluted at14,000, 18,000, 2,000 and 35,000 years for which the rod pitch and fission productconcentrations are linearly evaluated. he general geometry for these cases is presented inFigure 2-1. The reactivity of the collapsed cases is compared to the nominal case at the sametime in life. The time in life of maximum increase of waste package reactivity is chosen to runthe cases needed for the probability calculation. These cases cover all possible combinations offission product loss and collapse fractions with which regression analyses were performed.

The MCNP cases of the three combinations of enrichment and bumup and all four decay times atoriginal rod pitch were taken fion the Tae Attaciment of Reference 3. Input Cards 56 through59 were modified to reflect original rod pitch between assemblies.

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Waste Package Operations Calculationdtie: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier, CA-EBS-NU0002 REV 00 Page 6 of 30

hZN'g. Sw t Mflu. O w

(L100J0 ..0000 W100)aim WI000 MM000W. .10000

giuFe 1 i Uftm 5 or1 1o 4,;Xut D

3.1 Principal+ Istpb p cret is asue tob an =qta meto toacut fr

Controlled Desig Awmpio Ie 00 (Rf 4). M aspin sue throuhou

3.2~ge o SF th lit o rnia stoe rvusystbihdO ., . 3-6 fo log-

asut21. Degraed 21roueo astion ge t o t D3t fu

,~~~~~3 ASUMTIN

3.1 Principal Isotope burnup credit is assmed to be an accale mehod to acount forreduced reactivty of SNF In criticality vutCiouL The basis for this assupion iscOnlld Design Assumption Key 009 (Ref. 4). This assumption is used throughoutSection 5.

3.2 For SNF, the list of '"Principal Isotopes" previously established (Ref. 5, p. 326) for long-term ctcit control was used. lhe 29 pripal isotopes are shown in Tabic 3-1. Thebasis for this asspion is to maintain tconsistencyt wih established preedens Thisassumption is uised throughout Section 5.

I

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wastfi Pnirnsue Anprfinwe e"Tsrtfn

Title: Simulating the Effec on Criticality of Simultaneous Matrix Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier- CAL-EBS-NU-000002 REV 00 Page 7 of 30

Table 3-1. Pncipat Long-Term Bumup Credit Isotopes

._ MoOS To49 Ru-101 Rh-103Ag-09 Nd-143 Nd-145 Sn147 Sn-149SM-i150 Sm151 SM-152 Eu-151 Eu-153Gd- 155 13 1-4 L25 U-M. = Np-.37 P*238 Pu-2W Pu-240Pu-241 Pu-242 Am-241 . Am-242m Am-243

3.3 It is assumed that B&W Mark B 1S x 15 fiuel type is atypical PWR assembly designs tobe used in this analysis. The basis for this assumption is that this assembly design is usedin several existg PWRS. his assumption is used throughout Section 5.

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W�.#� nv%.-44ft-W tI.eta4aw~V a.4a A aifAr ma IFSXa.a.. YW. FJ. St4ALZ.3a -mA- .uU

Title: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier: CAL-EBS-NU-000002 REV 00 Page 8 of 30

4. USE OF COMPUTER SOFTWARE AND MODELS

4.1 Software Approved for Quality Assurance (QA) Work

The calculation of I:z of degraded nternal WP configurations was performed with the MCNPcomputer code version 4B2 (CSCI: 30033; Ref. 2), which calculates kff for a variety ofgeometric configurations wnth neutron cross sections for elements and iotopes described in theEvaluated Nuclear Data File version B-V (ENDF-BV). The calculations using the MCNPsoftware were executed on a Hewlett-Packard workstation. The software qualification of theMCNP software version 4B2, including problems related to calculation of kr for fissile systems,is summarized in the Software Qualification Report for the Monte Carlo N-Particle code (Ref. 2).The MCNP evaluations performed for this calculation are fully within the range of the validationfor the MCNP software versions used. Access to and use of the MCNP software for this analysiswas granted by Software Configuation Management and performed in accordance with eappropriate procedures. Inputs and outputs for the MCNP software are included as AttachmentII as descibed in Section 7.

4.2 Software Routines

Microsoft Excel 97. loaded on a Pentium H PC. This software was used to perform regressionanalyses for which the data are listed in Section 6.

4.3 Models

None used.

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Waste Paekaie Oneratlons CakkulationTitle: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier: CAL-EBS-NU-000002 REV 0 Page 9 of 30

5. CALCULATION

5.1 Inputs

5.1.1 Spent Ful Assembly Parameters

The fuel as bly upon which this calculon is based is the Babcock & Wlcox S x 15 Mark Bfuel assembly. Ihe mechanicalpameters for this assembly tpe are shown in Table S-1. Thisinformation represents actual B&W fel assembly dimensions and is considered qualified data.Table 5-2 provides information on the fel region node heights used in this calculation.

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Waef, Patjmtop nnirsntlnnt

Title: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Jdentifier CAL-EBS-NU-000002 REV 00 Pse 10 of 30

Table 61. Mechanical Parameters of B&W 15 x 15 Fuel Assembly(Ref. 3, p. 9)

Parameter Metric Units

Fuel rods 208 /assembly

Fuel Rods on lawce sde 15 side

Guide tubes 16 lassembty

nsruentadon b bes 1 /assembly

Wotai ude + k ntnent tubes 17 fassembly

dftube materibl Ziro4

u! pellet outer dlameter OD) 0.9398 cm

u £tadc helg* 360.172 cm

Fuel assembly helght 420.7 cm

Aass ofU 464 kg

Mass of UO2 526.38 kg

Percent of ca l densy 95

Fuel dad OD 1 cm

Clad thickness 0.06731 cm

Fuel clad Iner diameter DM 0.657I8 cm

Fuel rod pikh 1.4422 cm

Gde tube OD 13482 cn

de tUbe thickness 0.04064 cm

Guldetel? 126492 cm

Instumentallon ube 9D 125222 cm

tQIpIaced Volume per Fuel Assembly 0.081 R

Table 6-2 Fuel Reglon Node Heights and Volumes(Ref. 3. p. 10)

Node Height (cm) Volume (cmY. 1 1 7800 2585.404521o 17 20.0025 2886.0801

Volumes calculated as (Pellet OD)2(HelghW4

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Waste Pscklge Onerations CalculationTitle: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier: CAL-EBS-NU-0002 REV 00 Page 11 of 30

5.1.2 Intact Waste Package Geometry Parameters

The intact waste package geometry parameters used In this calculation are listed in Table S-3.This information is based on unqualified drawings or QAP-3-9 analyses and is thereforeconsidered unqualified. Corrosion product volume information for the 21 PWR WP wascalculated in Reference 6 and is ummarized in Section S.1.5. The corrosion productinformation is considered unqualified.

Table 6-. Waste Package Dimensions(Ref. 3. p. 10)

21 PWRWP Material, Component Dimensions R.. p. 0)

Outer barrier length (skirt edge to skirt edge) 633.60Outer baier skir length (both ends) 22.50Outer barrier Rd Uckness 11.00 Aste CarcnOuter barrir hner radi 73.17Outer barrer outer radU 63.17Gap between Inner and outer lids 3.00 NotAppcable

Inner barrier length (overall 483.60

Iner barrier Ed tickness 2.60 Alloy 22nner barrer nner radi 71.17 (UNS N0=02)

innr barrier outer radi 73.17

S13 Material Properties

Densities of non-fuel materials used in this analysis are listed in Table 54, which are consideredunqualified:

Table 64. Densiltes of Non-Fuel Materials(Re£ 3, p. 11)

Mterial |Dense (kmS) |

A 16 Grade 70 carbon teel 7832

Inconel Aloy U2 (UNS N065) 8442

;oddyite (U02(SO4)2H2O 4700

Zrcaloy.4 6560Aloy 22 HastelloyAfloyC-22, UNS N060 8890

Water 1000

The atomic weights of isotopes are listed in Table 5-5 ef. 3, p. 11). Avogadros Number [NA]

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Waste Package Onerations CalculationTItle: Simulating the Effect on Criticality of Simultaneous Matrix Degrdation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier CAL-EBS-NU-000002 REV 00 Page 12 of 30

= 0.602252 x 104 (atoms/mole) (Rel 3, p. 1 1) Chemical compositions of alloys used in tbiscalculation are given in Table 5-6. This nformation is obtained fom qualified QAP-3-9analyses, or is considered established filt, and is therefore considered qualified.

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Wase i-Pn-L-akve Onpratflnn - Plenlh'nwWsitf� Pn�ltau� fl,�vnfAYIw fati.ful.44

a..

Title: Simulating th* Eec on Citicality of Simultaneous Ma& Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument dentifien CAI-EBS-NU-000002 REV 00 Page 13 of 30

Table 5. AtomIc Weihts (moe)(Ref. 3, p. 12)

isotope MCNP ID$ Atomc WelghtB-10 6010.600 10.0129388B-11 5011.66C 11.093

NaL 0 ot sed 15.90-16 8016.600 15.094915tF 2000.650: 65.847

Mo5 42095. 94.9Tc-9 43099C 98.90827501Ru-101 44101.0 10.905576Rh103 45103600 102.08511Ag-109 47109.500 108.90756Nd-143 60143fX0: 142.909779Nd-145 6014SfXX0 144.912538SG 147 62147.500 146.914867Sm-149 62149.500 148.91718Sm-150 6210O5 149.917276SM-151 62151.500 150919919Sn-152 62152.500 151.919756Eu-151 63151.55C 150.919838Eu-153 63153.550 152.921242Gd-155 64165f.50 15492664 U33 92 60C 233.039522U-234 92234600 234.04904U-235 92235.500 235.043915U-236 9380 236.045637TUM-238 92238.500 238.05077Np-237 93237.f5C 237.048056Pu-238 94238.ZX0 238.049511Pu-239 94239.550 239.052146Pu-240 94240.500 240.053882PU-241 94241J500 241.05637PU-242 9424250 242.058725Am-241 9241.500 241.056714

Arn242m 95242.50 242.059502Am-243 95243.50 243.061387

* i

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--

WUe#A% P. t4'. wb flp,.uM~n*InW P0V2"Mn11;nT... -..- . -"�& -.. w

Tide: Simulating the Effect on Criticality of Simultaneous Mat Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier, CALEBS-NU-O00002 REV 00 Psge 14 of 30

Table 6. Chem~cal Compositons of WP nd Fuel Assembly Alloys Modeled(Ref. 3, p. 13)

Alloy 22 InconeAlloyMat"rlalIElement A 616 ade (Hastelloy Alloy C- 625 Zlrcay4

65Carbon Steel 22, UNS N06022) (UNS 406625)Fe 95835% 3.000% 6.00% 0.200%Cr _______ 22.000Y 21500% 0.10WeNl . 66.000Y 68.000%

Mn 090% 0.00% 0.600%Mo . 13.000% 9.000% -

6 0.035% 0.015% .Sl 0275% 0.080% 0A.00YeP 0.035% 0.015%C 0220%6 0.010% 0.100%o . 0.120%Co . 2.060% 0930% W -3.000% -

T1 0.400% Al _ * 0A00% -

V 0.350Y% .6Y0Nb+50%Ta -. 3600%Y

Zr N 98.180%Sn . 1.A00%

TOTAL 100.00% 100.% 100.00% 100We%

I

.. -1 �

.IA Fuel Isotopic Concentrations

The fiel isotopic concentritions are the same as those In the MCNP cases from Reference 3 for18 axdal nodes per assembly. The following combinations of enrichment and burnup wereutilized for this calculation: 3 wt% at 20 gigawatt dayshton (OWd/l), 4 wPK at 35 GWdtF and4.5 wt/o at 40 GWd/T.

5.1.5 Basket and Fuel Degradation Product Compositions

Reference 6 performed gcochemsty calculations to determine the composition of the corrosionproduct mixte remaining in the 21 PWR waste package following complete basketdegradation. Table 5-7 summaizes the concentrtions of insoluble corrosion products thatremain after the basket has completely degraded. Reference 6 indicates that this finalcomposition remains fairly constant over the range of possible borated stainless steel degradationrates and drip rates. The molestWP column is calculated by multiplying the moles/L H20column by 4,550 liters of 120, which is the amount of water considered to be in the WP inReference 6 (equivalent to the void space available in a loaded WP with an undegraded basket).

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WAste Package Oeratious. CalculationTitle: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier, CAL-EBS-NU-000002 REV 00 Page S of 30

Table 67. Corroslon Products e"alniV Folowing Basket Degradatlon(lRef. 3, P. 14)

Vouatwer molesfilterBast Corrosion Product WP tnv HIO matesw~

Daspore 0 1.8392E-01 2291 10424.05Hemnate (F02 1.7707E+00 12.7? 68103.6Pyusite n2 2.7361E-02 0.35 1592.5N 4S1 04 3D867E-02 0.1592 724.36Nonbon!t-Ca CaAlm Fe2Ha00) 12874E.02 0216 9828Non(Ste-K (S6,KvAJ= Fe*2 O) 6.25E04 0.0009151 4.1630Nortordle-Mg (Ss4X1g2AuS F 402H) BS323E-03 0.01513 68.8415Norfronte-Na (SaINaAlasn Fe2O,2 9.0407E.04 0.001504 6.8U2

OTAL , 2.0362E400

Reference 6 also examined the effects that fiiel degradation will have on the principal isotopeinventory. Reference 6 examined two cases for both commercial and mixed oxide (MOX) PWRfuel: I) fuel degradation concurrent with basket degradation, and 2) fuel degradation beginningafter basket degradation is completed. The former case for the commercial PWRnasulted in thegreatest loss of principa Iotopes due to lower pH conditions during degradation of the boratedstainless steel and fuel. Table 58 summariz the percentage of each principal isotoperaining at different times from the beginning of fuel degradation. Note that the geochemistrycalculations of Reference 6, and thus the results in Table 54, do not account for the decay of theprinciple isotopes. Decay was accounted for by applying the reduced principle isotopeconcentrations for a given degradation time to a decay time that is equally offset from the pointat which degradation began (i.e., if degridtion is assumed to begin at 10,000 years, the principleisotopeinventories at 12,000 years will be reduied as indicated for a degradation time of 2,000years).

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Waste Packnae Oneratlons CalculationTite: Simulating the Effect on Criticality of Simultaneous Mai Degdation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier, CAL-EBS-NU-000002 REV 00 Page 16 of3O

Tnble 64. Effects of Fuel Degradation on Principal Isotope Inventory(Ref. 3. p. 16)

_______ ~~Fuel Degradatlon Time &O)_______ ___

Element ZO0 4,O0 8,000 15,000 15,00 35.000 90,000 24000U 100% 100% 100% 100% 09% 9% 08% 88%NP 85% 70% % 0% 0% 0% 0% 0%Pu 100% 100% 100% 100% 100% 100% 100% 100%Am 0% MD 0% 0% 0% 0% 0% 0%Mo 0% 0% 0% 0% 0% 0% .o% 0%Tc 0% 0% 0% 0% 0% 0% 0% 0%Ru 100% 100% 100% 100% 100% 100o 100% 100%Rh 100% 100% 100% 100% 100% 100% 100% 100%A_ 87% 80% Gm 43% 12% 0% 0% 0Nd 09% 98% 97% 95% 95% 95% I5Y% 95%Sm 80% 70% 46% 27% 26% 26% 24% 20%Eu 82% 71% 48% 9% . 8% 7% 2% 0%Gd 66% 35%. .14% 6% 6% %: C% 3%

I

52 Calculation of Number Densities for Degraded Basket Material

Based on the total volume of corrosion products remaining following full basket degradation (seeSection 5.1.5), and the total volume contained within the nner barrier minus that occupied by thefitel assemblies (volume of the fiel rods), the corrosion products will ocupy 36.4% of theinterior void space of a 21 PWR WP. If the corrosion products settle to the bottom of the WP,the physical geometry of packed solids will result in a density that is less than theoretical. Forexample, the percent solid content noted for a tight packing of sand (Ref. 3, p;.15) is 58%. Theporosity (the complement of the solids content) of tightly packed carbon-.steel tubesheetcorrosion products that led to the denting of steam generator tubes at two Westinghouse plantswas found to be between 7% and 2S% (Ref. 3, p. 15). Since the oxides in the tubesheet werecompressed to the point of denting the tube, and no such restriction of the oxides in the VIP iscxpected, the tight.packing of sand will be taken to be r ste of that of iron oxide scalethat has settled. At 58% dense packing, If all of the oxides settle to the bottom, they willcompletely cover the bottom three rows of assemblies, and cover more than 95% of the fourthrow (93% or 14 rod rows of a B&W 1 x 15 Mark B assembly is conservatively used for thisanalysis). Number densities were calculated for the above corrosion product and water mixturesby dividing the moles of each element per WP (as indicated in Table 5-7) by the void space theyoccupied and multiplying by Avogadro's Number (0.602252 x 10" atoms/mole). Thesecalculations are performed in Reference 3.

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Waste Packase Operatons CalculationTitle: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and AsssmbiyCollapse for the 21 PWR Waste PackageDocument Identifiern CAL-1BS-NU000002 REV 00 Pare 17 of 30

5.3 Calculation of Number Densities for Ful Region

The gratns/assembly output for each time step was used to calculate the number density of eachprincipal sotope (see Assumption 3.1). Ie number densities of e principal isotopes in thenominal cases for each combination of enrichment and burnup were calcuIated in Reference 3.The reduced number densities in the degraded matrix cases are simply calculated as a frationalchange from the nominal.

5.4 MCNP Case Description

The purpose of this section is to describe the MCNP cases considered for the 21 PWR wastepackage design with intact fuel and filly degraded basket structures. In all of the cases, eachB&W 15 x 15 fuel assembly is treated as a heterogeneous system with the fuel rods and controlrod guide tubes and instrument tubes represented explicitly using the information contained inSection 5.1.1. The fuel assemblies are conservatively represented with water in the fuel rod gapregion, and the instrument and guide tubes, even when surrounded by watercorosion productmixtures, as there is no physical mechanism for getting basket corrosion products into theselocations while the assembly remains intac The composition and dimensions of thecontainment barriers are represented explicitly using the information in Section 5.1.2.

The MCNP cases will consider the evaluation of basket corrosion product composition discussedin Sections .1.5 and S2. The uniformly distributed corrosion product configurations isevaluated. Figure 2-1 shows the geometry details of the MCNP4B2 model for the 21 PWR WPwith a fully degraded basket and uniformly distributed corrosion products for a range of rodpitch values of nominal spacing 1.44272, 1A0266, 13626, 1.2925, 1.19235 cm and touchingrods in a square lattice 1.0922 cm which correspond to decay times of 10,000, 14,000, 18,000,25,000, 35,000 to 45,000 years, respectively. The following combinations-of enrichment andburnup will be evaluated: 3 wP% U-235 at 20 GWdIr, 4 wtc/ 23U at 35 GWd/T, and 4.5 wt/U-235 at 40 GWdIT. The diameter of the guide tubes is slightly larger than the collapsed pitchsuch that a small portion of the clad is lost in the case representation, which has no effect on thesystem reactivity. he pitchldecay time combination that yields the highest increase in wastepackage reactivity will be used to perform the cases for the probability calculations. The threecombinations of burnup and enrichment at the most reactive time in life will be used to evaluatethe waste package reactivity at all pitch values and fission loss fractions such that a total of 108cases will be run.

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Waste Package Operatlons CalculationTitle: Simulating the Effect on Citicalt of Simultaneous Matrix Degradation and AssemblyCollapse for the 21 PWR Waste PackageDocument Identifier: CAT-EBS-NU000002 REV 00 Page 18 of 30

6. RESULTS

Table 6-1 lists cff and standard deviation (a) values for the cases used to determine epitchldecay time combination that yields the highest increase in reactivity. The ases at 25,000years with a pitch of 0.64625 cm yield the highest activity inrease Table 6.2 lists the kvalues for the cases for the three combinations of enrichment and brnup at 25,000 years decayfor all possible fission product loss (FPL) fiactions and pitch combinaons Using the data inTable 6-2. a regression analysis was performed to evaluate Ak as a function of pitch and fissionproduct loss for each combination of enrichment and bumup as listed in Table 6-3. The averageof the three regression fits was evaluated and is listed in Table 6-3. The average energy ofneutron causing fission (AENCF) is also included is the aforementioned tales . The fissionproduct loss fraction used for some of the cases in Table 6-1 was rounded off, thus some of thekeff values are slightly different but within the standard deviation, than the simila cases in Table6-2.

The results reported in Section 6 are based on unqualified data and must be verified prior to usein quality affecting activities or for use n analyses affecting procurement, construction, orfabrication.

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vu..#..flna..aNa..s "-'-'a"--

Title: Simulang the Effect on Criticality of Simutameous Maix Degmdatin and Assembly Collpe for lhe 21 PWR WastePackageDocunit Identifier-, CAL-EBS..NU-000002 REV 00 Nre 19 gf 30

Table 6-1. Readily Evaluaon clShiftrno Md Degradalon and Ass~mby Collpse

0e"d"o k0FP_ AENCF MM AZNCPEzuchment unmi nm 072138 n I FPL . F.(wU-235) (OWd) 7 r4 Pitch so Ma Me Nam (CM) 1 kw 2 (MaY "me k

4.50 40 1000.0 as883 0420 WJ4540bo 0.13 C.M. 0 .00 m.24m8 4Sbo t OOO

4.iO 40 1400.00 0 0.0030 024519 A540do 0.70133 113 0U50 0.00 0.25J R540do 4.00151

4.0 40 18000.00 U886 0AM03024384 m54no 013810 .8 CAM G0022 527004 M454o 001004

: - :.4~~~~50 0. 00= - --:0.oo8 _OS .0.0020 ;Wi5. *2X:40.,,52 S AM- 1 UM Z=0F

4.50 40 35000.00 O0 0 M 03882 u4540go 0.6 177.4 03 2 003 0.305 w45dgo 0O013

4.50 40 45000.00 O 184 0.00304 023039 nu4UOh 05410 100.00 085289 002 8 428 4ho ..02895

4;00 35 10000D0 0.7101 .0280 0250M nSbo 0.72130 0.0 O.7O 0. 002M 0250 nu403o OD004.00 85 UOOO.0 0.87427 0.0028 @248 nu4do 0.70133 11A3 06 o00350 02=03do 0.001524.00 35 18000.00 O.8241 0.00248 0.45 m 035eo 0.130 2.S 0.89 0 8 017133 uOSSeo OA

- 4m-.-' 7-735. -25000-.00 :. 087934 ... ~ -os*'. 2 u4 403Wo0 2- 0 .8524... " iU i iR 0 ; *'0904.00 35 35000.00 OS03S4 0.08 014020 035go 517 T1A3 073 0.00242 0O9 w Sg40040

4.00 35 45000.00 _0755 0.0028 021 mO35ho O.510 1OAO 0.3905 oCoozu OA329 nh435ho 450

3.00 20 10000*0 09948 000218 52455 iuO2bo 0.72138 0.00 094 .00216 024555 nu32Obo 0*00003.00 20 14000.00 O.909 O.014 02475 n6302do 0.70133 11 090475 0. 2 02509 nOOdo OO

3.00 20 1000 007 .0204 24230 nu32o 08130 2Z8 0.100 0.00300 2882 3 o 0093

3.00 20 . 2 0- 0 02 so00. 0.e394 mz'O2Of 04525 . ii 0.00242 n3.00 20 35000.00 0775 0.01 023SU So 0917 713 0.983 0.00318 0451 tOo 00130

3.00 20 45000w*0 09408 00418 M23735 m t3 OS(1 100.00 014 .4327 nOOho 0* 0

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Vawn.,, Paoega vat~, 9"Al0en

Title: Simulating the Effect on Criticalty of Simultaneous Matrix Degradation and Assembly Collapsefor the 21 PWR Waste PackageDocument Identifier: CALEBS-NU- 02 REV 00 Page 20 of 30

Table 6-2. Reacity Evaluabon of Simuftaneous Matrbx Degradation and AssemblyCollapse

Enrlchmern Bup _AENCF FPL Collapse ICase I(w% U235) (GWdT) w 2 (MOV) ) I ) a

32Oaao: 3.00 20 0.R021 0.005 024083 0 0.00 03020abo: 3.00 20 0.897 0.07 0250 0 11.4 1 . 0444302Oaco: 3.00 20 0.88834 .44 027114 0 22. -0.0138530208do: 3.00 20 0U77 0044 03266 0 42.88 .0.024313020aeo: &00 20 0.83745 0.0027 0.37118 0 714 -004743020ahb: 3.00 20 0.797 0.00258 0A8549 0 100.00 -0.142923020bao: 3.00 20 0.02 0.0074 023759 11A3 0.00 0.00509S02Obbo: 3.00 20 0.9042 0.00268 025147 11.43 1.A3 0323020bco: 3.00 20 088 0.00242 026771 11A3 22.86 0.003763020bdo: 3.00 20 88706 029 0.30091 11A3 4286 .0.015133o20beo: 3.0 20 0.84516 0.00348 0.8887 1143 71.43 .0.057033020bfo: 3.00 20 0.76537 .0096 0.48038 1 A3 100.00 .0.13682302Ocao: 3.00 20 0.9151 0.0023 023607 22.86 0.00 0.01291302Ocbo: 3.00 20 001185 0.00196 024890 22.86 11.3. 0.009330200: 3.00 20 O93 0J00228 028387 22.88 22.86 0.00774320cdo 3.00 20 09484 0.00288 029725 22.8 42.88 :.o035S020ceo: 3.00 20 0.85174 0.00276 O.87 22.86 71A 0.050453020do: 3.00 20 0.7732 0.00298 0.47534 22.86 100.00 .0.128993020dao: 3.00 20 0M27 0.00296 0.23543 42.9 0.00 0.020513020dbo: 3.00 20 0M491 0.00274 0.24612 42.9 11.A3 .O022723020dco: 3 3.00 20 0.921 0.03266 0282 42.9 22.86 0.018813020ddo: &00 20 0.9099 0.00244 027 42.9 428 0.007773020deo: . 3.00 20 O.88818 OA068 0.3036 42.9 71.43 0.034013020dfb: 3.00 20 0.78912 0.00270 0.48849 42.9 100.00 .0.113073020eao: 3.00 20 094988 0.00256 022653 71A3 0.00 0.047673Q20ebo: 3.00 20 0.94823 0.00294 024076 71A3 11.43 0.048043020eco: 3.00 20 0.94893 0.00288 025248 71.A3 22.6 0.044743020edo: 3. 20 0.3497 O07 028711 71A3 42.86 0.032783020eeo: 3.00 20 0.893 0.00252 080 71.43 7tA3 -0.009193020oefo: 3.00 20 0.81187 0.00254 0.45823 71.43 100.00 .0.090323020fao: 3.00 20 0.97601 0.00258 0.22135 100 0.00 0.073823020fbo: 3.00 20 0.97392 0.00276 023494 100 11A3 0.07173302M0f: 3.00 20 0.97359 0.00306 024792 100 22.8 0.07143020fdo: 3.00 20 0.96038 0.00312 027983 100 42.86 0.058193O2Ofeo: 3.00 20 0.92103 0.00274 0.34198 100 71A3 0.018843020fo 3.00 20 0838 0.00Q84 U.44057 100 100.0 .006333

4035aao: 4.00 135 0.87686 0.00348 024338 0 0.00 04035abo 4.00 35 0.87492 I000302 025518 O 11.43 .O004

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-

.

Wattg Paeker nnisraflnnv Calcutline~a- - . f . .

Title: Simulating the Effect n Criticality of Simultaneous Matix Degradation and Asembly Collapsefor the 21 PWR Waste PackageDocument Identifier: CAL-EBS-NU-000002 REV 00 Pae 21 of 30

Table 6-2. Reactivt EvaluatIon of Simultaneous Matrx Degradation and AssemblyCollapse

Enrichmant BuInIp AENCF I FPL Colapse Case tot%1 5) (GW4m k j Z (MOV) (%) In c

4o3a: 4.00 35 0668 0.0054 027289 0 22.86 -O09438do: 40 35 0.84407 O03 0.31335 0 42.6 .031794035aeo: 4.0 35 M M 003 0.8 0 7143 4.07584035ab: 4.00 35 02499 0 0.6077 0 100.00 4.15W7403Sbao: 4.00 35 0824 02 024189 114 O0 MO0=4035bbo: 4.00 35 08189 0.002 025820 1A 1143 0.00634035bco: 40 35 0.86819 0.00328 0277 1143 228 -0.007674035bdo: 4.00 35 0.84986 0.00272 0.31202 11.43 42.86 -0264035beo: 4.00 35 0.81253 000328 038307 1.43 71.43 . 0.063334035blo: 4.0 35 0.73908 0 0026 0.49194 1.43 100.00 -0.13878=35cao: 4.00 35 0.89574 0.00322 024138 22.88 O.O 0.01988

40do: 4.00 35 0.9537 0.00294 025430 2286 113 0.019514035cco 4.00 35 0.8816 0.00288 027345 22.86 22. 8 0.00834035cdo: 4.0 35 0.8883 o0033 o 22.86 42.8 .0.0070343ceo: 40 35 0.82394 0.00344 0.37389 22.86 7143 -0.051924035do: 4.00 5S 0.74846 0.0032 0A9118 2288 100.00 4.12744035dao: 4.00 35 0.91255 OA0284 023662 42.9 00 0.03694035dbo: 4.00 35 0.91682 0.00286 0.242 42.9 1.43 0.039964035do: 4.00 35 0.9048 O.O058 026527 42.9 22.86 0030624035ddo: 4.00 35 0.87908 0.00286 00382 42 42.86 00x34035deo: 4.0 35 0.84197 0.O294 0.3573 42.9 71.43 .0.033894035dfo: 4.00 35 0.76791 0.00304 04303 42.9 100.00 .0.107954035eso: 4.00 35 0.94328 0.00278 022864 71.3 0.00 0.067424035ebo: 4.00 35 04076 0.0031 024208 71.43 11.A3 0.0644035eco: 4.00 35 0.93187 O.0028 025938 713 22.68 0M014035edo 4.00 35 09196 000274 029138 71A3 4288 0.043744035eeo: 4.0 35 0.87468 o0266 035808 71.3 71.43 4.001184035efo. 4.00 35 0.70494 0.00256 0.48596 71.43 100.00 4.080924035fao 4.0 35 0.979 0.0026 022015 100 0.00 0.103634035fbo 4.00 35 0.9764 0.00302 023309 100 1A3 0.099544035fc=o 4.00 35 0.97445 0.002U 024663 100 22.88 0.098594035fdo: 4.0 35 0.96187 0.0076 027614 100 42. 0.086014035feo- 4.00 35 .91677 032 0.34297 100 71A3 0.040914035ffo: 4.00 35 03295 0.0032 044631 100 100.00 4.04291454aao: 450 40 0.a3 0.0043 024202 0 0.00 04540abo: 450 40 087585 0.00328 025514 0 .11A3 4.007374540aco: 4.50 40 0.88737 0.00376 027197 0 22.86 0.015854540ado * 4.50 40 08448 000372 031176 0 428 4.03842

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Wnw#^ o prik nrvnf;n ^slenlt;nnTitle: Simaing the Effect on Criticality of Simultaneous Matrix Degradation and sly Collapsefor the 21 PWR Waste PackageDocument Identifier: CAL-EBS-NU.0OOD02 REV 00 Page 22 of 30

Table 6-2. ReactvIty Evaluation of Simultaneous Matrix Degradation and AssemblyCollapse

Enrchment mup I Il I AENCF FPL IColapselCase (wt U-235) (WdJT) j_ 20o (MOV) 4%) [%) 6k

4540seo: 4.50 40 0.80341 0.0034 0.8390 0 713 -.. M7814540Saf 4.5O 40 o.m276 0.00348 0A9870 0 100.00 .0.15#84540bao: 4.50 40 0.94 . 0.00316 024048 1A3 0.00 0.007184S40bbo: 4.I0 40 0.88711 0.00372 025825 11.43 11.43 0.003894540boo: 4.60 40 0.88601 00034 026774 11.A3 22.88 0.00O274540bdo: 4.60 40 O5572 0.00352 0074 s13 42.86 0.02764540beo 4.60 40 08124 0.00398 o.m53 t1.A 71A3 0.070824540b60: 4.C0 40 0.74004 0.00328 .902 11.A3 100.00 *0.143184S4Omo: 4.50 40 0.90395 0.00406 023400 22.86 0.00 0.020734540cbo: 4.50 40 0.90054 0.00292 024939 22.8 AS 0.01732440cco: 4.50 40 0.89134 0.00316 026629 22 22 2286 0.008124540cdo: 4.50 40 0.87262 0.0030 30071 22.86 42i6 - 0.01064540ceo 4.50 40 .8563 000308 072 22.86 7143: .0.057594540do: 4.60 40 0.7498 0.00348 Q48670 22.86 100.00 .0.133424540dao: 4.5D 40. 0.91819 020 02332 42.9 0.00 0.034974540dbo: 4.50 40.- 0.9153 0.00330 024811 42. 11A3 0.032314540dco 4.50 40. 0.913 0.00358 026363 42.9 22.86 0.029784540ddo: 4.50 40 0.89357 0.00354 029618 42.9 42.86 0.010354540deo: 4.60 40 0.84152 0.00324 0.36605 42.9 71A3 .0.04174540dfo: 4.50 40. 0.76986 0.00346 0.47709 42.9 100.00 0.113364S40eaeo 4.60 40 0.95989 .00364 022425 71.3 0.00 0.076674540ebo 4.50 40 0.95205 0.00288 024043 71A3 11.3 O68834540eco: 4.50 40 .4811 0.00306 025294 71.A3 22.88 0.064894540edo: 4.60 40 0.92473 0.00292 028479 71.3 42.6 0.041514540eeo: 4.50 40 0.8831 O.O07 0.35276 71.43 71.A3 *0.000124540efo: 4.50 40 0*013 0.00338 0.45987 71.3 100.00 .0.081924540fao: 4.60 40 0.99W 0.0024 021681 100 0.00 0.109054540tbo: 4.60 40 0.99148 0.O2 022990 100 11.3 0.108264540fco: 4.50 40 0Q887 0.0028 024262 100 22.68 0.105484540ftdo: 450 40 0.6699 0.0027 0277 100 42.B 0.083774540feo: *.50 40 0.92047 0.00316 0.33767 100 71.43 0.03725454ff o: 4.50 40 0.84063 0.00258 0.44114 100 100.00 0.04259

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RVU-4a- Da tn fl nno4

fh fPai.,,Ia4;rnVW X% A dPLJf UUj_- IIIWA .0

tle: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and Assembly Collapsefor the 21 PWR Waste PackageDocument Identifier: CAL-EBS-NU.0002 REV 00 Parc 23 of 30

Table 63. Regression Resuts of Ak as a Funclion of Fission Product Loss and AssemblyCollapse

Enruichment Bumup Intercept % FPL % Collapse(wMU-2 (GWd)

3.0 20 0 0.00090428 .0.0012381

4.0 35 0 0.0011859 .0.0013417

4.6 40 0 0.0012478 .0.0014189

Average 0 0.0011127 .. 001332

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Waste Paclaze Onerations - - ~~~~~~~~~~~. CculationTitle: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and Assembly Collapsefor the 21 PWR Waste PackageDocument Identifier: CAL-EBS-NU-0MO2 REV 00 Page 24 of 30

7. ATTACHMENTS

Attaclments to this document are listed in Table 7-1 below.

Table 7-1. LstofAttachments

Attachment DescriptionNumber

I Document Input Reference Sheets (DIRS)

nI CD-ROM Cntainingte Input and Out Fles for the MCNPuIculstions.

The following supporting documents listed n Table 7-2 are in electronic form on a CD. Each file isidentified by its name, size (in bytes), the date and time of last access. Note that for files transferredfrom the Hewlett-Pacard to the Personal Computer, the date and time will reflect the time of trander.The actual date and time of run completion can be found in the file.

Table 72. List of Fies in Altachment II

Foe Name Date Time Size.__ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ (bytes)

u3020b 082499 02:48 PM 44,372Ci530ow- 08124)9 02.49 PM 699,267

u ad 0124/99 02:49 PM 4,835UiX3020do 0824199 02:49 PM 692,466mz3020e 0 499 02:49 PM 42,718nu302Oeo 0814)99 02:49 PM 678,408n3020f 0884/9 02:49 PM 42,720

nu3020fo 0824/99 02:49 PM 678,328m:3020g -0824199 02:49 PM 42,701uu3020go _ 081499 02:49 PM 678,508m3020h 08124)99 02:49 PM 42,710nu3020ho OJ24199 02:49 PM 678,369nu4035b OV24199 02:49 PM 44,394nu4O3Sbo MUM 02:49 PM 699,206nu4035d 08124199 02:49 PM 43,832nu4O3Sdo 0812499 02:49 PM 692,553uu403Se 084/99 02:49 PM 42,675nu403$co 0824/99 02:49 PM 678,321ou4035f 08124/99 02:49 PM 42,712=u403Sfo 0&499 02:49 PM 678,529u403Sg OV12499 02:49 PM 2,728

nu4035go 0824f9 02:49 PM 678,707nu403Sh 0884199 02:49 PM 42,706nu403Sho 0824199 02:49 PM 678,360im4$40b ii747 02:49 PM 44,377nu4S40bo 0&4/99 02:49 PM 699,206DU4540d OU24f99 02:49 PM 43,856nu4S40do 08M24)99 02:49 PM 692,S08

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.Wade Package Operations CalculationTitle: Simulatg the Effect on Criticality of Simultaneous Matrix Degradation and Assembly Collapsefor the 21 PWR Waste PackageDocument Identifier, CAI-EBS-NU-00002 REV 00 Page 25 of 30

---l~c Narnt Date Time She_ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ ~(byt s)

=n4S40c 08W4199 02:49 PM 42,735ru4S40eo 084bUst 02:49 PM 678,622nu4S40f 08r2/99 _ QQ:49 PM_ 42,732nu4S40fo GUAMg9 02:50 PM 678,538nu4540g ftt24__9 02:50 PM 42,747nu4S40zo M MSUU59 02:50 PM 678,408nu4S40h CF224U9i 02:50 PM = 42,759u4S40ho 0 F2:50 PM 676,408w3mw 0V24M 03:26 PM 45,313

ru3020do OW2419 03:26 PM 624,498su3020c OW224/99 333 PM< 4,15_

ru3020co 024/99 0333 PM 609,476nu32f OM S 03:33 PM 44,121

* ni3S2Ofo 082499 03:33 PM 608,428ru3 Oat" 03:33 PM - 44,121ru02g OU2419 03:33 PM WOMru3020h 009709 03:27 PM 34,020ru302Oho 0824/99 1 03 27 PM 488,177MOM____2 P499 03:27 PM 4S313_ _

n4O3Sdo 03:27 PM 624,443ni403Sc 08*4199 03:33 PM 44,125ru4O35eo V2499 03:33 PM 609,517wr4033 0884/99 03 33 PM 44,121

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ru4S40do O08W 03:27 PM 624w_ _ 0824199 03:34 PM 43,388

zu4S40eo 0 99 03:34 PM 609,610ru4540f OV24199 0334 PM 43,383MUM________ 0V24/99 03:34 PM 608,494u4540g 08099 03:34 PM 43,383454jo- 0 03:34 PM 606903u4S40h II24/99 03:28 PM 33 211u4S40ho 08 9 03:28 PM 48,2233020aa 08/24199 03:01 PM 42,7193020aao 024f99 03:01 PM 61129930Qs 08n499 03:01 PM 42,9073020abo 0824/99 03:01 PM 610,5273020ac 08849 03:01 PM 42,9073020aw 0824/99 03:01 PM 6095693020ad OW24/99 03:01 PM 429033020ado 0__499 03:01 PM 60,5693020ae 0824/99 03:01 PM 42,9033020a 0849 03:01 PM 607.1323020af W-24-99 03:01 PM 42,9033Q20afo 08f2U99 03:01 PM 605,249

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Waste Package Operations - Calculation'Title: Simulating the Effect on Criicality of Simultaneous Matrx Degradation and Assembly Collapsefor the 21 PWR Waste PackageDocument Identifier; CAL-EBS-NU-0002 REV 00 Page 26 of 30

Foe Name Date Time sin_ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ ~~~~ ~~~(bytes)

302Oba 02/ 03:01 PM 43,9383020bao 0L?4l99 03:01 PM 611,4903020bb Of1 03.01 PM 44,12S3020bbo a 4199 03:02 PM 610,3933QQ0bc ouml 0)3.02 PZ- 4412 -3020bo__ 03.02 PM 609,0073020W 08D4199 ~ 03-02 PM 44,1213020bdo MUMW9 03:02 PM 607,9573020be _ V24/U99 03-02 PM 44,121

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3Q20cfo 0824/99 03:02 PM 605,2983024da 0824f99 03:31 PM 44,121

3020dao O-24J99 03:31 PM 608,9523020db 012499 03:31 PM 44,121

3020dbo 084f99 03:32 PM 610,44030Q0dc 08f24f99 03 32 PM 44,121

3020dco O2499 03-32 PM69,S33020dd 0824/99 03.32 PM 44,119

3Q20ddo 08f2499 03:32 PM 608,4763020dc 08t2499032 PM 44,119

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3020cfo 084199 03:03 PM 605,2023024h 08f24)99 03.03 PM 33,839

3020fao 08f24f99 03:03 PM 494,127

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Tile: Simuling the Effect on Criticality of Simultaneous Matrix Degadation and Assembly Collapsefor the 21 PWR Waste PackageDocument Identifier: CALBS-NU-000002 REV 00 Page 27 f 30

File me Date Time Sie__ _.__ .___ _ ,___ (b*1e)

3020Ft 02W499 03:03 PM 34.0273020fbo 081499 0304 PM 493,6793020Sc 081249 03:04 PM 34,0273020foo 0 M" 03:04 PM 492,6673020(d RPIiM* 03.04 PM 34,023302"fdo 084799 03:04 PM 491,7143020fe 08a4M 03:04 PM 34,024

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Waste Packlne Opnrations CalculationTitle: Simulating the Effect bn Criticality of Simultaneous Matrix Degradaion and Assembly Collapsefor the 21 PWR Waste PackageDocument Identifier: CAL.EBS-NU-000002 REV 00 Page 28 of 30

File Name Date Time Sie_ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ ~~~~(byte)

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403Scao 0I41F9 03.06 611,443403Seb 08/24/99 0306 PM 44,12S403Sebo OV4/99 03.06 PM 610,44S4035ec iU24l9 03:06 PM 44,125

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403Seeo - 499 03:07 PM 606,9S0403Sef 024199 0307 PM 44,1214035efo 0J299 0307 PM 605,2394035fiL 0 03:07 PM 33,8394035ho 2499 307 PM 494,2564035fb OFRW99 03:07 PM 34,027403Sfbo 08124/99 03:07 PM 493,6264035& 08249 0307 PM 34,027403_f_ o _24_99 03 07 PM 492,714403Sfd OVU24"9 03 07 PM 34,023403Sfilo __ 0 _ 03:07 PM 491,666403Sf;: O24/99 03:07 PM * 34,023403Sfco 2499 03:07 PM 490,094403Sff 0824/99 03.07 PM 34,0234035ffo 0824199 0307 PM 488,0814S40aa _ 08PU99 03 07 PM 42,731

4S40aao W81249 03_07 PM 611,5614540b - 124M 03:07 PM 42,9194S40abo 024/99 03:07 PM 610,6964S40ac 024/99 03:07 PM 42,919

4S40aco 08)24/99 03:07 PM 609,6884S40ad 0n4/99 03:07 PM 42,9114540sdo GLIU 03:07 PM 608,6154S40ae - 0_99 0307 PM 42,911

4S40seo 08nu99 03:07 PM 607,0434540af 081V - 03:07 PM 42,9114340afo 024199 03:07 PM 605,3424540ba 024/99- 03:07 PM 43,937

4S40bao 08499 03:08 PM 611,2514540bb 084/99 03:08 PM 44,125.4S40bbo GVFV 99 03:08 PM 610,2904S40bc 084l99 03:08 PM 44,125

4S40bco _ _24_99 .03:08 PM 609,474

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Waste Package Operations Calculation.Title: Simulating the Effect on Criticality of Simultaneous Matrix Degradation and Assembly Collapsefor the 21 PWR WastePacageDocument Identifler CAL4BS-NU-00O02 REV 00 Page 29 of 30

file Name Dte Time Sie_ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ _ ~~~~(bytes)

4540bd 08/2499 0308 PM 44,1174S40bdo 08499 03:08 PM 608,541.T540be W4i99 0308 PM 44,1174540beo 0&249 03.08 PM 64540bf 08n4 0308 PM 44,1174540bfo P24/9 - 0308 PM 6Q5,2494540c _4_99 _0___OR PM 43,9374$40cw OM/99 03:0 PM 611,34144kb 0W4s9 0308 PM _ 44,125*1340** ~0= 9 03:08 PM 610,4384S40cc 20894N9 03:08 PM 44,1254S40cco n124i99 03.08 PM 60,S294S4odd 0 49 03:08 PM 44,1174S4do nif799 03:08 PM 608,4744540ce OV24/99 03:08 PM 44,117

4S40cc OV24/99 03:08 PM 606,902* S40d 0 n i*M 03:08 PM 44,117

4540cfo 084199 03:08 M 605,0517=4S40da =_ .0&8/2499 03:32 PM 43,3854S40dto 0VW 03:33 PM 1,1W34S40db 0847/99 03:33 PM 43,355S40do O 4/99 03.33 PM 610,3914W40dc UMT~w9 03:33 PM 434S40dco 0&4199 03.33 PM 609,S69454W iM49 03:33 PM 43,3834540ddo 082499 03:33 PM 608,4264540de 0804199 0333P 433834S40deo 0V24199 03 33 PM 606,9564S40df 08499 03.33 PM 43,3834S40tfo 024/99 03:33 PM 605,18S4S40ca 0812499 03:08 PM 43,937

4540eao 08124199 03:08 PM 61 1,3464S40eb O W24/99 03:08 PM 44,125

. 4S40ebo 08f 03:08 PM 610,4934540ec 0824/99 03:08 PM 44.1254 4S40eco- 0 03.09 PM 609,7384S40ed 0 03:09 PM 44,1174540cdo 0U24199 03:09 PM 608,4274540ce 0814199 03:09 PM 44,1174S40eo M M 03:09 PM 606,9084S40f 03:09 PM 44,1174S40efo 099 03.09 PM 605,1524540fa 08499 03:09 PM 33,8394S40io U2499 03:09 PM 493,6614340fb 0&24 03.09 PM 343 f 0iJ2 03:09 PM 493,3194 v40fb 08199 0309 PM 34,0274540fco 0249 03:09 PM 492,655440d 0 03:09 PM 34,0194S40fdo 08VWtg9 03.9 PM 491,714

6.

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Waste Package Operations CalculationTitle: Simulating the Effect on Criticality of Simultaneous Matix Degradation and Assembly Collapsefor the 21 PWR Waste PackageDocument Identifier CAL-EBS-NU-000002 REV 00 - Pac 30 of 30

LE Name Date Time Size)(bye)

S40fe 08&2499 03:09 PM 34,0194340feo 824199 03019 PM 490,0414I 3 0 8 03:09 PM 34,0194S40o 0 8 03:09 PM 488,122

Page 32: OFFICE OF CIVILIAN RADIOACTIVE WASTE SPECIALDocument Identifier, CA-EBS-NU0002 REV 00 Page 6 of 30 hZN'g. Sw t Mflu. O w (L100J0 .0000 . W100) aim WI000 MM000W. .10000 giuFe 1 5 1o

Waste Psekne Ofions CalculationsTide: Simulating the Effect an Criticality of Sinmltao Matrix Degradation and Asembly Collapse for te 21 PWRWage PackageDPocument Identifer: CAL-EBS-NU0002 REVO Attnehmentl Pae1 of 3

OFFICE OF CIUAN RADIOACTIVE WASTE MANAGEMENTDOCUMENT INPUT REFERENCE SHEE

1. Doax Wler w AWev Chu TOb:

CAL-EBS-NU-000002 REV 00 N/A Simulating the Effect on Citiclity of Simultaneous Madrix Degradation and Assembly.____________ _ JColpse for te 21 WR Waste Packe

2. TecMlca Pdi~~ a lThe Sd 2. Cen .d hp4, 0 U. hl ?.IWIUD - p,* fnMmUrc Un.2 M oddasftw WA go" M VW Stbtim Ued inN ame amfamed

2a CRWMS M&O 1999. DPfor Entire N/A 1 Developmentplan; N/A N/A N/A N/A

1 Simlnaing the Effect on CrifcaItfy of Reference, not an inputSfmutaneous Mairk DegradationandAsebb yCollqpse. TDP-EBS-NU00000QREV00. Las Vegas,Nevada: CRWM M&O. ACC:MOL19990824.0146.

2 CRWMS M&O 1998. Software Entire N/A 2 SQR; Reference, rot an N/A N/A N/A N/AQualification Repartfor ACNP 4.1 iV4B2. 30033-2003 REV 01. LasVegas, Nevada CRWMS M&O.ACC: MOL.19980622.0637.

AP-3.150.1 Rev. 0=6001999

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,n 9 i..WtVAMC rpeiZce tnon_ uiunn

Tft!e Simu g thc Efdc on Criily of Simuftaeous Mtix Dgdaton and mbly Collpse for tbe 21 PWR Waste Pgejiocument Identifier CAL-EBS-NU-0002 REV 00 Attaelment I Pae 2 of 3

OFFICE OF CMUAN RADIOACTIVE WASTE MANAGEMENTDodIJMENT INPUT REFERENCE SHE&

1.DomultetNoJRev.

CAL-ES-NU-000002 REV 00 IN/A Simati o Effec o Cidctality of Sim es Merix Dcgad and AssemblyCollapse for the 21 PWR Waste Package

bhtV 1 OoaM _D TV Ous Tc

2. Tedm~IPu 1 Tlb rd a. s.n 4T htL 6. Selon 6 P4*uD.ObaC 7 .TDO F, n Urn-Todw_101Pn Used oufiSW

3 CRWMS M&O 1998. Sqlemertal Enti TBV- 2 MCNP CLIOs 3 Yes N/ . N/ACftlcalfty Evaluationfor Degraded 3376 3 calculation of wmbernernal Colfguratlons of a 21 PWR densitiesWaste Package. BBAOOOO Based on unqualified dat.01717-0210-0002 REV 00. Las 5VeMgasNevadw CRWMS M&O.ACC: MOL.19980918.0086.

4 CRWMS M&O. 199& Cntrolled yR TBV- 3.1 Basis for an assumptin 3 Yes N/A N/ADesign Assuwptions Document. 009 3377B00000000-01717-4600w0002 REV05. Ls Vegas, Nmvda: CRWMS wACC. M&;O. MOL.1998u8u4.0481.

AP-.150.1 Rov. 00t'19

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1Waste Package Oneratons CalculationsTide: Simulating the Effect on Criticality of Simultnous Matrix Degadation aud Assembly Collapse for he 21 PWR Waste PacagDoeymentIdenfller CALEBSN000002 REVOO Attachment IPae 3 of 3

OFFICE OFCIVIIAN RADIOACTIVE WASTE MANAGEMENTDOUMENT INPUT REFERENCE SHEET

1. Doun WWntJerNJsv2 Th Ift

CAL-EBS-NU-00002 REV 00 N/A Simulating 1he Effect on Criticality of Siultaneow Matrix Degradation nd Assembly.__ _ _ __ . Collapse for the 21 PWR Waste Package

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5 CRWMS M&O 1997. Disposal p. 3-26 TBV. 32 Basisforamassumption 3 Yes N/A N/Aarffcat Anaysk Methodology 3378TechicalReport B000O00-01717-5705-00020 REV 01. LasVegas, Nevada: CRWMS M&O.AC: MOLI9980108.0700.

6 CRWMS M&O 1998. EQ6 5 TBV- 5.1.5 Basket and Fud 3 Yes N/A N/ACalculatfons for Chemca 3379 Degradion PodutDegradation ofPWR LEUanwdPWR CompositionsMOXSpew Fuel Waste Packages.BsdO'wplfe aaBBAOOODOO01717-0210-0009.REV 00. Las Vegas, NevadaCRWMS M&O. ACC:MOL19980701493.

AP-3.150.1 Rev. o U999