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1/16 System for Prediction of Environmental Emergency Dose Information Multi-model Package International Workshop, Feb. 22-23, 2012 Source term estimation and atmospheric Source term estimation and atmospheric Source term estimation and atmospheric Source term estimation and atmospheric dispersion simulations of radioactive materials dispersion simulations of radioactive materials di h df th Fk hi D ii hi di h df th Fk hi D ii hi discharged from the Fukushima Daiichi discharged from the Fukushima Daiichi Nuclear Power Plant due to Accident Nuclear Power Plant due to Accident Haruyasu NAGAI, Masamichi CHINO, Hiroaki TERADA, Genki KATATA, Hiromasa NAKAYAMA, and Masakazu OTA J At i E A Japan Atomic Energy Agency

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Page 1: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

1/16System for Prediction of Environmental Emergency Dose Information Multi-model Package

International Workshop, Feb. 22-23, 2012

Source term estimation and atmosphericSource term estimation and atmosphericSource term estimation and atmospheric Source term estimation and atmospheric dispersion simulations of radioactive materials dispersion simulations of radioactive materials

di h d f th F k hi D ii hidi h d f th F k hi D ii hidischarged from the Fukushima Daiichi discharged from the Fukushima Daiichi Nuclear Power Plant due to AccidentNuclear Power Plant due to Accident

Haruyasu NAGAI, Masamichi CHINO, Hiroaki TERADA,Genki KATATA, Hiromasa NAKAYAMA, and Masakazu OTA

J At i E AJapan Atomic Energy Agency

Page 2: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

Development of SPEEDI-MPSimulations in the multiple environments

2/16

Changes and needs of the society• Advance in nuclear fuel cycle, increase of nuclear facilities in East Asia, and so on

Diversification of nuclear activities and complication of release conditionsDiversification of nuclear activities and complication of release conditions• General environmental problems: global warming, water cycle problems, and so on

To be solved by applying any kind of science and technology

Simulation for elucidation of the behavior f t i l i th lti l i t

Expansion of SPEEDI

of materials in the multiple environments

Atmospheric model(SPEEDI)Dispersion, Transfer WSPEEDIWSPEEDI--ⅡⅡ(SPEEDI)

Exchange of heat, materials and so on

Mixing, depositionApplication to Fukushima Daiichi

Nuclear Power Plant Accident

Leaching

Flowing-out

Mixing, Settling

Transfer

Leaching

Terrestrial model Oceanic model

g g

Page 3: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-ⅡModel structure of WSPEEDI-Ⅱ

3/16

C l l ti d MM5

Global meteorological forecast by JMA (GPV)

Global geographical database

Regional meteorological modelWind, turbulence, cloud, rain, etc.

Calculation code: MM5MM5MM5

LocalRegionalWind, turbulence, cloud, rain, etc. LocalRegional

Incorporated in ver. 2To improve meteorological predictions

Source term

3-D meteorological fieldTo improve meteorological predictions,diffusion and deposition processes

Particle dispersion modelAi t ti d iti d

GEARNGEARN

Source termCalculation code: GEARN

Air concentration, deposition, dosesLocalRegional

Air concentration, deposition, dosesRegional and local calculationsat any place of the world

Page 4: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-ⅡNesting calculations

4/16

【MM5】2-way nesting up to 5 domains: select arbitrary 2 domains

MM5 domain

Off-line or on-line coupling【GEARN】2-way nesting for 2 domains: exchange input/output data via MPI2-way nesting for 2 domains: exchange input/output data via MPI between 2 model domains separately executed as parallel tasks

GEARN domains

Flow in/out between

Coupling

Flow in/out betweenlocal and wide domains

Page 5: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-ⅡApplication to Fukushima NPP accident

5/16

【Source term estimation】Collaboration with the Nuclear Safety Commission (NSC) of JapanEstimation by coupling monitoring data with atmospheric dispersion simulationsEstimation by coupling monitoring data with atmospheric dispersion simulations⇒ M. Chino, et al., 2011: J. Nucl. Sci. Technol., 48,1129–1134

Available from (http://www.jstage.jst.go.jp/article/jnst/48/7/1129/_pdf)

Re-estimation of release rate from 12 to 15 March (Report to NSC on 22 Aug.)(http://www.nsc.go.jp/anzen/shidai/genan2011/genan063/siryo5.pdf, in Japanese)

【Analysis of atmospheric dispersion】Analysis on the local dispersion during significant release (15 to 16 March)- Formation process of high dose rate zone around the northwest region of the plantp g g p⇒ JAEA News Release (http://www.jaea.go.jp/english/jishin/press/press110613.pdf)

G. Katata, et al., 2012: J. Environ. Radioactiv., (in press)Available from (http://www.sciencedirect.com/science/article/pii/S0265931X11002335)Available from (http://www.sciencedirect.com/science/article/pii/S0265931X11002335)

Preliminary estimation of 2-month accumulated radiological doses over Japan⇒ JAEA Technical Report (http://www.jaea.go.jp/english/jishin/kaisetsu03.pdf)

2000

Analysis on the deposition process of 137Cs over Eastern Japan area⇒ JAEA Technical Report (http://nsed.jaea.go.jp/fukushima/data/20110906.pdf, in Japanese)

Page 6: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-Ⅱ source term estimationMethod and data for source term estimation

6/16

SPEEDI domainSimple source estimation method

CalculationU it l (1 B /h)

MonitoringC t ti

d

fgjh

iUnit release (1 Bq/h)

Dilution factor

Concentrationand

Air dose rated

c,eh

No. Sampling date and time Point1 2011/3/15 06:00-07:00 a2 2011/3/15 06 55 07 15 b

ComparisonMonitoringRelease rate b Tokai

(JAEA)

2 2011/3/15 06:55-07:15 b3 2011/3/16 06:05-06:25 b4 2011/3/18 10:50-11:18 c5 2011/3/21 04:45-05:05 b6 2011/3/21 10 50 11 08 d

gRelease rate = Calculation

a Chiba(JCAC)

6 2011/3/21 10:50-11:08 d7 2011/3/22 14:17-14:31 c8 2011/3/23 13:15-15:10 e9 2011/3/24 14:55-15:15 f

10 2011/3/25 15:05 15:22 g

[Preliminary estimation](M. Chino, et al., 2011:

10 2011/3/25 15:05-15:22 g11 2011/3/27 11:45- h12 2011/3/29 11:17-12:15 f13 2011/3/30 15:11-15:32 g14 2011/3/31 12:22 13:12 e

WSPEEDI domain

(JNST, 48,1129–1134)

(M. Chino, et al., 2011: JNST, 48,1129–1134)

14 2011/3/31 12:22-13:12 e15 2011/4/1 12:00-12:20 i16 2011/4/3 11:04- j17 2011/4/5 13:07-13:27 f

Page 7: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-Ⅱ source term estimationMethod and data for source term estimation

7/16

[Re-estimation]Release rate from 12 to 15 March by using newly released data(Report to NSC on 22 Aug.)

Environmental monitoring points used for the estimation of release rates on March 13

Environmental monitoring points used for the estimation of release rates on March 12the estimation of release rates on March 12

Page 8: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-Ⅱ source term estimationPreliminary and re-estimated results

8/16

Preliminary estimated release rates of 131I & 137Cs (M. Chino, et al., 2011: JNST, 48,1129–1134)- Total release amount from 11 March to 5 April 131I:1.5×1017 Bq 137Cs:1.2×1016 Bq

Re-estimated release rates(http://www.nsc.go.jp/anzen/shidai/genan2011/genan063/si

Correspond to H2 explosion at Unit 3 Correspond to H2 explosion at Unit 1

ryo5.pdf)

p 2 p(assumed to be same as Unit 1)

p 2 p(assumed 30 min release)

Page 9: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-Ⅱ local analysisFormation process of high dose rate zone

9/16

Analysis on the formation process of high dose rate zone in the northwest gdirection of the plant and the middle part of Fukushima PrefectureN i l i l ti f thNumerical simulations of the atmospheric dispersion of radioactive materials discharged from the plant g pduring the period from 15 to 16 March

Results of airborne monitoring by MEXT and DOEReport of Japanese Government to the IAEA Ministerial Conference on Nuclear Safety- The Accident at TEPCO's Fukushima Nuclear Power S iStations –(http://www.kantei.go.jp/foreign/kan/topics/201106/iaea_houkokusho_e.html)

Page 10: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-Ⅱ local analysisCalculation conditions

GEARN d i

10/16

JMA-GPV(MSM) MM5 domainDomain 1

Domain 2

GEARN domain

MM5 calculation

Domain 1

Domain 2 1FCorrection of data assimilation

Comparison with met. observations

on o

f m

ilatio

n

Domain 3

GEARN calculation Correction of

t

Cor

rect

ioda

ta a

ssim Domain 3

Analysis and observational nudging:AMeDAS data, Wind data at 1F and 2F

3 d i t 9 k (D1) 3 k (D2) 1 k (D3)Comparison with

radiation monitoring

source term

3 domain nest: 9 km (D1), 3 km (D2), 1 km (D3)Period: 17JST on 14 to 00JST on 17 March 2011Radionuclide: 131I, 132Te (+132I), 134Cs, 137Cs

radiation monitoring

Reconstruction of the Release rate: Correct the initial condition based on Chino et al. (2011) to fit monitoring data

Reconstruction of the atmospheric dispersion

Page 11: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-Ⅱ local analysisDistributions of air dose rate, conc., rain

11/16

Calculated concentration and rainRain intensity: shaded areaV i l l d d

Air dose rateCalculation: shaded areaM i i l i h lVertical accumulated conc.: red contours Monitoring: plot with values

Page 12: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-Ⅱ local analysisFormation process of high dose rate zone

12/16

30

40

50

60

Sv h

‐1

Calc. Obs.

Fukushima Obs.Calc.

μGy h‐

1

10

15

20

25

μ Sv h‐1

Calc. Obs.

Minami-soma Obs.Calc.

Gy h‐

1

15 MarPM

Air dose rate (21JST on 16 March)

0

10

20

3/15 0

0:0

0

3/15 0

6:0

0

3/15 1

2:0

0

3/15 1

8:0

0

3/16 0

0:0

0

3/16 0

6:0

0

3/16 1

2:0

0

3/16 1

8:0

0

3/17 0

0:0

0

μ Sμ

0

5

10

3/15 0

0:0

0

3/15 0

6:0

0

3/15 1

2:0

0

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8:0

0

3/16 0

0:0

0

3/16 0

6:0

0

3/16 1

2:0

0

3/16 1

8:0

0

3/17 0

0:0

0

μGPM

20

25

Calc. Obs.

KoriyamaObs.C l1

50

60

Calc. Obs.

IitateObs.Calc

15 MarAM0

5

10

15

0 0 0 0 0 0 0 0 0

μSv h‐1

Koriyama Calc.

μGy h‐

1

0

10

20

30

40

μ Sv h‐1

Iitate Calc.

μGy h‐

1

Marks (○) and values:i i l

3/15 0

0:0

0

3/15 0

6:0

0

3/15 1

2:0

0

3/15 1

8:0

0

3/16 0

0:0

0

3/16 0

6:0

0

3/16 1

2:0

0

3/16 1

8:0

0

3/17 0

0:0

0

2

3

4

μ Sv h‐1

Calc. Obs.

TamuraObs.Calc.

μGy h‐

1

3/15 0

0:0

0

3/15 0

6:0

0

3/15 1

2:0

0

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8:0

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0:0

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6:0

0

3/16 1

2:0

0

3/16 1

8:0

0

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0:0

0

10

15

20

25

μ Sv h‐1

Calc. Obs.Kawauchi Obs.Calc.

h‐1

μGy h‐1

monitoring values0

1

3/15 0

0:0

0

3/15 0

6:0

0

3/15 1

2:0

0

3/15 1

8:0

0

3/16 0

0:0

0

3/16 0

6:0

0

3/16 1

2:0

0

3/16 1

8:0

0

3/17 0

0:0

0

μ

0

5

3/15 0

0:0

0

3/15 0

6:0

0

3/15 1

2:0

0

3/15 1

8:0

0

3/16 0

0:0

0

3/16 0

6:0

0

3/16 1

2:0

0

3/16 1

8:0

0

3/17 0

0:0

0

μμG

◆A B

◆: near main gate

■: near west gate

▲: near gym.

era

te(μ

Sv/h

) A B

Air dose rate at theFukushima Daiichi NPP

Rapid pressure decrease in Unit 2Period A: 7 to 11 JST on 15 Mar.

Air

dosFukushima Daiichi NPP

Period B: 13 to 15 JST on 15 Mar.

Page 13: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-Ⅱ regional analysisDeposition of 137Cs over eastern Japan

13/16

■Domain: (Horizontal) 690 km × 960 km(vertical) 10 km

■Resolution: 3 km grid

■P i d 05JST 12 M h 24JST 30 A il 2011Local Domain 3■Period: 05JST on 12 March to 24JST on 30 April 2011

■Input meteorological dataJMA GPV(MSM) 3 h i l 1

Domain 3

・JMA-GPV(MSM): 3 h interval・AMeDAS data, Wind data at 1F and 2F

■R l

1F

■Release rate・Chino et al.(2011) + re-estimated source term・Assume that the release rate on 5 April continue until the end of calculation period

Validation of the estimated source term

Page 14: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-Ⅱ regional analysisFormation process of 137Cs deposition

14/16

Deposition until the end of March Airborne monitoring of 137Cs deposition by MEXT

Comparison with monitoring data:

20 Mar.Wet depo.monitoring data:

monthly depositionp

OverestimatedUnderestimated12 Mar.Dry depo.15 Mar.

Wet depo.15 Mar.Dry depo.

p

21 Mar.

Bq m-2

Wet depo.

Page 15: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

WSPEEDI-Ⅱ regional analysisComparison with measured 137Cs deposition

15/16

137Cs daily deposition

Factor 2 39 0 %Factor 2 39.0 %Factor 5 69.5 %Factor 10 86.4 %ac o 0 86. %Correlation coefficient 0.72

This result indicates the validity of estimated source term.

Page 16: Source term estimation and atmosphericSource term ...€¦ · System for Prediction of Environmental Emergency Dose Information 1/16 Multi-model Package International Workshop, Feb

Summary and future work 16/16

Activities during the Fukushima Daiichi nuclear accidentSource term estimation by coupling environmental monitoring data with t h i di i i l ti b SPEEDI/ WSPEEDIatmospheric dispersion simulations by SPEEDI/ WSPEEDI

Prediction of air concentration, deposition and radiological doses by WSPEEDIprovided to the Japanese government, local authorities, etc.

In present, prediction of oceanic dispersion by coupling oceanic dispersion model with WSPEEDI to consider the fallout to sea surface

Future workC li f t h i i

(Left) Predicted depositionof 137Cs until 31 March(Below)

Coupling of atmospheric, oceanicand terrestrial transport modelsDose evaluation modeling in

( )Example of predictedoceanic dispersion

contaminated circumstances