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THE ABC’S OF RADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, [email protected]

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Page 1: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

THE ABC’S OF RADIOACTIVITY

Physics of Atomic Nuclei - Lecture 3

Peggy Norris, [email protected]

Page 2: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

WHAT IS RADIATION?

Radiation is energy released after being stored in atoms Radiation can be natural or man-made Radiation can be in the form of particles or

electromagnetic radiation When radiation comes from the nucleus of an atom it is

called radioactivity

We will be focusing on ionizing radiation and its health effects.

Page 3: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

ATOMS

… are made of

Electrons and the Nucleus

Electrons

… are very light but take up most of the space in an atom

The nucleus

… lies at the center of the atom, has almost all of the mass but takes up almost none of the space inside an atom

Page 4: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

THE NUCLEUS

The number of protons in a nucleus is equal to and determines the number of orbiting electrons• determines the chemistry• determines the element name

An atom is electrically neutral (# of protons (q=+1) = number of electrons (q=-1))

An ion is a charged atom; can be positive (electron removed) or negative (electron added)

Page 5: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

ISOTOPES

•Uranium-238 (238

92U)

92 protons, 146 neutrons, mass 238

•Uranium-235 (235

92U)

92 protons, 143 neutrons, mass 235

•Hydrogen (11H)

1 proton, 0 neutrons, mass 1

•Deuterium (21D)

1 proton, 1 neutron, mass 2

•Tritium (31T)

1 proton, 2 neutrons, mass 3

•Helium (42He) (a-

particle)

2 protons, 2 neutrons, mass 4

•Helium-3 (32He)

2 protons, 1 neutron, mass 3

Page 6: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

THE NUCLEAR LANDSCAPE

Where do they come from?

Natural Radioactivity … natural processes occurring in the sun or other stars, in our atmosphere, and part of the gas clouds that formed our solar system.

Man Made Radioactivity … Reactors, accelerators etc.

• Most elements have several stable isotopes. Every element has many unstable (radioactive) isotopes. • There are about 200 different stable isotopes. There are about 7000 possible different radioactive isotopes.

Page 7: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

The Nuclear Landscape

Page 8: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

LET’S EXPLORE SOME PROPERTIES OF RADIOACTIVITY

Each type of radiation is ionizing but each has different properties which affect the hazards they pose, the detection mechanism and the shielding required to stop them.

Five Common Types

Alpha Decay

Beta Decay

Gamma Decay

Fission

Neutron Emission

Page 9: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

ALPHA PARTICLE RADIATION

The daughter might also be radioactive and emit a second alpha particle. This is called a decay chain and is pretty common for heavy nuclei.

Page 10: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

DECAY CHAINS

PuU

Th

Ra

Rn

Po

Pb

Hg

Au

Page 11: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

BETA PARTICLE RADIATION

Page 12: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

GAMMA-RAY RADIATION

Page 13: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

FISSION

The heavy parent nucleus fissions …

… into two lighter (radioactive) fission fragment nuclei plus some left over neutrons

Sometimes a very heavy nucleus will fall apart before it can emit an alpha particle.

Fission can release an enormous amount of energy and is utilized in power plants and fission bombs.

Page 14: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

NEUTRON EMISSION

Neutron emission doesn’t happen naturally because a neutron has no charge, so it has no barrier to overcome!

Page 15: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

A nucleus is made up of nucleons (protons and neutrons):

Mass Spin Charge

Proton 938.272 MeV/c2 1/2 +1e

Neutron 939.565 MeV/c2 1/2 0

size: ~1 fm

In a nucleus, nucleons attract each other via the strong force ( range ~ 1 fm)

neutron proton(or any other charged particle)

V

r

R

V

rR

Coulomb Barrier Vc

R

eZZVc

221

Pote

nti

al

Pote

nti

al

Nucleons in a Box:Discrete energy levels in nucleus

R ~ 1.3 x A1/3 fm

WHAT HOLDS A NUCLEUS TOGETHER?

Page 16: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

HOW UNSTABLE IS A RADIOACTIVE ATOM? The “Half-Life” describes how quickly Radioactive Material

decays away with time.

It is the time required for half of the unstable atoms to decay.

Some Examples: Some natural isotopes (like uranium and thorium) have

half-lives that are billions of years, Most medical isotopes (like Technicium-99m) last only a

few days

Page 17: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

ELECTRONS, NEUTRONS AND PROTONS ARE FERMIONS (SPIN = HALF-INTEGER)

Electron (intrinsic spin = ½) + Orbital angular momentum (quantized) =

Total angular momentum

Also gives rise to magnetic moment

And ‘spin-orbit’ splitting

Page 18: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

PROPERTIES OF IRON ISOTOPES

Z A AtomicMass (u)

NuclearMass(Ge

V/c2

Binding Energy(

MeV)Spin Natural

Abund. Half-life Decay QMeV

26 54 53.9396

13 50.2315 471.77 0 0.059 stable ... ...

26 55 54.9382

96 51.1618 481.07 3/2 ... 2.7y EC 0.23

26 56 55.9349

39 52.0902 492.26 0 0.9172 stable ... ...

26 57 56.9353

96 53.0221 499.91 1/2 0.021 stable ... ...

26 58 57.9332

77 53.9517 509.96 0 0.0028 stable ... ...

26 60 59.9340

77 55.8154 525.35 0 ... 1.5My b- 0.24

Page 19: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

mp = proton mass, mn = neutron mass, m(Z,N) = mass of nucleus with Z,N

2),( BcNmZmNZm np

Most tables give atomic mass excess in MeV (so for 12C: =0):

Masses are usually tabulated as atomic masses

2/ cAmm u

Nuclear Mass~ 1 GeV/A

Electron Mass511 keV/Z

Electron Binding Energy13.6 eV (H)to 116 keV (K-shell U) / Z

m = mnuc + Z me + Be

MASS OF AN ATOM OR NUCLEI

M(Z,N) – Zmp – Nmn is known as the nuclear binding energy

Page 20: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org
Page 21: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

Magic numbers:

Nuclei are more stable if the proton or neutron number is magic; doubly magic is most stable, e.g. 4He, 208Pb

NUCLEI HAVE SHELL STRUCTURE184

126

82

50282082

Page 22: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

MARIA GOEPERT-MAYER While working at Argonne National

Laboratory in 1948, physicist Maria Goeppert Mayer developed the explanation of how neutrons and protons within atomic nuclei are structured. Called the "nuclear shell model," her work explains why the nuclei of some atoms are more stable than others and why some elements have many different atomic forms, called "isotopes," while others do not. For this work, she shared the 1963 Nobel Prize in physics.

Goeppert Mayer was only the second woman to receive the Nobel Prize in physics, following Marie Curie, and only the fourth American woman to win a Nobel Prize.

Page 23: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

NUCLEI ALSO ACT LIKE A LIQUID DROP

The factors that determine whether the drop is ‘stable’ include Volume (Z+N) Surface energy (Z+N) Asymmetry (N/Z)

The combination of liquid drop energy (macroscopic) and effect of shell structure (microscopic) determine the binding energy of a nucleus

Page 24: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

WHY DOES A RADIOACTIVE NUCLEUS DECAY? Think back to chemistry

A chemical reaction could be exothermic (generate energy) Endothermic (require energy to make it work)

Nuclear reactions or decays are the same A B + C

Q-value = energy generated by reaction = (mB + mC – mA)c2 (E = mc2) If Q > 0, energy is generated and decay may happen If Q < 0, energy is consumed

Example: Reaction Q

d p + n = 2. – 1. -1. =

d 14.003241982(27)

n 10.0129370(4)

p 14.0030740052(9)

4.0026032497(10)

Mass Table (u)

Page 25: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

Decay of A in B and C is possible if reaction A B+C has positive Q-value

BUT: there might be a barrier that prolongs the lifetime

Decay is described by quantum mechanics and is a pure random process, with a constant probability for the decay to happen in a given time interval.

N: Number of nuclei A (Parent)l : decay rate (decays per second and parent nucleus)

NdtdN therefore ttNtN e)0()(

lifetime =1/t lhalf-life T1/2 = t ln2 = ln2/l is time for half of the nuclei present to decay

WILL A NUCLEUS WITH Q > 0 DECAY?

Page 26: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

V

rR

Coulomb Barrier Vc

R

eZZVc

221

Pote

nti

al

unboundparticle

Example: for 197Au -> 58Fe + 139I has Q ~ 100 MeV ! yet, gold is stable.

most common: • b decay• n decay• p decay• a decay• fission

THE COULOMB BARRIER

For anything other than a neutron (or a neutrino) emitted from the nucleusthere is a Coulomb barrier The particle has to ‘tunnel’

through the barrier if it doesn’t have enough energy to get over the top

If that barrier delays the decay beyond the lifetime of the universe (~ 14 Gyr)we consider the nucleus as being stable.

not all decays that are energetically possible happen

Page 27: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

In the middle of the chart, most nuclei beta decay:

Z

N

blue: neutron excessundergo b- decay:

AZ A(Z+1) + b- + +

red: proton excessundergo b+ decay:

AZ A(Z-1) + b+ + +

isobaric chain

Page 28: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

b+ decay

electron capture

b- decay

p n + e+ + ne

e- + p n + ne

n p + e- + ne

Electron capture (or EC) of atomic electrons or, in astrophysics, of electrons in the surrounding plasma

BETA DECAY ENERGETICS

Page 29: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

b decay basically no barrier -> if energetically possible it usually happens(except if another decay mode dominates)

therefore: any nucleus with a given mass number A will be converted into the most stable proton/neutron combination with mass number A by b decays

valley of stability(Bertulani & Schechter)

Page 30: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

When no more neutrons can be bound, the neutron drip line is reached

Neutron drip line:

Sn= 0

beyond the neutron drip line, neutron decay occurs:

(Z,N) (Z,N-1) + n

Q-value: Qn = m(Z,N) - m(Z,N-1) - mn

beyond the drip line Sn<0

Neutron Separation Energy Sn

Sn(Z,N) = m(Z,N-1) + mn - m(Z,N) = -Qn for n-decay

As there is no Coulomb barrier, and n-decay is governed by the strong force,for our purposes the decay is immediate and dominates all other possible decay modes

the nuclei are neutron unbound

Neutron drip line very closely resembles the border of nuclear existence !

NEUTRON DECAY

Page 31: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

30 40 50 60 70 80 90 100neutron num ber N

-5

0

5

10

15

20S

n (M

eV)

Example: Neutron Separation Energies for Z=40 (Zirconium)

neutron drip line

valley of stability

add 37 neutrons

At Michigan State Univ, the National Superconducting Cyclotron Lab (NSCL) is exploring the limits of nuclear stability by trying to reach neutron drip line through fragmenting Uranium nuclei.

Page 32: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

neutrons

protons

Mass knownHalf-life knownnothing known

H(1)

Fe (26)

Sn (50)

Pb (82)

neutron dripline

proton dripline

note odd-even effect in drip line !(p-drip: even Z more bound - can take away more n’s)(n-drip: even N more bound - can take away more p’s)

Page 33: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

ALPHA DECAY

yelloware a emitter

Page 34: THE ABC’S OF R ADIOACTIVITY Physics of Atomic Nuclei - Lecture 3 Peggy Norris, pnorris@sanfordlab.org

Nuc le a r C ha rg e Yie ld in Fissio n o f 234U

25 30 35 40 45 50 55 60 65

80 100 120 140 160 M a ss Num b e r A

Pro to n Num b e r Z

0

5

10

15

20

Yie

ld Y

(Z

) (%

)

FISSION

green = spontaneous fission