y-90,i-131 and cs-137 production: fission yields
DESCRIPTION
Capture Cross-Sections and Fission Yields for the Production of Therapeutic Radionuclides J-Ch Sublet CEA, CE de Cadarache DEN/DER/SPRC 13108 Saint Paul les Durance, France Agreement number: FRA 12487 E-mail : [email protected]. Y-90,I-131 and Cs-137 production: Fission yields. - PowerPoint PPT PresentationTRANSCRIPT
1
Capture Cross-Sections and Fission Yields for the
Production of Therapeutic Radionuclides
J-Ch Sublet
CEA, CE de CadaracheDEN/DER/SPRC
13108 Saint Paul les Durance, France
Agreement number: FRA 12487E-mail : [email protected]
2DEN/DER/SPRC
Y-90,I-131 and Cs-137 production: Fission yields
Three established therapeutic radionuclides are produced as fission products in reactors
The main fissile isotope is the U-235, although other fissionable isotopes generate those products in the same manner
The energy dependence of the fission yields is reported
The experimental cumulated fission yields measurements have been extracted from a Nexia Solutions database (UK)
The thermal cumulated fission yields for those isotopes are
known with an associated uncertainties of 1-2%
3DEN/DER/SPRC
Mass Distribution with uncertainty / U – 235 / Thermal
Good agreementin the humps
4DEN/DER/SPRC
Mass Distribution with uncertainty / U – 235 / 400 keV
Yields # energy
5DEN/DER/SPRC
Mass Distribution with uncertainty / U – 235 / 14 MeV
reducedhumps
6DEN/DER/SPRC
Charge Distribution / U – 235 / Thermal
odd #even
7DEN/DER/SPRC
Charge Distribution / U – 235 / 400 keV
largedifferences
8DEN/DER/SPRC
38-Sr-90 fission yields : thermal, Kev and MeV Yields Yields Z A Independent Uncert. Cumulative Uncert.UKFY3-6 38 89 2.183E-05 8.003E-04 4.689E-02 5.678E-03 12.1% UKFY3-6 38 90 3.134E-04 1.180E-04 5.729E-02 1.319E-03 2.3%UKFY3-6 38 90 1.248E-04 4.608E-05 5.221E-02 1.830E-03 3.5%UKFY3-6 38 90 2.109E-03 7.407E-04 4.408E-02 1.808E-03 4.1%
= JEFF-3.1 /FY
JENDL33 38 90 0.356E-03 0.000E+00 0.590E-01 0.000E+00JENDL33 38 90 0.219E-03 0.000E+00 0.543E-01 0.000E+00JENDL33 38 90 0.760E-03 0.000E+00 0.466E-01 0.000E+00 JEF2.2 38 90 0.357E-03 0.134E-03 0.585E-01 0.188E-02 3.2%JEF2.2 38 90 0.120E-03 0.700E-04 0.525E-01 0.400E-02JEF2.2 38 90 0.130E-02 0.551E-03 0.459E-01 0.119E-02 ENDFB65 38 90 0.737E-03 0.442E-04 0.578E-01 0.578E-03 1% ??ENDFB65 38 90 0.343E-03 0.154E-03 0.546E-01 0.383E-03ENDFB65 38 90 0.112E-02 0.719E-03 0.459E-01 0.184E-02
Thermal >400 KeV >14 MeV >
-20%
14x
9DEN/DER/SPRC
90-Y generator
10DEN/DER/SPRC
53-I-131 Fission yields: thermal, Kev and MeV
Yields Yields Z A Independent Uncert. Cumulative Uncert. UKFY3-6 53 131 1.364E-05 4.745E-06 2.878E-02 3.166E-04 1.1%UKFY3-6 53 131 4.434E-05 1.671E-05 3.365E-02 5.384E-04 1.6%UKFY3-6 53 131 2.678E-03 9.195E-04 4.110E-02 1.356E-03 3.3%
= JEFF-3.1 /FY
JENDL33 53 131 0.415E-04 0.000E+00 0.288E-01 0.000E+00JENDL33 53 131 0.320E-04 0.000E+00 0.318E-01 0.000E+00JENDL33 53 131 0.105E-02 0.000E+00 0.399E-01 0.000E+00 JEF2.2 53 131 0.190E-04 0.620E-05 0.289E-01 0.324E-03 1.1%JEF2.2 53 131 0.601E-04 0.349E-04 0.333E-01 0.631E-03JEF2.2 53 131 0.929E-04 0.424E-04 0.393E-01 0.133E-02
ENDFB65 53 131 0.392E-04 0.431E-05 0.289E-01 0.289E-03 1% ??ENDFB65 53 131 0.108E-04 0.692E-05 0.322E-01 0.451E-03ENDFB65 53 131 0.120E-02 0.769E-03 0.410E-01 0.164E-02
Thermal >400 KeV >14 MeV >
11DEN/DER/SPRC
55-Cs-137 Fission yields: thermal, Kev and MeV
Yields Yields Z A Independent Uncert. Cumulative Uncert. UKFY3-6 55 137 7.225E-04 2.557E-04 6.221E-02 6.936E-04 1.1%UKFY3-6 55 137 1.225E-03 4.398E-04 5.889E-02 9.572E-04 1.6%UKFY3-6 55 137 1.138E-02 3.203E-03 5.567E-02 1.308E-02 23.5%
= JEFF-3.1 /FY
JENDL33 55 137 0.158E-02 0.000E+00 0.627E-01 0.000E+00JENDL33 55 137 0.299E-02 0.000E+00 0.620E-01 0.000E+00JENDL33 55 137 0.889E-02 0.000E+00 0.492E-01 0.000E+00 JEF2.2 55 137 0.872E-03 0.309E-03 0.624E-01 0.539E-02 8.6%JEF2.2 55 137 0.151E-02 0.855E-03 0.600E-01 0.844E-02JEF2.2 55 137 0.436E-02 0.169E-02 0.559E-01 0.708E-02 ENDFB65 55 137 0.600E-03 0.660E-04 0.619E-01 0.309E-03 0.5% ??ENDFB65 55 137 0.228E-02 0.731E-03 0.622E-01 0.311E-03ENDFB65 55 137 0.948E-02 0.303E-02 0.493E-01 0.296E-02
Thermal >400 KeV >14 MeV >
12DEN/DER/SPRC
JEFF-3.1 cumulative and chain yields measurements
Cumulative Experimental + chainyields - JEFF-3.1 yields (Nexia Solutions)
38-Sr-90 (28.869 y +/-0.19%)5.729E-02 2.3% (7+) 5.77E-02 7%5.221E-02 3.5% (4+) 5.27E-02 6%4.408E-02 4.1% (3+) 4.41E-02 4%
53-I -131 (8.040 d +/-0.12%)2.878E-02 1.1% (15+) 2.88E-02 9%3.365E-02 1.6% (11+) 3.36E-02 5%4.110E-02 3.3% (5+) 4.09E-02 5%
55-Cs-137 (30.172 y +/-0.54%)6.221E-02 1.1% (11+) 6.21E-02 8%5.889E-02 1.6% (7+) 6.02E-02 8%5.567E-02 23.5% (1+) 5.90E-02 10%
numbers of experiments
13DEN/DER/SPRC
Capture channels and decay
Nuclear data production of the therapeutic radionuclides through capture channels and decay:
Re186: 185Re(n,g)186Re
Re188: 186W(n,g)187W(n,g)188W, - 188Re
Cu64: 63Cu(n,g)64Cu
In114m: 113In(n,g)114In (114mIn)
Ho166: 164Dy(n,g)165Dy(n,g)166Dy, - 166Ho
Yb169: 168Yb(n,g)169Yb
Lu177: 176Yb(n,g)177Yb, - 177Lu176Lu(n,g)177Lu
14DEN/DER/SPRC
Re186 T½ 3.77 d +/- 0.12%; β−:93.1%; β+:6.9%
Re-185(n,g)Re-186
EAF-2005.1
Cro
ss s
ectio
n (b
)
Energy (eV)
1.0E+05
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
1.0E+04
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30RI 87RI 87TAT79FLA63GA 68ORL60ORL52LRL76LRL76LRL76 gGA 68GA 68LEB71
Re-185 0.0253eV cross section Barns Uncert. Lab. 127. 36 ORL60 114. 30 GA68 101. 20 ANL47 116. 6 LRL78 112. 9-13% EAF-2005
Re-185 Resonance Integral E. Min. Barns Uncert. Lab.
0.5 1810. 150. LRL78 0.5 1419. 77. GHT74 0.5 1790. 60. LRC68 0.5 1650. 90. STF66
1705. 3-6% EAF-2005
15DEN/DER/SPRC
Re186 T½ 3.77 d +/- 0.12%; β−:93.1%; β+:6.9%
Re-185(n,g)Re-186
EAF-2005.1 g EAF-2005.1 m EAF-2005.1 tot
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+05
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
1.0E+04
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataExp dataExp dataExp dataRI 87RI 87TAT79FLA63GA 68ORL60ORL52LRL76LRL76LRL76 gGA 68GA 68LEB71A very long lived isomer
exists
decaying by IT only
Re186m T½ 2.00E+05 y +/- 25.4%; IT 100%
16DEN/DER/SPRC
Lu177 T½ 6.70 days +/-0.3%; β-
Lu-176(n,g)Lu-177
EAF-2005.1
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+05
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
1.0E+04
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataExp dataIJI87IJI87 mHAR60MUN76 mCOP62 mLRL78LRL67 mORL67ORL84WUR75
Lu-176 0.0253eV cross section Barns Uncert Lab. 2100 150 HAR60 3640 728 ANL47 2097 8% EAF-2005
m 2.1 0.7 MUN76m 7.0 2.0 LRL67m 2.0 EAF-2005
17DEN/DER/SPRC
Lu177 T½ 6.70 days +/-0.3%; β-
Lu-176(n,g)Lu-177
EAF-2005.1 g EAF-2005.1 m EAF-2005.1 tot
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+05
1.0E-05
1.0E-04
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
1.0E+04
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataExp dataExp dataExp dataIJI87IJI87 mHAR60MUN76 mCOP62 mLRL78LRL67 mORL67ORL84WUR75
18DEN/DER/SPRC
Lu177 T½ 6.70 days +/-0.3%; β-
Yb-176(n,g)Yb-177
EAF-2005.1
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+04
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataExp dataRI 87RI 87AUW70JYV76OSL70LRL78MCM56ANL68FEI74FEI96
Yb - 176 0.0253eV cross section
Barns Uncert. Lab.
3.02 0.5 LRL78
2.40 0.2 OSL70
2.85 10 - 20% EAF - 2005
19DEN/DER/SPRC
Lu177 T½ 6.70 days +/-0.3%; β- Yb-176(n,g)Yb-177
EAF-2005.1 g EAF-2005.1 m EAF-2005.1 tot
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+04
1.0E-04
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataExp dataRI 87RI 87AUW70JYV76OSL70LRL78MCM56ANL68FEI74FEI96
Yb-176 Resonance Integral E. Min. Barns Uncert Lab.
0.5 1.33 0.13 LRL70 0.4 2.7 0.3 OSL70 0.5 9.2 1.8 KJL75
0.55 14.4 1.2 GHT73 6.83 10-20% EAF-2005
Yb177 T½ 1.88 Hrs +/-5.8%; β-
Yb177m T½ 6.41 s +/-0.31%; IT
20DEN/DER/SPRC
Yb169 T½ 32.01 days +/- 0.06%; β+ Yb-168(n,g)Yb-169
EAF-2005.1
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+06
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
1.0E+04
1.0E+05
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataExp dataExp dataRI 89 gAUW70 gOSL70LAS68TNC61CPO70CPO70Yb-168 0.0253eV cross section
Barns Uncert. Lab. 3660 50 CPO70 5500 2640 TNC61 2840 600 LAS68 2600 60 LRL78 4400 200 OSL70 2305 20% EAF-2005
Renormalized to CPO70
21DEN/DER/SPRC
Yb169 T½ 32.01 days +/-0.06%; β+ Yb-168(n,g)Yb-169
EAF-2005.1 g EAF-2005.1 m EAF-2005.1 tot
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+06
1.0E-04
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
1.0E+04
1.0E+05
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataExp dataExp dataRI 89 gAUW70 gOSL70LAS68TNC61CPO70CPO70
Yb-168 Resonance Integral E. Min. Barns Uncert. Lab.
35706 1714 CNE70 38000 2000 OSL70 23040 5440 GHT73
0.55 19800 4200 CPO70 0.55 21000 4200 CPO70 0.5 16600 1700 LRL78 0.5 14700 1900 KJL69
21212 25% EAF-2005
22DEN/DER/SPRC
Ho166 T½ 1.117 days +/-0.07%; β- Dy-164(n,g)Dy-165
EAF-2005.1
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+06
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
1.0E+04
1.0E+05
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataExp dataARK60MNZ54LRL58ARK60 mARK60OSL72 gOSL72 mNPL74 gSAC77 gANR91 gMUA65MUA68 mMUA68 gAUW72 mMUA62RI 87OSL72 gBNL61VIP72 gWIS59FEI88FEI81
Dy-164 0.0253eV cross section Barns Uncert. Lab. 2695 - SAC77 2700 100 NPL74 2800 140 OSL72 1700 240 OSL72m 1056 - ANR91g 951 - MAU62g 1100 - OSL62g 507 - MNZ54
2650.6 15% EAF-2005
23DEN/DER/SPRC
Ho166 T½ 1.117 days +/-0.07%; β- Dy-164(n,g)Dy-165
EAF-2005.1 g EAF-2005.1 m EAF-2005.1 tot
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+06
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
1.0E+04
1.0E+05
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataExp dataExp dataExp dataARK60MNZ54LRL58ARK60 mARK60OSL72 gOSL72 mNPL74 gSAC77 gANR91 gMUA65MUA68 mMUA68 gAUW72 mMUA62RI 87OSL72 gBNL61VIP72 gWIS59FEI88FEI81
Dy-164 Resonance Integral E. Min. Barns Uncert. Lab.
0.5 527 89. ANR05 0.5 649 24 KTO01 0.5 335 27 KJL75 0.5 470 20 GHT74m
342 50% EAF-2005
Integral C/E for Dy-164(n,g)Dy-165m
C/E
Neutron Spectrum
C/E = 0.8524
1.50
0.670.70
0.80
0.90
1.00
1.10
fns_5min
fusion spectrum
24DEN/DER/SPRC
Ho166 T½ 1.117 days +/-0.07%; β- Dy-165(n,g)Dy-166
EAF-2005.1
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+06
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
1.0E+04
1.0E+05
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataOSL72JAE81
Dy-165 0.0253eV cross section Barns Uncert. Lab. 2000 - JAE81 3900 - OSL72 3530 300 JAE81 3573 10% EAF-2005
Dy-165 Resonance Integral E. Min. Barns Uncert. Lab.
0.5 22000 3000 OSL72 20801 15% EAF-2005
Dy166 T½ 3.4 days +/-0.12%; β-
25DEN/DER/SPRC
Re188 T½ 16.981 hrs +/- 0.13%; β- W-186(n,g)W-187
EAF-2005.1 tot
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+05
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
1.0E+04
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataExp dataExp dataExp dataExp dataRI 87NIR81MUN87LND80IRK76MTR70ORL60BNL79ORL77BRC86BRC80LRL76RPI66ORL83FEI86
W-186 0.0253eV cross section Barns Uncert. Lab. 37.0 1.5 ORL77 35.4 8.0 MOL67 37.8 1.2 AGA66 38.5 8.0 MUN87 37.5 3-6% EAF-2005
W-186 Resonance Integral
E. Min. Barns Uncert. Lab. 0.5 426. 32. LRL78 0.5 490. 15. ORL77 0.5 410. 47. GHT74 0.5 345. 99. BGK69
519 5-30% EAF-2005
26DEN/DER/SPRC
Integral validation
Integral C/E for W-186(n,g)W-187C
/E
Neutron Spectrum
C/E = 0.9256C/E = 1.0108
C/E = 0.9312
C/E = 2.0835
C/E = 0.6672
C/E = 0.1790
C/E = 0.7624
1.50
0.67
0.00
0.50
1.00
1.50
2.00
2.50
fng_tung.asc fns_5min rez_DF
fng_f82h.asc sneg_1 fzk_ss316 rez_DF
27DEN/DER/SPRC
Re188 T½ 16.981 hrs +/- 0.13%; β- W-187(n,g)W-188
EAF-2005.1
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+05
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
1.0E+04
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataORL66
W-187 Resonance Integral
E. Min. Barns Uncert. Lab. 0.5 2760 550. ORL66
1652 70% EAF-2005 W-187 0.0253eV cross section Barn. Uncert Lab.
64 - ORL66 70 10 ORL77
70.8 10%. EAF-2005
W188 T½ 69.44 days 0.83%; β-
Single level Breit-Wignerformalism: SRA
28DEN/DER/SPRC
Cu64 T½ 12.702h +/-0.02%; β−:38.86%;β+:61.14%
Cu-63(n,g)Cu-64
EAF-2005.1
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E-04
1.0E+03
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataANR91ORL59MOL67NPL74NPL70MUN74ORL77GOE58DEB70MUA68TAT79BHU70BRC86FEI69IFU68FEI66
Cu-63 0.0253eV cross section Barns Uncert. Lab. 4.45 +/-0.5 ORL77 4.66 +/-0.5 ORL60 4.44 +/-0.2 NPL74 4.52 +/-0.2 Mu01 4.47 1-4% EAF-2005
29DEN/DER/SPRC
Cu64 T½ 12.702h +/-0.02%; β−:38.86%;β+:61.14%
Integral C/E for Cu-63(n,g)Cu-64
C/E
Neutron Spectrum
C/E = 0.5906
1.50
0.67
0.50
0.60
0.70
0.80
0.90
1.00
1.10
cf252_flux_1
Not so reliable integral data
Cu-63 Resonance Integral E. Min. Barns Uncert. Lab.
0.5 5.3 0.1 ORL77 0.55 5.0 - ANL64 0.5 5.15 0.10 LRL78 0.1 2.79 0.18 NPL74 0.55 4.7 0.3 GHT72
4.92 4-7% EAF-2005
30DEN/DER/SPRC
In114m T½ 50.0 d +/- 0.4%; β+:3.5%;IT:96.5%
In-113(n,g)In-114
EAF-2005.1
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+04
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataRI 87 mAUW73 mGHT72MTR63 gMTR63KFK66 mLOK68 mLOK68 mLOK68 gLOK68 m
In-114 0.0253eV cross section Barns Uncert lab 9.45 0.4 GHT72 m 7.5 0.7 ROS68 m 8.1 0.8 MTR63 m 3.1 0.7 ROS68 g 3.9 0.4 MTR63 g
12.04 4-10% EAF-2005
In-114 Resonance Integral E. Min. Barn Uncert. Lab
0.55 258 18 GHT73 0.55 258 10 GHT69 0.5 243 29 CNE70
321 7-12% EAF-2005
134 186
EAF-2005g EAF-2005m
31DEN/DER/SPRC
In114m T½ 50.0 d +/- 0.4%; β+:3.5%;IT:96.5%
In-113(n,g)In-114
EAF-2005.1 g EAF-2005.1 m EAF-2005.1 tot
Cro
ss s
ect
ion
(b
)
Energy (eV)
1.0E+04
1.0E-03
1.0E-02
1.0E-01
1.0E+00
1.0E+01
1.0E+02
1.0E+03
6.0E+071.0E-04 1.0E-03 1.0E-02 1.0E-01 1.0E+00 1.0E+01 1.0E+02 1.0E+03 1.0E+04 1.0E+05 1.0E+06 1.0E+07
SystmSys30Exp dataExp dataExp dataExp dataExp dataExp dataRI 87 mAUW73 mGHT72MTR63 gMTR63KFK66 mLOK68 mLOK68 mLOK68 gLOK68 m
In-114 Branching ratio Energy B.r. Uncert. Lab.
2.53E-01 2.6 0.1 ROS68 2.53E-01 2.1 0.1 MTR63 7.80E+03 2.14 0.3 KFK66 3.00E+04 2.67 0.5 KFK66 6.40E+04 5.05 1.0 KFK66 3.68E+05 3.2 0.3 LOK68 1.00E+06 3.5 0.3 LOK68
Modified B.R. m/gthermal 2.1above urr: 3.0 – 4.0
32DEN/DER/SPRC
Conclusions
10 capture channels have been evaluated with their associated uncertainties
3 cumulated fission yields selected, with the associated uncertainties
All products isotopes decay data assembled
– file format, with uncertainties– derived quantities– final documentation