magnetic plasma
TRANSCRIPT
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Influence of magnetic fields on negative corona discharge currents
Junfeng Mi, Dexuan Xu*, Yinghao Sun, Shengnan Du, Yu Chen
Laboratory of Discharge Plasma and Pollution Control Engineering, Department of Environmental Science and Engineering,
Northeast Normal University, Changchun 130024, China
a r t i c l e i n f o
Article history:
Received 1 July 2007
Received in revised form 31 March 2008
Accepted 16 April 2008
Available online 28 May 2008
Keywords:
Magnetically enhanced
Negative corona discharge
Plasma
a b s t r a c t
The mechanism of magnetically enhanced negative corona discharges was studied by comparing the
influences of two different magnetic fields on the negative corona discharge current. In the magneticallyenhanced corona discharge, a local magnetic field is formed near the discharge electrode by using the
small permanent magnets, and the corona discharge currents are enhanced because the Larmor
movements of free electrons enhance the ionizations of the gas molecules in the ionization region. It is
assumed that the increase of the discharge currents attributes to only the enhanced ionization process in
the small ionization region, and is not relevant to the lengthening trajectory of free electrons in the wide
drift inter-electrode region. In the enhanced ionization-region magnetic field, the mechanism of mag-
netically enhanced corona discharges was explained and the relative increase of the discharge current
could exceed 150%. However, in a weakened ionization-region magnetic field, the mechanism of mag-
netically enhanced corona discharges was inconspicuous and the relative increase of the discharge
current could only reach about 25%. It is predicted that after the magnetic field of magnetically enhanced
negative corona discharges had been fixed, the relative increases of the discharge current for varied
mean electric fields in the inter-electrode region could have a maximum value, according to the
mechanism of magnetically enhanced negative corona discharges. The above predication was completely
validated by the current experiment data. In addition, the optimum combinations between the electric
field and the magnetic field were obtained. In order to reach the largest relative increase of the discharge
current under 4 kV/cm mean electric field intensity in the inter-electrode region for a practical elec-trostatic precipitator, the optimum magnetic field with a magnetic flux density of about 0.43 T at the
edges of magnetic st rings should be selected.
2008 Elsevier B.V. All rights reserved.
1. Introduction
Recently, more and more countries are beginning to limit the
emissions of micron and sub-micron aerosol particles. Thus the
corona discharges have progressively employed for electrostatic
precipitators (ESP) and pre-chargers as well as some new applica-
tions, such as sterilization [1], the enhancement of chemical vapor
deposition [2], separation [3], and the production of ozone [4].The theory for charging particles is well developed for the better
application of ESP. Pauthenier and Moreau-Hanot [5] developed an
expression for field charging of large aerosol particles. Fuchs and
Bricard developed the same statement for diffusion charging of
smaller aerosol particles, and the combined field and diffusion
charging theory was discussed by Liu and Kapadia [6]. A few
experimental and theoretical studies [710] indicated that Fuchs
theory had successfully predicted the charging probability of fine
particles. The experimental and mathematical study carried out by
Reischl et al. [11] demonstratedthat Fuchs theory was also valid for
bipolar diffusion charging of fine particles, while the charging
probability of positive ions was less than that of negative ions. In
addition, there was no difference between varied gases and particle
materials. The charges on fine aerosol particles also vary in agree-
ment with diffusion charging theory, which tended to promote the
charging of fine aerosol particles.Based on the above charging theories, the diffusion charging
should be intensified for removal of fine aerosol particles in ESP. In
addition, the diffusion charging will be a determined factor when
the fine aerosol particles pass through ESP with a weak intensity of
the applied electric field as well as a higher gas temperature.
However, the field charging will be a determined factor when the
large aerosol particles pass through ESP with a strong intensity of
the applied electric field and a lower gas temperature [12].
According to the diffusion charging theory of ions, it is advan-
tageous for diffusion charging to supply a higher concentration of
ions when the intensity of the electric field is weaker. However, the
weak electric field could not induce a high concentration of ions in* Corresponding author.
E-mail address: [email protected] (D. Xu).
Contents lists available at ScienceDirect
Journal of Electrostatics
j o u r n a l h o m e p a g e : w w w . e l s e v i e r . c o m / l o c a t e / e l s t a t
0304-3886/$ see front matter 2008 Elsevier B.V. All rights reserved.doi:10.1016/j.elstat.2008.04.010
Journal of Electrostatics 66 (2008) 457462
mailto:[email protected]://www.sciencedirect.com/science/journal/03043886http://www.elsevier.com/locate/elstathttp://www.elsevier.com/locate/elstathttp://www.sciencedirect.com/science/journal/03043886mailto:[email protected] -
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the general corona discharges. Therefore, the fine aerosol particles
could be effectively captured when a higher concentration of ions
and weaker electric field are supplied by ESP. In order to charge fine
aerosol particles, it is necessary to enhance the corona discharge
currents in ESP with a weak intensity of electric field.
Researches on enhancing corona discharge current using
a magnetic field have been carried out in recent years. Initially, the
study on a small cylinder corona nozzle posited in the inner-hole of
a cylindrical permanent magnet where a weakened ionization-
region magnetic field was formed, was reported [13]. Although the
propagation of an ionization region was noticed in the experiment,
the influence of the magnetic field on ionization was not given
enough attention. We then conducted research on a magnetically
enhanced corona pre-charger [14]. An enhanced ionization-region
magnetic field was formed by installing a small permanent magnet
near the discharge electrode, which causes the magnetic flux
densityto be higher in the ionization region than in the drift region.
When the magnetic flux density was 0.43 T at the edges of mag-
netic strings, the discharge current was increased by 1.3 times
under a high voltage of 15 kV. The concentration of negative ions in
the charging region of the pre-charger was greatly increased as
well. This result is of great benefit to the charging of fine aerosol
particles. It was supposed that the dominant mechanism of mag-netic enhancement in the corona discharges involves the Larmor
movements of free electrons which enhance ionizations of the gas
molecules near the discharge electrode, and the lengthening
trajectory of free electrons also induces a little increase of corona
discharge current.
In the current study, we conductedthe research on the influence
of the magnetic field on negative corona discharge current to fur-
ther explore the mechanism of magnetically enhanced corona
discharge. Only the magnetically enhanced negative corona dis-
charges were discussed in this paper for its wide use.
2. Experimental apparatus
The magnetic field was applied near the discharge electrode;
herein called the ionization-region magnetic field. The experi-
mental apparatus is shown in Fig. 1. The effective length of the
stainless-steel wire electrode (4) was 10 mm and 0.5 mm in di-
ameter. Two cylindrical, permanent magnet strings (5) of 6 mm in
diameter were made from permanent magnet disks and assembled
at opposite ends of the wire electrode. The magnetic flux density
near the discharge electrode could be changed by increasing or
decreasing the numberof magnet disks in the magnetic strings. The
spacing between the two magnetic strings was kept at 12 mm. The
wire electrode was positioned exactly in the center of stainless
cylinder electrodes (3). The length of cylinder electrode was 70 mm
and its diameter 70 mm. A high-voltage power supply (1) (Beijing
Electrostatic Instrument Factory, China, GJ F 100), capable of de-
livering negative voltage, was measured using a high voltage
divider (2) (Shanghai Huisha Instrument Co., Ltd., China, FRC-50).
Between the cylinder electrode and grounding wire, two ammeters
with different measurement ranges were connected. One ammeter
(Cany Precision Instruments Co., Ltd., China, BS15/6) was used to
measure the corona onset voltage, and the other (Cany Precision
Instruments Co., Ltd., China, BS15/16) was used to measure the
discharge current.
Fig. 2 shows the magnetic and the electric lines of force between
discharge and cylinder electrode when the strongest magnetic flux
density (near magnetic string edge) is 0.43 T. The magnetic lines of
force were approximately perpendicular to the electric lines of
force near the wire electrode. The magnetic flux density of mag-
netic string edges was measured using a gaussmeter (Shanghai NO.
4 Multimeter Manufacturing Co., Ltd., China, CT5 A). It is obvious
that the magnetic flux density gradually decreases from the wireelectrode to the cylinder electrode when a permanent magnet is
applied near the wire electrode, i.e., the influence of the magnetic
field on the ionization region is stronger than the drift region.
In the second experiment, the magnetic field was applied near
the collecting electrode; herein called the drift region magnetic
field. The experimental apparatus is shown in Fig. 3. The effective
length of the stainless-steel wire electrode (4) was 70 mm and
0.5 mm in diameter. The length of the cylinder electrode (3) was
100 mm, with an insidediameterof 56 mmand an outside diameter
of 60 mm. The cylinder magnet (5) was made from permanent
magnet rings and was installed outside the cylinder electrode, and
the cylinder magnet was 50 mm long with an inside diameter of
60 mm and an outside diameter of 72 mm. The magnetic flux
density in theentire inter-electrode regioncouldalso be changed byincreasing or decreasing the numberof magnet rings of the cylinder
magnet. The wire electrode was positioned exactly in the center of
the cylinder electrode (3). The functions of the high-voltage power
Fig.1. Schematic of experimental apparatus with the ionization-region magnetic field.
1. HV power supply, 2. HV divider, 3. cylinder electrode, 4. wire electrode, and 5.magnet strings.
Fig. 2. Schematic of the magnetic lines of force and the electric lines of force in theionization-region magnetic field.
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supply (1) and the high voltage divider (2) in this experiment wereaccordant with those in the experiment of the ionization-region
magnetic field.
Fig. 4 shows the magnetic and the electric lines of force between
the wire and cylinder electrodes when the mean magnetic flux
density is 0.015 T near the wire electrode in the drift region mag-
netic field experiment. The strongest magnetic flux density is
0.39 T. In order to determine the mean magnetic flux density near
the wire electrode, four equidistant points on the axis in the ioni-
zation region were considered. The average of the four values was
taken as the mean magnetic flux density in the ionization region.
It is obvious that this permanent magnet could induce a stron-
ger magnetic field in the drift region than that in the ionization-
region magnetic field. The magnetic lines of force were also
approximately perpendicular to the electric lines of force near thewire electrode. Clearly, the magnetic flux density gradually in-
creased from the wire electrode to the cylinder electrode.
3. Influence of magnetic fields on the currents of negative
corona discharges
As seen in Fig. 5, the corona discharge current was greatly en-
hanced by increasing the magnetic flux density in the ionization-
regionmagnetic field. When the magnetic fluxdensity was0.43 Tat
the edges of magnetic strings, the current increased by about 1.5
times under the mean electric field intensity of 4 kV/cm, which isthe ratio of the inter-electrode voltage to the spacing between the
discharge electrode and the collecting electrode. The current in-
creased by about 1.2 times under the mean electric field intensity of
4 kV/cm, when the magnetic flux density was 0.38 T at the edges of
magnetic strings.
However, as seen in Fig. 6, it was inconspicuous of the increase
of corona discharge current in the drift region magnetic field. As an
external cylinder magnet was employed, the discharge current
increased about 25% when the mean magnetic flux density was
0.015 T near the wire electrode.
In order to decrease the magnetic flux density near the dis-
charge electrode, the magnet rings were decreased. The discharge
current was almost unchanged when the mean magnetic flux
density was about 0 T in the ionization region. However, themagnetic flux density was stronger in the drift region under this
condition. It could be concluded that the corona discharge current
could not be enhanced by the Larmor movements of free electrons
in the drift region, i.e., the increase of the discharge current is not
relevant to the lengthening trajectory of free electrons in the wide
drift region.
The inter-electrode region can be divided into two parts as we
know, namely, the ionization region and the drift region. The ion-
ization region occupies only about 0.5% of the whole inter-electrode
Fig. 3. Schematic of experimental apparatus with drift region magnetic field. 1. HV
power supply, 2. HV divider, 3. cylinder electrode, 4. wire electrode, and 5. cylinder
magnet.
Fig. 4. Schematic of the magnetic lines of force and the electric lines of force in thedrift region magnetic field.
Fig. 5. Characteristic curves showing the discharge current as function of inter-elec-
trode mean electric field intensity for the negative corona discharges under different
magnetic field intensities in the ionization-region magnetic field experiment.
Fig. 6. Characteristic curves showing the discharge current as a function of inter-
electrode mean electric field intensity for negative corona discharges under differentmagnetic field intensities in the drift region magnetic field experiment.
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volume, while the drift region occupies about 95.5%. In the current
study, two different applications of the magnetic field have been
designed to produce different influences, respectively, on the ion-
ization region and drift region.
It is obvious that the increase of the corona discharge current is
mainly determined by the magnetic flux density in the ionization
region and is independent of the magnetic flux density in the drift
region. The increase of the discharge current is only due to the
enhanced ionization process in the small ionization region near
discharge electrode, and is not relevant to the lengthening trajec-
tory of free electrons in the drift region.
3.1. Influence of magnetic fields on the free electrons in the
ionization region
In the conventional negative corona discharges, free electrons
move along the electric lines of force due to the Coulomb forces of
the electric field. In the ionization magnetic field, however, the
magnetic lines of force lie perpendicular to the electric lines of force
in the vicinity of the wire electrode. The free electrons are acted
upon both Lorentz and Coulomb forces, hence Larmor movements
are formed.In order to elucidate this process, some correlative numerical
values of Larmor movements were estimated as follows.
The Larmor frequency of free electrons
f Bq2pm
(1)
where B is the magnetic flux density, q is an electronic charge, and
m is electronic mass. In the ionization-region magnetic field, f is
1.21010 rad/s when the magnetic flux density is 0.43 T at theedges of magnetic strings. The period of gyration T thus is about
0.8 1010 s.According to Ref. [15], we can also get the radius of ionization
region and the electric field intensity.
The radius of ionization region
a r0 0:03ffiffiffiffiffi
r0p
(2)
where r0 is the radius of the curvature on the discharge electrode.
So the radius of ionization region is about 7.1104 m.The electric field intensity can be estimated by using the Peek
formula in the ionization region [16]
E 3 106f
T0p
Tp0 0:03
ffiffiffiffiffiffiffiffiffiffiT0p
Tp0a
s !(3)
wherefis the coarseness of surface of the wire electrode,fz0.6; T0is the standard temperature, T0 273 K; p0 is the thermodynamicstandard state pressure,1.013
105 Pa; Tis the real temperature, K;
p is the real pressure, Pa.
Therefore, the electric field intensity is about 1.7 106 V/m inthe ionization region when the magnetic flux intensity is 0.43 T at
the edges of magnetic strings. Besides, when the collision is not
taken into account, the mean velocity can be calculated when a free
electron moves from the surface of wire electrode tothe edge of the
ionization region by the following two Equations:
qE$a 12
mV2 (4)
V 12
V (5)
where Vis the velocity of free electron at the edge of the ionizationregion, and V is its mean velocity, which is about 1.0 107 m/s.
Thus, it will take the free electron about 7.11011 s moving fromthe surface of the wire electrodeto the edge of the ionization region
when the magnetic flux density is 0 T. The moving time of free
electrons will increase in the ionization region when the ioniza-
tion-region magnetic field is applied, and the gyration time is at
least about 0.88 period.
And the radius of gyration
R mVBq
1:3 104 m (6)
According to the above analyses, the moving distance of free
electrons will increase at least by 8.2104 m in the ionizationregion when the free electrons move from the surface of the dis-
charge electrode. Therefore, the number of collisions will increase
to 215.2% and the mean energy of free electrons will decrease by
115.2% between two collisions (an electron free path) for these free
electrons under this condition. In conclusion, the discharge cur-
rents will be enhanced due to the exponential increase of collisions
for all the free electrons in the ionization region.
However, the trajectory of free electrons is very complicated
because of the collisions. In any case, it is certain that the trajectory
of free electrons substantially lengthened and the mean energy offree electrons decreases in the ionization region when the ioniza-
tion-region magnetic field is applied.
3.2. Influence of magnetic fields on the free electrons in
the drift region
In the drift region, the collisions could not promote ionization
because of the lower kinetic energy of free electrons. In addition,
the neutralizations could notoccur because only the negative space
charges (free electrons and negative ions) existed in the drift region
in the magnetically enhanced negative discharges. In the above two
experiments, the number of collisions between free electrons and
gas molecules also increased in the drift inter-electrode region forthe influence of the magnetic field. However, more free electrons
were attached by the gas molecules to form the negative ions in the
drift inter-electrode region. In a word, the charge concentration
increased and the drift velocity along the electric line of force for
both negative ions and free electrons decreased in these two
experiments.
It can also be explained why the increase of the discharge cur-
rents is not relevant to the lengthening trajectory of free electrons
in the wide drift region. We suppose that the output negative
charges from the ionization region are Q within per unit time (t).
Since both the neutralizations of charges and the ionizations are
inexistent in the drift region, all the charges Qshould come into the
collecting electrode in the same unit time according to the principle
of electric current continuity. Therefore, the discharge currentIQ/t, is a fixed value. It is obvious that the increase of the dis-charge currents is not relevant to the lengthening trajectory of free
electrons in the wide drift region, which is in accordance with the
experimental data. The discharge currents cannot be enhanced by
the lengthening trajectories of negative ions as well as that of the
free electrons in the magnetically enhanced negative corona
discharges.
In summary, the mechanism of the magnetic enhancement is
that the magnetic field could affect the ionization region. Therefore,
the corona discharge current was enhanced by the Larmor move-
ments of free electrons in the ionization region, and the space
charge concentration is enhanced in the whole inter-electrode
region. Moreover, the lengthening trajectories of free electrons and
negative ions cannot increase the corona discharge current in thedrift region. Remarkably, to increase the corona discharge current,
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it is important to install the permanent magnet near the discharge
electrode to induce a stronger magnetic flux density.
3.3. Optimum combination between electric field and
magnetic field
In the ionization-region magnetic field, the radius of gyration for
the Larmor movements increases with the mean electric field in-
tensity when the magnetic field remains unchanged. The moving
distance of a free electron consists of both the distance along the
electric line of force and the distance caused by Larmor movement
in an electron mean free path. When the magnetic field was fixed,
the moving distance of a free electron along the electric line of force
will increase with the inter-electrode electric field intensity in ev-
ery electron mean free path. That means the moving distances of
free electrons caused by Larmor movements will decrease with the
increasing inter-electrode electric field intensity in every electron
mean free path when the magnetic field was fixed. Therefore, the
relative increase (magnetically enhanced corona discharge to con-
ventional one) of the collision number between free electrons and
gas molecules should decrease with the enhancing electric field
intensity when the magnetic field remains unchanged. This tendsto restrain the enhancement of ionizations. However, the mean
energy of free electrons will increase with the electric field in-
tensity which tends to enhance ionization.
According to above analyses, it is predicted that the relative
increase of corona discharge current could have a maximum value
at a special point because the change of the relative increase of
collision number is in the opposite direction of that of the mean
energy of free electrons.
The characteristic curves (Fig. 7) were generated by analyzing
the data of the ionization-region magnetic field experiment,
showing the relative increase of discharge current as a function of
the inter-electrode mean electric field intensity for negative corona
discharges under different magnetic flux densities of 0.38 T and
0.43 T. Fig. 7 shows that the relative increase of the discharge cur-rent has a maximum value, which is accordant with our prediction.
The optimum combination between the electric field and the
magnetic field was obtained when the relative increase of the
discharge current is the maximum value. It greatly saves the energy
at this time.
The relative increase of discharge current would exceed 150%,
when the mean electric field intensity is about 4.2 kV/cm and the
magnetic flux density is 0.43 T. The characteristic curve (Fig. 8) was
generated by analyzing the data of the ionization-region magnetic
field experiment, showing the relative increase of current asa function of the magnetic flux density for negative corona dis-
charges under mean electric field intensity of 4 kV/cm, which is the
value for the practical operation of the ESP. According to Fig. 8, the
relative increase of the discharge current could attain the maxi-
mum value by using a proper magnetic field when the mean
electric field intensity is 4 kV/cm. The efficiency of the ESP will be
enhanced at the maximum value in the ionization-region magnetic
field because of the increased concentration of negative ions. The
optimum combination between the mean electric field of 4 kV/cm
and the magnetic field in the ionization region of about 0.43 T is
especially significant in the industrial applications of corona
discharges. Moreover, the relative increase of discharge current
could reach about 150%.
According to the mechanism of the magnetic enhancement, therelative increase of the discharge current is determined by two
factors: (1) The collision number between the free electrons and
the gas molecules in the ionization region; and (2) The mean
energy of free electrons. If the mean energy of free electrons is
beneath the minimum ionization energy of the gas molecules, most
of the gas molecules will not ionize. Under that condition, the
discharge current could not increase even if the collisions between
the free electrons and the gas molecules increase. In contrast, when
the number of the collisions decreases, the discharge current may
not increase even if the mean energy of free electrons exceeds the
minimum ionization energy of the gas molecules.
In the ionization region, besides elastic collisions between the
free electrons and the gas molecules, ionizations, excitations and
attachments are present at the same time. If the mean electric fieldintensity is fixed, the mean energy of the free electrons will
decrease when the magnetic field is used. Therefore, when the
collisions between the free electronsand gas molecules occurin the
ionization region, the probability of excitations and attachments
increases, whereas the probability of ionization collisions decreases
in the magnetically enhanced corona discharges. However, the
number of collisions between the free electrons and gas molecules
increases when the magnetic field is applied.
According to above analyses, the mean energy of the free elec-
trons decreases in the ionization region when the magnetic field is
applied, while the number of the collisions between free electrons
and gas molecules increases. Therefore, the optimum combinations
between the electric fields and magnetic fields may be as follows.
If the mean electric field intensity is fixed, the number ofcollisions between the free electrons and gas molecules will
Fig. 7. Characteristic curves showing the relative increase of current as a function of
inter-electrode mean electric field intensity for negative corona discharges underdifferent magnetic field intensities.
Fig. 8. Characteristic curves showing the relative increase of current as a function
of magnetic flux density for negative corona discharges under mean electric field of
4 kV/cm.
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increase with the magnetic flux density increasing, while the
mean energy of free electrons will decrease with the magnetic
flux density increasing. Initially, due to the increased number of
collisions (a decisive factor), the relative increase of the discharge
current grows with the magnetic flux density. Subsequently, the
relative increase of the discharge current attains a maximum
value when the magnetic flux density is a particular value. Then
the relative increase of the discharge current decreases with the
increase of the magnetic flux density because of the obvious
decreased mean energy of free electrons, which, in turn, becomes
the decisive factor. Thus the relative increase of the discharge
current would have a maximum value with the magnetic flux
density increasing.
Furthermore, if the magnetic flux density is fixed, the mean
energy of free electrons increases with the mean electric field in-
tensity in the ionization region, while the number of the collisions
between the free electrons and gas molecules decreases with the
mean electric field increasing. At first, due to the increased mean
energy of free electrons, which is a decisive factor, the relative in-
crease of the discharge current grows with the mean electric field
intensity. After that, the relative increase of the discharge current
attains a maximum value when the mean electric field intensity is
a particular value. Then the relative increase of the discharge cur-rent decreases with the increasing of the mean electric field
intensity because of the obvious decreased number of collisions,
which becomes decisive factor. Thus, there would be a maximum
value of relative increase of the discharge current with the mean
electric field intensity increasing.
4. Conclusions
In this paper, according to the research on the corona discharges
in the magnetic field, the following conclusions can be established:
(1) The mechanism of the magnetic enhancement is that the
magnetic field could affect the ionization region. Therefore, thecorona discharge current was enhanced by the Larmor move-
ments of free electrons in the ionization region, and the space
charge concentration is enhanced in the whole inter-electrode
region. Moreover, the lengthening trajectories of free electrons
and negative ions cannot increase the discharge current in the
drift region.
(2) The relative increase of the discharge current is much larger
when the permanent magnet is applied near the discharge
electrode than near the collecting electrode.
(3) When the magnetic field is fixed, the relative increases of the
discharge current for varied inter-electrode mean electric fields
have a maximum value in the magnetically enhanced negative
corona discharges.
(4) In order to reach the largest relative increase of the discharge
current under the inter-electrode mean electric field intensity
of 4 kV/cm for a practical ESP, the optimum magnetic field with
a magnetic flux density of about 0.43 T at the edges of magnet
strings should be selected.
(5) The relative increase of the discharge current is determined by
two factors. One is the collision number between the free
electrons and the gas molecules in the ionization region, and
the other is the mean energy of the free electrons. Moreover,
the changecharacteristic of the relative increase of the collision
number is in contrast to that of the mean energy of free elec-
trons, leading to optimum combinations between the electric
fields and the magnetic fields.
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