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7-11-2010
Challenge the future
DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 1
Tim van der HagenDelft University of Technology
vision from 1939
Sustainable Nuclear EnergyWhat are the scientific and technological challenges
of safe, clean and abundant nuclear energy?
7-11-2010
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 2
# NPPs within 500 km
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 3
IEA Energy Technology Perspectives 2008IEA Energy Technology Perspectives 2008June 6, 2008June 6, 2008
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 4
IEA Energy Technology Perspectives 2008IEA Energy Technology Perspectives 2008June 6, 2008June 6, 2008
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 5
• 1932: Discovery of the neutron (Chadwick)
• 1939: Demonstration of nuclear fission(Meitner, Hahn, Strassman)
• 1942 (Dec. 2): First controlled chain reaction in CP1 (Enrico Fermi)
HistoryHistory
• 1951 (Dec. 20): First ‘nuclear’ electricity, EBR-1, Idaho
• 1955 (Jan. 17): First nuclear submarine at sea, Nautilus
• 1954 (June 26): First NPP, Obninsk, USSR (5 MWe)
• 1956: (Aug. 27): First NPP, Calder Hall, UK (50 MWe)
• 1957 (Dec. 2): First PWR, Shipping Port, USA (60 MWe)
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 6
1954: Launching of Nautilus1954: Launching of Nautilus
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Nautilus passes the poleNautilus passes the pole
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 8
Fissioning of 1 gram uranium yields as much energy asburning 2500 liters petrolor 3000 kilograms coal
radioactive
Nuclear fissionNuclear fission
no CO2
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 9
• all electricity in the Netherlands nuclear:0.4 gram uranium fissioned (=waste) per family per year
• in a human life: a volume of 1 billiard ball
• ‘Borssele’ produces 1.3 m3 highly radioactive waste per year, but ‘prevents’ the emission of2 billion kilograms CO2 per year
• a radioactive material emits radiation it clears itself (the more radioactive, the quicker)
Small volumes of material neededSmall volumes of material neededstrategic stock possiblelow amounts of waste
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 10
239Pu
neutron energy / eV
# n
eutr
ons
chain reaction possible
# neutrons released# neutrons releasedper absorption of 1 neutronper absorption of 1 neutron
1 neutronextra!
Neutrons available for• scientific research (Delft)• production of medical isotopes (Petten)• breeding of fuel
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Cross sectionsCross sections(interaction probability)(interaction probability)
Neutrons have to be slowed down (moderated)to keep the chain reaction going
235U 238U
fission
capture
total
fission
total
capture
Neutron energy / eV Neutron energy / eV
(moderator: water, graphite)
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 12
• Fissile isotopes (can be fissioned by neutron absorption):233U, 235U, 239Pu, 241Pu (rare)
• Fissionable isotopes (threshold in neutron energy):232Th, 233Th, 234U , 236U , 238U , 239U , 240Pu, 242Pu …
• Fertile isotopes (can be turned into a fissile isotope):232Th, 238U
fissile fissile –– fissionable fissionable –– fertilefertile
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 13
Production of fissile isotopes (conversion)
extra neutron needed
232 233 233 23390 90 91 9222 3 27
β β. min dTh Th Pa Un − −
⎯⎯⎯⎯⎯→ ⎯⎯⎯⎯→+ →
238 239 239 23992 92 93 9423 5 2 3
β β. min . dU U Np Pun − −
⎯⎯⎯⎯⎯→ ⎯⎯⎯⎯→+ →
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 14
If more fissile isotopes are produced from fertile isotopes than were destroyed in the chain reaction:
breeding
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 15
Moderator
U-238
U-239
Pu-239
Np-239
U-235
Moderator
U-238 Pu-239
U-235
neutron
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Fuel tabletsFuel tablets
Composition of:
5% 235U
95% 238U(0.7% 235U in natural ore)
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FuelFuel assemblyassembly of a PWRof a PWR
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 18
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Energy balance (Energy balance (Life Cycle AnalysisLife Cycle Analysis))(1000 MWe PWR, 80% availability, 40 years of operation)
enrichment with centrifuges:input / output = 1.7 %
energy input (centrifuge)input / output = 1,7 %
1
2
3
4
5
6
7
construction & operation
enrichment
fuel fabrication
conversion
decommis-sioning
waste storage & transport
mining & milling
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 20
CoNi
UTh
AuPtPb
SnAg
Fe Cu
CSiO
Element abundance in earth's crustElement abundance in earth's crust
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 21
• The earth’s crust contains 40 x as much uranium as silver;as much uranium as tin
• Cheap uranium (up to 130$ per kg): 5.5 million tons;enough for 80 years (0.1 ct/kWh)
• For the double price:10 times as much; enough for 800 yearsusing fast reactors: 80,000 years
• Uranium as byproduct from phosphate deposits(22 Mt recoverable)
• Uranium from seawater (450$ per kg): 4 billion tons;enough for 6,000,000 years
Uranium resources:Uranium resources:
Source: OECD NEA & IAEA, “Uranium 2007: Resources, Production and Demand“("Red Book").
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 22
COCO22 productionproduction
0
300
600
900
1200
1500
CO2
(g/k
Wh e
)
kolen olie gas zon PV water bio wind nucleair fusiecoal oil gas solar PV hydro bio wind nuclear fusion
Source: IAEA (2000)
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 23
Source: OECD, “Projected Costs of Generating Electricity”, 2010
Costs of electricity productionCosts of electricity production
assumptions:5% discount rateCO2 price: 30 USD/tonne (plant level, without transport and storage)
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 24
Breakdown of costs ofBreakdown of costs ofnuclear electricity productionnuclear electricity production
0,1 ct/kWhe
0,1 ct/kWhe
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 25
Netherlands
in total 441 NPPs
375 GWe
Nuclear Power Plants in operation
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 26
NuclearNuclear Power Power PlantsPlants
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 27
Status nuclear power plansStatus nuclear power plansJanuary 2008January 2008
0
50
100
150
200
250
300
1 2 3 4 5
gepland (316)
in aanbouw (34)
in bedrijf (439)
Asia Western Eastern N.- and S.- AfricaEurope Europe America
planned (316)construction (34)in operation (439)
now 61 (60 GWe)
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 28
Core cooling is always needed, also after shutdown !
Safety issue:Safety issue:decay heat per MW nominal powerdecay heat per MW nominal power
Dec
ay p
ower
/ M
W
Dec
ay e
nerg
y /
MW
d
Time / day
7-11-2010
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 29
Fuel (pellet and cladding)
Primary system (steel)
Containments(2x concrete + steel)
Safety of nuclear power plantsSafety of nuclear power plantsmultiple barriers to keep radioactive nuclides inside
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 30
spent fuel
95%
4%
1%
uranium
plutonium
fissionproducts
Spent fuel: only 4% is wasteSpent fuel: only 4% is waste
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 31
erts
101 102 103 104 105 106102
103
104
105
106
107
108
109
Rad
ioto
xici
ty (S
v)
Storage time (a)
ActinidesFiss ProdsOre
Rad
ioto
xici
ty/
Sv
fission products(450 kg)
250 years
220,000 years
actinides (Pu, Am)(140 kg)
ore
Time / yearsnumbers: yearly production Borssele
Two sorts of radioactive productsTwo sorts of radioactive products
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 32
FastFast reactors can fission actinides,reactors can fission actinides,like plutoniumlike plutonium
100 102 104 10610-4
10-2
100
102
104
106
108
1010
Energy (eV)
α (σ
fis/ σ
cap)
Pu-239Pu-240Pu-241Pu-242
fiss
ion
pro
babi
lity
neutron energy /eV
7-11-2010
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 33
Radioactive wasteRadioactive waste
450 kg
130 kg
6 kg
uranium13000 kg
plutonium
fissionproducts
other actinides
numbers: yearly production Borssele
Two routes possible:
1) Without reprocessing:● ‘lifetime’ rest products 220,000 year
2) With reprocessing + fast reactors:● ‘lifetime’ waste 500-5,000 years● volume reduced to 4%● up to 100x better use of base material
7-11-2010
Challenge the future
DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 34
Early PrototypeReactors
Generation I
- Shippingport- Dresden, Fermi I- Magnox
Generation II
- LWR-PWR, BWR- CANDU- VVER/RBMK
1950 1960 1970 1980 1990 2000 2010 2020 2030
Generation IV
- Highly Economical
- Enhanced Safety
- Minimal Waste
- Proliferation Resistant
- ABWR- System 80+- AP600- EPR
AdvancedLWRs
Generation III
Gen I Gen II Gen III Gen IV
Evolutionary Designs Offering Improved Economics
Generations of nuclear reactorsGenerations of nuclear reactors
7-11-2010
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 35
Advanced reactors, Generation IIIAdvanced reactors, Generation III
reliable and safe due to:
• redundancy• separation• diversification• less and shorter pipelines• large water volumes
ABWR (in operation since 1995), EPR, ACR1000,System-80+, BWR-90+, KNGR, VVER-91, ...
7-11-2010
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 36
reactor
vessel
turbine buildingreactor building
4 safety buildings4 x 100%
European Pressurized Water ReactorEuropean Pressurized Water Reactor4500 MWth
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 37
– Concrete –– Steel –
– Concrete –
Resistant against the impact of
a large airplane
Double containmentDouble containment
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 38
cooling water
Passively cooled Passively cooled ‘‘Core CatcherCore Catcher’’
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 39
Advanced, evolutionary designs Advanced, evolutionary designs (Generation III(Generation III++))
with ‘passive’ components:
• natural circulation core cooling• convection cooling of the containment• heat removal by radiation
AP1000, ESBWR, SWR-1000, PBMR, HTRM, GT-MHR,APWR, EP-1000, AC-600, MS-600, V-407, V-392, JSBWR,JSPWR, HSBWR, CANDU-6, CANDU-9, AHWR, ...
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 40
AdvancedAdvanced PassivePassive PWRPWR1117 MWe (Westinghouse – VS)
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Passive emergency coolingPassive emergency coolingof the containmentof the containment
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 42
Passive safety due to fewer Passive safety due to fewer components and less pipingcomponents and less piping
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 43
High Temperature ReactorHigh Temperature Reactor generation IIIgeneration III++
AVR (Germany, 1967-1988) – HTTR (Japan, 1999) – HTR10 (China, 2000)
gas turbine
process heat:hydrogen productionwater desalination ...
helium as coolant
inherently safe
7-11-2010
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 44
VHTRVHTR: nuclear e: nuclear e-- plus hydrogen productionplus hydrogen production
Nuclear HeatNuclear HeatHydrogenHydrogen OxygenOxygen
H2O22
1
900 C400 C
Rejected Heat 100 C
Rejected Heat 100 C
S (Sulfur)Circulation
SO2+H2O+O22
1H2SO4
SO2+
H2OH2O
H2
I2
+ 2HI
H2SO4
SO2+H2OH2O
+
+ +
I (Iodine)Circulation
2H I
I2
I2
WaterWater
Nuclear HeatNuclear HeatHydrogenHydrogen OxygenOxygen
H2O22
1 O22121
900 C400 C
Rejected Heat 100 C
Rejected Heat 100 C
S (Sulfur)Circulation
SO2+H2O+O22
1H2SO4
SO2+
H2OH2O
H2
I2
+ 2HI
H2SO4
SO2+H2OH2O
+
+ +
I (Iodine)Circulation
2H I
I2
I2
WaterWater
Idaho 2015 ?
H2O in,O2 and H2 out
eH2
VHTR
7-11-2010
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 45
Commercial PowerReactors
Early PrototypeReactors
Generation I
- Shippingport- Dresden, Fermi I- Magnox
Generation II
- LWR-PWR, BWR- CANDU- VVER/RBMK
1950 1960 1970 1980 1990 2000 2010 2020 2030
Generation IV
- Highly Economical
- Enhanced Safety
- Minimal Waste
- Proliferation Resistant
- ABWR- System 80+- AP600- EPR
AdvancedLWRs
Generation III
Gen I Gen II Gen III Gen IV
Evolutionary Designs Offering Improved Economics
Generations of nuclear reactorsGenerations of nuclear reactors
7-11-2010
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 46
Gen-IV Roadmap
(2002, 97 pages)
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NNV Section Subatomic Physics; November 5, 2010; Lunteren 47
Sustainable Nuclear Energy
Technology Platform
Strategic Research Agenda
(2009, 87 pages)
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 48
The 6 selected reactor concepts
Hydrogen production:
• Very High Temperature Gas Cooled Reactor
Evolution of Light Water Reactors:
• Supercritical Water Cooled Reactor (thermal/fast)
Waste reduction and high efficiency:
• Gas Cooled Fast Reactor
• Sodium Cooled Fast Reactor
• Lead Cooled Fast Reactor
Very innovative:
• Molten Salt Reactor (epithermal)
The The GenerationGeneration--IVIV InitiativeInitiative: sustainable nuclear energyArgentine, Brazil, Canada, France, Japan, South Africa, South Korea,Switzerland, United Kingdom, United States and the European Union
closedfuel cycle
7-11-2010
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 49
U.S. DOE initiativesU.S. DOE initiativesU.S. DOE initiativesAdvanced Fuel Cycle Initiative
• Recovery of energy value from SNF• Reduce the inventory of civilian Pu• Reduce the toxicity & heat of waste• More effective use of the repository
Nuclear Hydrogen Initiative
Develop technologies for economic,commercial-scale generation of hydrogen
Nuclear Power 2010
• Explore new sites• Develop business case• Develop Generation III+ technologies• Demonstrate new licensing process
Generation IV Better, safer, more economic nuclearpower plants with improvements in• safety & reliability• proliferation resistance &
physical protection• economic competitiveness• sustainability
Source: US DOE
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 50
AFCI Approach to Spent Fuel ManagementAFCI Approach to Spent Fuel Management
Once ThroughFuel Cycle
Direct Disposal
SpentFuel
U and PuActinidesFission Products
Repository
ConventionalReprocessing
PUREX
Pu UraniumMOX
LWRs/ALWRs
Interim Storage
less U and PuActinides
Fission Products
CurrentEuropean/Japanese
Fuel Cycle
Advanced RecyclingClosed Fuel Cycle
+ ADS Transmuter?
Trace U and PuTrace Actinides !less Fission Products
Repository
Gen IV Fast Reactors
Advanced RecyclingClosed Fuel Cycle
Gen IV Fuel Fabrication
LWR/ALWR/HTGR
Advanced Separations Technologies
Source: US DOE
Spent Fuel FromCommercial Plants
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DelftUniversity ofTechnology
NNV Section Subatomic Physics; November 5, 2010; Lunteren 51
Research themes GenResearch themes Gen--IVIV
• fuel (fast reactors, transmutation, high burn-up, thorium cycle …)
• materials (corrosion, embrittlement, radiation damage, high temperatures)
• heat transport
• multiphase flows
• neutron data (cross sections of materials)
• chemical treatment of spent fuel
• core design
• system design (safety, efficiency, flexibility, …)
• safety (decay heat removal)
• coupling nuclear heat – process heat (hydrogen production)
• gas turbines
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• large scale
• no CO2, no air pollution
• security of supply
• economical competitive
Positive Negative
• radioactive waste
• acceptance (safety)
• large investment
• proliferation
ResumResuméé nuclear energynuclear energy
savings, clean fossil and nuclear energy are now necessary to give renewables a chance