in situ measurements of aerosol size distributions inside the … · 2016-03-29 · in situ...

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In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone Ru-Shan Gao, Hagen Telg, Pengfei Yu, and Karen Rosenlof NOAA Earth System Research Laboratory Jianchun Bian, Zhixuan Bai, Dan Li, Yunjun Duan Lageo, Institute of Atmospheric Physics, Chinese Academy of Sciences March 9, 2016 Asian Monsoon Workshop NCAR

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Page 1: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

In situ measurements of aerosol size

distributions inside the Asian Summer

Monsoon Anticyclone

Ru-Shan Gao, Hagen Telg, Pengfei Yu, and Karen Rosenlof

NOAA Earth System Research Laboratory

Jianchun Bian, Zhixuan Bai, Dan Li, Yunjun Duan

Lageo, Institute of Atmospheric Physics, Chinese Academy of

Sciences

March 9, 2016

Asian Monsoon Workshop NCAR

Page 2: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

POPS description:

Size range: 140 – 3000 nm diameter (dry)

Sampling: 3 cm3 s-1

Weight: 1 kg

Communication:

8 size bins with O3,

CFH, COBALD (limited

by the iMet bandwidth)

POPS

Page 3: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

The Institute for Atmospheric Physics/Chinese Academy of Science Long Trek VII

UAS

- POPS integration and test flights in November 2015

Page 4: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

UAS implementation

The NOAA Pacific Marine Environment Laboratory (PMEL) Manta UAS

- POPS and ULR have been fully integrated

- Successful test flights in January 2015

- First field mission in April 2015 – Svalbard, Norway in collaboration with

PMEL

The University of Colorado Pilatus UAS

- POPS integration in February 2015

- Test flight in March 2015

- First field mission in April 2015 – Oliktok Point, AK in collaboration with Dept.

of Energy, University of Colorado, and Physical Sciences Division (PSD)

The Laboratory for Atmosphere and Cyclone (LACy, Reunion, France) R2 Drone

- POPS integration right now

- Test flight in this month

- First field mission in Indian Ocean

in collaboration with LACy

Page 5: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

POPS (optical particle counter) and miniSASP (sun photometer):

Aerosol optical density and hygroscopicity

Page 6: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

miniSASP (sun photometer

POPS (optical particle counter)

ECC ozone sensor

Total weight = 5.6 lbs.

2.1 m

Instrumented auto-homing glider (Skywalker X8)

Flight control by Black Swift Technologies

Autopilot Tablet UI Ground station

Page 7: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

COBALD

O3

CFH

POPS (Printed

Optical

Particle

Spectrometer)

iMet

Page 8: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

Aug 13, 2015: NCEP 100 mb hgt

Balloon measurements Balloon measurements

Kunming, China

Asian summer monsoon anticyclone

Page 9: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

Aug 14, 2015: NCEP 100 mb hgt

Balloon measurements

Kunming, China

Asian summer monsoon anticyclone

Page 10: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone
Page 11: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone
Page 12: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone
Page 13: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

Aug 17, 2015: NCEP 100 mb hgt

Asian summer monsoon anticyclone

Balloon measurements Balloon measurements

Kunming, China

Page 14: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

Ascent data, 200-m average

8006004002000

Aerosol concentration (# cm-3

)

Flt 3, 2015 08 17

12008004000

Aerosol concentration (# cm-3

)

Flt 2, 2015 08 14 Total 98 - 144 nm 144 - 179 nm 179 - 231 nm 231 - 360 nm CPT

30

25

20

15

10

5

Altitu

de

(km

)

10008006004002000

Aerosol concentration (# cm-3

)

Flt 1, 2015 08 13

Page 15: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

20

18

16

14

12

10

Altitud

e (

km

)

403020100 403020100

Particle concentration (# cm-3

)

403020100

252015105 252015105

455 nm backscatter ratio

252015105

Kunming PC CPT Houston PC Backscatter

13 August 2015 14 August 2015 17 August 2015

Ascent data, 200-m average

ATAL is a great UT air tracer in the LS

Page 16: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

Size distribution 2015 08 13

10-4

10-3

10-2

10-1

dN

/dlo

g(D

p)

1002 3 4 5 6 7 8 9

10002

Dp (nm)

15 - 17 km 17 - 19 km

Particles were likely formed in the UT

Page 17: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

Flt 2, 2015 08 14

T, O3, and WV

Page 18: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

20

19

18

17

16

15

Altitu

de

(km

)

161412108642

Aerosol concentration (# cm-3

)

01 August 1996 08 August 1996 Cold point

STRAT data

Page 19: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

20

19

18

17

16

15

Altitu

de

(km

)

14121086420

Aerosol concentration (# cm-3

)

03 August 2007 05 August 2007 06 August 2007 08 August 2007 09 August 2007 Cold point

TC4 data

Page 20: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

• In a general sense the ATAL is NOT unique!

- Brock et al., Science (1995)

• The air in the ASMA, similar to the air in the tropics,

is trapped and moving upward slowly.

• Condensables have sufficient time to form new

particles or condense on existing particles.

• Tropical aerosol layer too thin to be detected by

satellites?

Page 21: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

35

30

25

20

15

10

5

0

Altitud

e (

km

)

1086420

O3 (ppm)

Hilo Tsukuba Kunming

Page 22: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

36

34

32

30

28

26

24

Altitud

e (

km

)

1086

O3 (ppm)

Hilo Tsukuba Kunming

O3 is significantly higher above ~26 km

Page 23: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

19

18

17

16

Altitud

e (

km

)

0.80.60.40.20.0

O3 (ppm)

Hilo Tsukuba Kunming

O3 is significantly lower ~16-18 km

Page 24: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

Ascent

Mixing

Tropopause

Strat

air

Tropo

air

A crude mixing model:

• Ascent rate determined

by the local heating rate

and local thermal structure

• Particles = Trop. tracer

• O3 = Strat. tracer

• Mixing in strat can be

derived from these three.

(Arguably ascent is easier

to calculate than mixing) O3 poor, particle rich

O3 rich, particle poor

Page 25: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone

Conclusions

1) ATAL appears to be robust feature

2) The particle enhancement has implications (additional

heating)

3) In the ASMA LS these particles are a good tracer of the

tropospheric air

- Size distributions suggest formation/growth in UT

- Tropospheric air is moving up into stratosphere

4) ATAL is similar to the tropical aerosol layer

5) Measureable mixing tracers: O3 and aerosol

6) A crude model may be useful for LS mixing rate

Page 26: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone
Page 27: In situ measurements of aerosol size distributions inside the … · 2016-03-29 · In situ measurements of aerosol size distributions inside the Asian Summer Monsoon Anticyclone