thz makes x-ray · 2012. 8. 7. · thz workshop, argonne national laboratory, july 30-31, 2012 1...
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THz Workshop, Argonne National Laboratory, July 30-31, 2012
1
János [email protected]
Gábor Almási, József Fülöp, Mechler Mechler, László Pálfalvi,
Zoltán Ollmann, Zoltán Tibai, György Tóth
University of Pécs, Institute of Physics
THz makes X-Ray
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MotivationVelocity matching by tilting of the pump-pulse-front
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MotivationComparison of THz pulse generation by ZnTe and by LN
Field strength of focused pulses: 0.2 – 1.2 MV/cm
125 J
THz p – p, 2 J
10 100 1000 10000 1000001E-4
1E-3
0,01
0,1
1
10
100
1000
10000
100000TH
z pu
lse
ener
gy (n
J)
Pump pulse energy (J)
ZnTe
LiNbO3 tilted pulse front excitation
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Linear (TDTS) THz spectroscopy (Emax ≈ 100 V/cm → 10 fJ energia)
High field THz pulses (Emax ≈ 100 kV/cm → µJ energia)
0 1 2 30,0
0,2
0,4
0,6
0,8
1,0
-2 0 2 4 6 8
-0,5
0,0
0,5
1,0
Spe
ctra
l am
plitu
de (a
. u.)
Frequency (THz)
Ele
ctric
fiel
d (a
. u.)
time (ps)
Emax
MotivationClassification of THz pulses by peak electric field (energy)
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Applications of high energy THz pulses
• Nonlinear THz optics (self-phase-modulation, Kerr-effect)
• Nonlinear THz spectroscopy (THz pump - probe)
• Electron wave packet sampling (streaking)Frühling: Nature Photonics 3, 523 (2009)
Schütte et al.: Opt. Express 19, 18833 (2011)
• Alignment/orientation of moleculesStapelfeldt, Seideman: Rev. Mod. Phys. 75, 543 (2003)
Fleischer et al.: Phys. Rev. Lett. 107, 163603 (2011)
Kitano et al.: PRA 84, 053408 (2011)
• „Single-shot” THz imaging
• „Single-shot” THz multi spectral imaging
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Linear (TDTS) THz spectroscopy (Emax ≈ 100 V/cm → 10 fJ energia)
High field THz pulses (Emax ≈ 100 kV/cm → µJ energia)
Extreme high field THz pulses(Emax ≈ 100 MV/cm → 10 mJ pulse energy)
0 1 2 30,0
0,2
0,4
0,6
0,8
1,0
-2 0 2 4 6 8
-0,5
0,0
0,5
1,0
Spe
ctra
l am
plitu
de (a
. u.)
Frequency (THz)
Ele
ctric
fiel
d (a
. u.)
time (ps)
Emax
MotivationClassification of THz pulses by peak electric field (energy)
Tomorrow: Alan Fischer: 500 J, József Fülöp: 125 J
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Application possibilities of THz pulses having extreme high electric field strength
• Increasing the cut-off frequency of HHG (ETHz = 20 ÷ 80 MV/cm)
• Quasi-phase-matched attosecond pulse generation (ETHz = 2 ÷ 6 MV/cm)
• Temporal compression of electron bunches by THz pulses
• Single-cycle (or shaped) pulse generation on the 50 nm – 400 nm
wavelength range by coherent Thomson-scattering
• Ultrashort X-ray pulse generation by incoherent Thomson-scattering
• THz driven undulator for UV – X-ray generation
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HHG in the presence of THz electric field
Combined THz + IR fields
THz broken the symmetry of IR field
Hong et al., Opt. Expr. 2009
One as pulse per IR cycle
Spectrum consists both odd and even harmonics
Lewenstein, PRA 1994
tEtEtE THzIR coscos)( 10
0THz
Elec
tric
field
Time
IR
Increasing the cut-off frequency of HHG
E. Balogh et al.: Phys. Rev. A (2011), University of Szeged
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1560 nm
IIR = 2 × 1014 W cm-2 EIR = 388 MV/cm
ETHz = 0 … 40 MV/cm
800 nm
Increasing the cut-off frequency of HHG
Both odd and even harmonics only one as pulse per IR period
E. Balogh et al.: Phys. Rev. A (2011), University of Szeged
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C. Serrat, J. Biegert: Phys. Rev. Lett. 104, 073901 (2010)
Quasi-phase-matched attosecond pulse generationSpatially periodically modulated mid-IR (CO2 laser)
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5 fs, 800 nm, Neon, 20 mbar, L=2mm
Quasi-phase-matched attosecond pulse generation
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Quasi-phase-matched attosecond pulse generationSpatial modulation by (chirped) THz pulse
K. Kovács et al.: Phys. Rev. Lett. 108, 193903 (2012)
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Quasi-phase-matched attosecond pulse generationSpatial modulation by (chirped) THz pulse
ETHz = 2 ÷ 6 MV/cm, WTHz = 2 ÷ 20 mJ
250 times enhancement around the cut-off frequency
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Single-cycle MIR – EUV pulse generation by „coherent” Thomson-scattering
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Single-cycle MIR – EUV pulse generation by „coherent”Thomson-scattering
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A. E. Kaplan, A. L. Pokrovsky: Optics Express 17, 6194 (2009)
Temporal compression of electron bunches
= 1 m, tf = 30 zs
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THz Workshop, Argonne National Laboratory, July 30-31, 2012
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THz Workshop, Argonne National Laboratory, July 30-31, 2012
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Creation of ultrashort electron bunches by inverse-FEL
-0.5 -0.4 -0.3 -0.2 -0.1 0.0 0.1 0.2 0.3 0.4 0.5
60
62
64
-0.5 -0.4 -0.3 -0.2 -0.1 0.0 0.1 0.2 0.3 0.4 0.50
50
100
150
parti
cles
Z (m)
FWHM : 22 nmparticle charge: 0.48 fC
-0.5 -0.4 -0.3 -0.2 -0.1 0.0 0.1 0.2 0.3 0.4 0.5-0.4
-0.2
0.0
0.2
0.4
Y (m
m)
Simulation by GPT
parameters of e-bunch:J. F. Yang: Jap. J. Appl. Phys. 44, 12 (2005)
= 62, E/E = 0.04 %,
Qb = 1 nC, tb = 1.8 ps,
n = 3.2 mm
wiggler: one-period, K = 1
laser:
= 1.3 m, P = 3.9 TW
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0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.00
10
20
30
40
50
60
0
5
10
15
20
25
30
35
Compressed bunch FWHMFW
HM
[nm
]
K
"Temporal" focal length
S [c
m]
Creation of ultrashort electron bunches by inverse-FEL
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0 20 40 60 80 100 120 140 1600
10
20
30
40
50
60
70
80
0
2
4
6
8
10
12
14
16
FWH
M [n
m]
E [GV/m]
Compressed bunch FWHM "Temporal" focal length
S [c
m]
Creation of ultrashort electron bunches by inverse-FEL
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Creation of ultrashort electron bunches by inverse-FEL
0.0 0.1 0.2 0.3 0.40
10
20
30
40
50
60
70
80
90
100
FWH
M [n
m]
[%]
= 62
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3
03
0 4)1(
4
RR
RRRq
RR
RRqE
BvqEqtp
dd
nm 85
pJ 15E 70
THz 3.0
MV/cm 30
EUV
EUV
THz
THZE
nm 65
pJ 128E120
THz 1.0MV/cm 10
EUV
EUV
THz
THZE
Single-cycle EUV pulse generation by coherent Thomson-scattering
0 100 200 3000.0
0.2
0.4
0.6
0.8
1.0
-0.4 -0.2 0.0 0.2 0.4 0.6 0.8
-40
-20
0
20
40
60
80
100
Wavelength (nm)
maximum at 65 nm
Inte
nsity
spe
ctru
m
EUV THz/100
Elec
tric
field
stre
ngth
(kV/
cm)
Time (fs)
= 120
-3 -2 -1 0 1 2 3
-3
-2
-1
0
1
2
3
EEUV = 128 pJ
= 120
X (mm)
Y (m
m)
0.0000.10000.20000.30000.40000.50000.60000.70000.80000.90001.0001.1001.2001.3001.4001.5001.600
at 8 m
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Three-cycle EUV pulse generation by coherent Thomson-scattering
-1.5 -1.0 -0.5 0.0 0.5 1.0 1.5
-1.5
-1.0
-0.5
0.0
0.5
1.0
1.5
EEUV = 17 pJ
X position (mm)
Y po
sitio
n (m
m)
0.0000.020000.040000.060000.080000.10000.12000.14000.16000.18000.20000.22000.24000.26000.28000.30000.32000.34000.36000.3800
= 100
3 cycles
0 100 200 3000.0
0.2
0.4
0.6
0.8
1.0
-0.5 0.0 0.5 1.0
-20
-10
0
10
20
Wavelength (nm)
max. at 79 nm
EUV THz/100
Ele
ctric
fiel
d (k
V/c
m)
Time (fs)
= 100
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3 Å X-ray source by incoherent Thomson-scattering
Electron bunch: Q = 50 pC, = 800, t = 20 fs Leemans et al.: N. Phys. 2, 696 (2006)
THz pulse: E = 6 MV/cm, = 750 m, N = 20, t = 12.5 ps, W = 24 mJ
X-ray: = 3 Å, t = 20 fs, W = 5 nJ
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Plettner et al.: Phys. Rev. Spec. Top. – Accel. and Beams 9, 111301 (2006) acceleration11, 030704 (2008) undulator
12, 101302 (2009) deflection, focusing
Electron manipulation by THz pulses
1 GV/m = 10 MV/cm peak field strength is needed!
Laser-plasma accelerator
THz beam
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Summary
improving attosecond pulse generation
generation single-cycle or prescribed shaped EUV – VIS pulse generation
ultrashort X-ray pulse generation
more detailed numerical modeling
experimental implementation
these are only the first examples (orientation of molecules, accelerating molecules, or nanostructures, etc.)
Acknowledgement: Hungarian Scientific Research Fund (OTKA), grant number 76101, 78262, 101846, SROP-4.2.1.B-10/2/KONV-2010-0002, and hELIos ELI_09-01-2010-0013
According to simple estimation and numerical simulations, -because of their appropriate wavelength and field strength-, extreme intense THz pulses are suitable for:
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70 80 90 100 110 120 130 140
40
80
120
160
200
240
Wav
elen
gth
(nm
)
Result of simulation for compressed bunches Theoretical limit
Single-cycle EUV pulse generation by coherent Thomson-scattering
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Quasi-phase-matched attosecond pulse generationSpatial modulation by (chirped) THz pulse
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0.1
1
10
100
0 100 200 300 400 500
0 100 200 300 400 500
0
1
2
3
4
5
Pump energy (J)
THz
puls
e en
ergy
(nJ)
Tilted pulse Line focus
Effi
cien
cy (1
0-4)
Pump energy (J)
Tilted pulse
ETHz = 240 nJ, ηph = 10 %, electric field (unfocused) 0.1 MV/cm
Opt. Express 13, 5762 (2005)
Scaling-up the THz pulse energy
Spot diameter: 1 mm
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THz driven undulator for UV – X-ray generation
J. Hebling et al.: arXiv 1109.6852 (2011)
u= 600 m, ETHZ= 40 MV/cm, K= 0.747, Q = 420 pC, L= 7 m, T= 30 m
21
2
2
2
Kur
22 mcEeK THzu
33/23
3/23
3)1(
II
KL ATu
G
6/5uGL
6u
2/3 T
WTHz = 14 J !!
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Primary sourcesPeak
/average power
Repetition rate
Pulse Energy
Pulse Duration Spectral Range Secondary sources
ALPS-WB 2-3TW / 300-500W 100kHz 3-5mJ 1.5-3fs 0.3-1.3μm
-T0 FIR/THz 0.3-3THz, 100µm-1mm, 1.24-12.4meV / 0.1-1 mJ, 10-30 MV/cm-T1 MIR 3-30THz, 10-100µm, 12.4-124meV / 10-100μJ, 3-300 MV/cm-T2 NIR 30-300THz, 1-10µm, 0.12-1.24eV / >100μJ, 0.3-30 GV/cm; as an alternative an IR OPCPA system can provide similar parameters-P1 UV/XUV 1-25PHz, 12-300nm 4-100eV / 100-10nJ-P2 SXR 25-100PHz, 3-12nm,100-400eV / >1nJ
SYLOS (Single-cycle
OPCPA System)
100TW / 300-
1000W1kHz 0.3-1J 3-5fs 0.5-1.3μm
-S1 10-100eV, 12-120nm / 100-1µJ -S2 100-1000eV, 1.2-12nm / 1-0.1µJ -H1 1-10keV, 0.12-1.2nm / 100-1nJ -H2 10-100keV, 0.12-1.2A / >1nJ
ALPS-HF1-3PW / 10-100W (>2PW / >400W)
1-10Hz(10Hz)
3-10J(>40J)
3-5fs(<20fs)
0.5-1μm/ 0.7-1.3µm
(0.7-0.9μm)
Controlled electric field: (3-5)x1014 V/mNormalized vector potential: 60-110/80-140 Peak intensity: (1-3)x1022 W/cm2
Ponderomotive potential: (0.6-2)x1022 / (1-3)x1022 W/cm2 × μm2
ELI-ALPS light sources
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Conversion efficiency depends on:
• ωTHz (η ~ ω2THz)
• material parameters
• phase-matching velocity matching:ph
THzgrvis vv
2
2
320
222
4
4sinh
2exp2
L
LL
cnnILd
THz
THz
THz
THzv
effTHz
THzL << 1
THzL >> 1
320
2222cnn
ILd
THzv
effTHz
3220
228cnn
Id
THzTHzv
effTHz
Optical rectification
THzv
effNA nn
LdFOM 2
22
22
24
THzTHzv
effA nn
dFOM
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grnmn800 THzn
grmn 55.1
THzMaterial deff
(pm/V) (cm-1)FOM
(pm2cm2/V2)
CdTe 81.8 3.24 2.81 4.8 11.0
GaAs 65.6 4.18 3.59 3.56 0.5 4.21
GaP 24.8 3.67 3.34 3.16 0.2 0.72
ZnTe 68.5 3.13 3.17 2.81 1.3 7.27
GaSe 28.0 3.13 3.27 2.82 0.5 1.18
sLiNbO3sLN 100K
168 2.25 4.96 2.18 174.8
18.248.6
DAST 615 3.39 2.58 2.25 50 41.5
Velocity matching condition: THzgrNIR
phTHz
grNIR nnvv
Figure of merits (FOMs) supposing 2 mm long crystals
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37fs laser
lens
Fülöp & Hebling,in: Recent Optical and Photonic Technologies, 2010
~100 fs typical
ddtan
gnn
pulse front tilt
angular dispersion
Tilted-Pulse-Front Pumping (TPFP) Setup